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Efficient Continuous Light‐Driven Electrochemical Water Splitting Enabled by Monolithic Perovskite‐Silicon Tandem Photovoltaics

Solar‐assisted water electrolysis is a promising technology for storing the energy of incident solar irradiation into hydrogen as a fuel. Here, an integrated continuous flow electrochemical reactor coupled to a monolithic perovskite‐silicon tandem solar cell is demonstrated that provides light‐drive...

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Bibliographic Details
Published in:Advanced materials technologies 2023-01, Vol.8 (2), p.n/a
Main Authors: Datta, Kunal, Branco, Bruno, Zhao, Yifeng, Zardetto, Valerio, Phung, Nga, Bracesco, Andrea, Mazzarella, Luana, Wienk, Martijn M., Creatore, Mariadriana, Isabella, Olindo, Janssen, René A. J.
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Language:English
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Summary:Solar‐assisted water electrolysis is a promising technology for storing the energy of incident solar irradiation into hydrogen as a fuel. Here, an integrated continuous flow electrochemical reactor coupled to a monolithic perovskite‐silicon tandem solar cell is demonstrated that provides light‐driven electrochemical solar‐to‐hydrogen conversion with an energy conversion efficiency exceeding 21% at 1‐Sun equivalent light intensity and stable operation during three simulated day‐night cycles. Solar‐assisted water splitting using a flow electrochemical cell and a monolithic perovskite‐silicon tandem solar cell is used to generate hydrogen at a solar‐to‐hydrogen efficiency of >21% at 1‐Sun equivalent light intensity.
ISSN:2365-709X
2365-709X
DOI:10.1002/admt.202201131