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Imaging the Breakdown and Restoration of Topological Protection in Magnetic Topological Insulator MnBi 2 Te 4
Quantum anomalous Hall (QAH) insulators transport charge without resistance along topologically protected chiral 1D edge states. Yet, in magnetic topological insulators to date, topological protection is far from robust, with zero-magnetic field QAH effect only realized at temperatures an order of m...
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Published in: | Advanced materials (Weinheim) 2024-06, Vol.36 (24), p.e2312004 |
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creator | Li, Qile Di Bernardo, Iolanda Maniatis, Johnathon McEwen, Daniel Dominguez-Celorrio, Amelia Bhuiyan, Mohammad T H Zhao, Mengting Tadich, Anton Watson, Liam Lowe, Benjamin Vu, Thi-Hai-Yen Trang, Chi Xuan Hwang, Jinwoong Mo, Sung-Kwan Fuhrer, Michael S Edmonds, Mark T |
description | Quantum anomalous Hall (QAH) insulators transport charge without resistance along topologically protected chiral 1D edge states. Yet, in magnetic topological insulators to date, topological protection is far from robust, with zero-magnetic field QAH effect only realized at temperatures an order of magnitude below the Néel temperature T
, though small magnetic fields can stabilize QAH effect. Understanding why topological protection breaks down is therefore essential to realizing QAH effect at higher temperatures. Here a scanning tunneling microscope is used to directly map the size of exchange gap (E
) and its spatial fluctuation in the QAH insulator 5-layer MnBi
Te
. Long-range fluctuations of E
are observed, with values ranging between 0 (gapless) and 70 meV, appearing to be uncorrelated to individual surface point defects. The breakdown of topological protection is directly imaged, showing that the gapless edge state, the hallmark signature of a QAH insulator, hybridizes with extended gapless regions in the bulk. Finally, it is unambiguously demonstrated that the gapless regions originate from magnetic disorder, by demonstrating that a small magnetic field restores E
in these regions, explaining the recovery of topological protection in magnetic fields. The results indicate that overcoming magnetic disorder is the key to exploiting the unique properties of QAH insulators. |
doi_str_mv | 10.1002/adma.202312004 |
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, though small magnetic fields can stabilize QAH effect. Understanding why topological protection breaks down is therefore essential to realizing QAH effect at higher temperatures. Here a scanning tunneling microscope is used to directly map the size of exchange gap (E
) and its spatial fluctuation in the QAH insulator 5-layer MnBi
Te
. Long-range fluctuations of E
are observed, with values ranging between 0 (gapless) and 70 meV, appearing to be uncorrelated to individual surface point defects. The breakdown of topological protection is directly imaged, showing that the gapless edge state, the hallmark signature of a QAH insulator, hybridizes with extended gapless regions in the bulk. Finally, it is unambiguously demonstrated that the gapless regions originate from magnetic disorder, by demonstrating that a small magnetic field restores E
in these regions, explaining the recovery of topological protection in magnetic fields. The results indicate that overcoming magnetic disorder is the key to exploiting the unique properties of QAH insulators.</description><identifier>ISSN: 0935-9648</identifier><identifier>EISSN: 1521-4095</identifier><identifier>DOI: 10.1002/adma.202312004</identifier><identifier>PMID: 38402422</identifier><language>eng</language><publisher>Germany</publisher><ispartof>Advanced materials (Weinheim), 2024-06, Vol.36 (24), p.e2312004</ispartof><rights>2024 The Authors. Advanced Materials published by Wiley‐VCH GmbH.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c622-d69669ba7242b993dbd3c70cde105fe63b6b3091f4ac52912586b17c4dfc09e3</cites><orcidid>0000-0003-0711-8514 ; 0000-0001-8054-5470 ; 0000-0002-5157-7737 ; 0000-0001-8253-8741 ; 0000-0002-8334-2465 ; 0000-0001-6183-2773 ; 0000-0002-1782-0756 ; 0000-0002-2364-5544 ; 0000-0001-7374-1692 ; 0000-0001-9455-5901</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38402422$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Li, Qile</creatorcontrib><creatorcontrib>Di Bernardo, Iolanda</creatorcontrib><creatorcontrib>Maniatis, Johnathon</creatorcontrib><creatorcontrib>McEwen, Daniel</creatorcontrib><creatorcontrib>Dominguez-Celorrio, Amelia</creatorcontrib><creatorcontrib>Bhuiyan, Mohammad T H</creatorcontrib><creatorcontrib>Zhao, Mengting</creatorcontrib><creatorcontrib>Tadich, Anton</creatorcontrib><creatorcontrib>Watson, Liam</creatorcontrib><creatorcontrib>Lowe, Benjamin</creatorcontrib><creatorcontrib>Vu, Thi-Hai-Yen</creatorcontrib><creatorcontrib>Trang, Chi Xuan</creatorcontrib><creatorcontrib>Hwang, Jinwoong</creatorcontrib><creatorcontrib>Mo, Sung-Kwan</creatorcontrib><creatorcontrib>Fuhrer, Michael S</creatorcontrib><creatorcontrib>Edmonds, Mark T</creatorcontrib><title>Imaging the Breakdown and Restoration of Topological Protection in Magnetic Topological Insulator MnBi 2 Te 4</title><title>Advanced materials (Weinheim)</title><addtitle>Adv Mater</addtitle><description>Quantum anomalous Hall (QAH) insulators transport charge without resistance along topologically protected chiral 1D edge states. Yet, in magnetic topological insulators to date, topological protection is far from robust, with zero-magnetic field QAH effect only realized at temperatures an order of magnitude below the Néel temperature T
, though small magnetic fields can stabilize QAH effect. Understanding why topological protection breaks down is therefore essential to realizing QAH effect at higher temperatures. Here a scanning tunneling microscope is used to directly map the size of exchange gap (E
) and its spatial fluctuation in the QAH insulator 5-layer MnBi
Te
. Long-range fluctuations of E
are observed, with values ranging between 0 (gapless) and 70 meV, appearing to be uncorrelated to individual surface point defects. The breakdown of topological protection is directly imaged, showing that the gapless edge state, the hallmark signature of a QAH insulator, hybridizes with extended gapless regions in the bulk. Finally, it is unambiguously demonstrated that the gapless regions originate from magnetic disorder, by demonstrating that a small magnetic field restores E
in these regions, explaining the recovery of topological protection in magnetic fields. The results indicate that overcoming magnetic disorder is the key to exploiting the unique properties of QAH insulators.</description><issn>0935-9648</issn><issn>1521-4095</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNpVkMtOAjEYhRujEUS3Lk1fYPDvZQpdCvFCAtEo-0lvM1ZnWtKOMb69IEri6izOJScfQpcExgSAXivbqTEFyggF4EdoSEpKCg6yPEZDkKwspODTATrL-Q0ApABxigZsyoFySoeoW3Sq8aHB_avDs-TUu42fAatg8bPLfUyq9zHgWON13MQ2Nt6oFj-l2Dvz4_iAV6oJrvfmX2QR8kertgN4FWYeU7x2mJ-jk1q12V386gi93N2u5w_F8vF-Mb9ZFkZQWlghhZBaTbYXtZTMasvMBIx1BMraCaaFZiBJzZUpqSS0nApNJobb2oB0bITG-1WTYs7J1dUm-U6lr4pAtaNW7ahVB2rbwtW-sPnQnbOH-B8m9g3dBGjI</recordid><startdate>202406</startdate><enddate>202406</enddate><creator>Li, Qile</creator><creator>Di Bernardo, Iolanda</creator><creator>Maniatis, Johnathon</creator><creator>McEwen, Daniel</creator><creator>Dominguez-Celorrio, Amelia</creator><creator>Bhuiyan, Mohammad T H</creator><creator>Zhao, Mengting</creator><creator>Tadich, Anton</creator><creator>Watson, Liam</creator><creator>Lowe, Benjamin</creator><creator>Vu, Thi-Hai-Yen</creator><creator>Trang, Chi Xuan</creator><creator>Hwang, Jinwoong</creator><creator>Mo, Sung-Kwan</creator><creator>Fuhrer, Michael S</creator><creator>Edmonds, Mark T</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0003-0711-8514</orcidid><orcidid>https://orcid.org/0000-0001-8054-5470</orcidid><orcidid>https://orcid.org/0000-0002-5157-7737</orcidid><orcidid>https://orcid.org/0000-0001-8253-8741</orcidid><orcidid>https://orcid.org/0000-0002-8334-2465</orcidid><orcidid>https://orcid.org/0000-0001-6183-2773</orcidid><orcidid>https://orcid.org/0000-0002-1782-0756</orcidid><orcidid>https://orcid.org/0000-0002-2364-5544</orcidid><orcidid>https://orcid.org/0000-0001-7374-1692</orcidid><orcidid>https://orcid.org/0000-0001-9455-5901</orcidid></search><sort><creationdate>202406</creationdate><title>Imaging the Breakdown and Restoration of Topological Protection in Magnetic Topological Insulator MnBi 2 Te 4</title><author>Li, Qile ; Di Bernardo, Iolanda ; Maniatis, Johnathon ; McEwen, Daniel ; Dominguez-Celorrio, Amelia ; Bhuiyan, Mohammad T H ; Zhao, Mengting ; Tadich, Anton ; Watson, Liam ; Lowe, Benjamin ; Vu, Thi-Hai-Yen ; Trang, Chi Xuan ; Hwang, Jinwoong ; Mo, Sung-Kwan ; Fuhrer, Michael S ; Edmonds, Mark T</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c622-d69669ba7242b993dbd3c70cde105fe63b6b3091f4ac52912586b17c4dfc09e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Qile</creatorcontrib><creatorcontrib>Di Bernardo, Iolanda</creatorcontrib><creatorcontrib>Maniatis, Johnathon</creatorcontrib><creatorcontrib>McEwen, Daniel</creatorcontrib><creatorcontrib>Dominguez-Celorrio, Amelia</creatorcontrib><creatorcontrib>Bhuiyan, Mohammad T H</creatorcontrib><creatorcontrib>Zhao, Mengting</creatorcontrib><creatorcontrib>Tadich, Anton</creatorcontrib><creatorcontrib>Watson, Liam</creatorcontrib><creatorcontrib>Lowe, Benjamin</creatorcontrib><creatorcontrib>Vu, Thi-Hai-Yen</creatorcontrib><creatorcontrib>Trang, Chi Xuan</creatorcontrib><creatorcontrib>Hwang, Jinwoong</creatorcontrib><creatorcontrib>Mo, Sung-Kwan</creatorcontrib><creatorcontrib>Fuhrer, Michael S</creatorcontrib><creatorcontrib>Edmonds, Mark T</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><jtitle>Advanced materials (Weinheim)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Qile</au><au>Di Bernardo, Iolanda</au><au>Maniatis, Johnathon</au><au>McEwen, Daniel</au><au>Dominguez-Celorrio, Amelia</au><au>Bhuiyan, Mohammad T H</au><au>Zhao, Mengting</au><au>Tadich, Anton</au><au>Watson, Liam</au><au>Lowe, Benjamin</au><au>Vu, Thi-Hai-Yen</au><au>Trang, Chi Xuan</au><au>Hwang, Jinwoong</au><au>Mo, Sung-Kwan</au><au>Fuhrer, Michael S</au><au>Edmonds, Mark T</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Imaging the Breakdown and Restoration of Topological Protection in Magnetic Topological Insulator MnBi 2 Te 4</atitle><jtitle>Advanced materials (Weinheim)</jtitle><addtitle>Adv Mater</addtitle><date>2024-06</date><risdate>2024</risdate><volume>36</volume><issue>24</issue><spage>e2312004</spage><pages>e2312004-</pages><issn>0935-9648</issn><eissn>1521-4095</eissn><abstract>Quantum anomalous Hall (QAH) insulators transport charge without resistance along topologically protected chiral 1D edge states. Yet, in magnetic topological insulators to date, topological protection is far from robust, with zero-magnetic field QAH effect only realized at temperatures an order of magnitude below the Néel temperature T
, though small magnetic fields can stabilize QAH effect. Understanding why topological protection breaks down is therefore essential to realizing QAH effect at higher temperatures. Here a scanning tunneling microscope is used to directly map the size of exchange gap (E
) and its spatial fluctuation in the QAH insulator 5-layer MnBi
Te
. Long-range fluctuations of E
are observed, with values ranging between 0 (gapless) and 70 meV, appearing to be uncorrelated to individual surface point defects. The breakdown of topological protection is directly imaged, showing that the gapless edge state, the hallmark signature of a QAH insulator, hybridizes with extended gapless regions in the bulk. Finally, it is unambiguously demonstrated that the gapless regions originate from magnetic disorder, by demonstrating that a small magnetic field restores E
in these regions, explaining the recovery of topological protection in magnetic fields. The results indicate that overcoming magnetic disorder is the key to exploiting the unique properties of QAH insulators.</abstract><cop>Germany</cop><pmid>38402422</pmid><doi>10.1002/adma.202312004</doi><orcidid>https://orcid.org/0000-0003-0711-8514</orcidid><orcidid>https://orcid.org/0000-0001-8054-5470</orcidid><orcidid>https://orcid.org/0000-0002-5157-7737</orcidid><orcidid>https://orcid.org/0000-0001-8253-8741</orcidid><orcidid>https://orcid.org/0000-0002-8334-2465</orcidid><orcidid>https://orcid.org/0000-0001-6183-2773</orcidid><orcidid>https://orcid.org/0000-0002-1782-0756</orcidid><orcidid>https://orcid.org/0000-0002-2364-5544</orcidid><orcidid>https://orcid.org/0000-0001-7374-1692</orcidid><orcidid>https://orcid.org/0000-0001-9455-5901</orcidid></addata></record> |
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title | Imaging the Breakdown and Restoration of Topological Protection in Magnetic Topological Insulator MnBi 2 Te 4 |
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