On the Nonlinear Response of Lower Stratospheric Ozone to NOx and CIOx Perturbations for Different CH4 Sources

The impact of sulfate aerosol, ClOx and NOx perturbations for two different magnitudes of CH4 sources on lower stratospheric ozone is studied by using a heterogeneous chemical system that consists of 19 species belonging to 5 chemical families （oxygen, hydrogen, nitrogen, chlorine and carbon）. The r...

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Published in:Advances in atmospheric sciences 2006, Vol.23 (5), p.750-757
Main Author: 王革丽 杨培才
Format: Article
Language:English
Subjects:
大气臭氧层
平流层
气溶胶
灾变说
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creator 王革丽 杨培才
description The impact of sulfate aerosol, ClOx and NOx perturbations for two different magnitudes of CH4 sources on lower stratospheric ozone is studied by using a heterogeneous chemical system that consists of 19 species belonging to 5 chemical families （oxygen, hydrogen, nitrogen, chlorine and carbon）. The results show that the present modeled photochemical system can present several different solutions, for instance, periodic states and multi-equilibrium states appearing in turn under certain parameter domains, through chlorine chemistry and nitrogen chemistry together with sulfate aerosol as well as the increasing magnitude of CH4 sources. The existence of catastrophic transitions could produce a dramatic reduction in the ozone concentration with the increase of external sources.
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subjects 大气臭氧层
平流层
气溶胶
灾变说
title On the Nonlinear Response of Lower Stratospheric Ozone to NOx and CIOx Perturbations for Different CH4 Sources
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