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Ion Exchange Membranes in Electrochemical CO2 Reduction Processes
The low-temperature electrolysis of CO 2 in membrane-based flow reactors is a promising technology for converting captured CO 2 into valuable chemicals and fuels. In recent years, substantial improvements in reactor design have significantly improved the economic viability of this technology; thus,...
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| Published in: | Electrochemical energy reviews 2023-12, Vol.6 (1), Article 26 |
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| creator | Habibzadeh, Faezeh Mardle, Peter Zhao, Nana Riley, Harry D. Salvatore, Danielle A. Berlinguette, Curtis P. Holdcroft, Steven Shi, Zhiqing |
| description | The low-temperature electrolysis of CO
2
in membrane-based flow reactors is a promising technology for converting captured CO
2
into valuable chemicals and fuels. In recent years, substantial improvements in reactor design have significantly improved the economic viability of this technology; thus, the field has experienced a rapid increase in research interest. Among the factors related to reactor design, the ion exchange membrane (IEM) plays a prominent role in the energetic efficiency of CO
2
conversion into useful products. Reactors utilizing cation exchange, anion exchange and bipolar membranes have all been developed, each providing unique benefits and challenges that must be overcome before large-scale commercialization is feasible. Therefore, to direct advances in IEM technology specific to electrochemical CO
2
reduction reactions (CO
2
RRs), this review serves to first provide polymer scientists with a general understanding of membrane-based CO
2
RR reactors and membrane-related shortcomings and to encourage systematic synthetic approaches to develop membranes that meet the specific requirements of CO
2
RRs. Second, this review provides researchers in the fields of electrocatalysis and CO
2
RRs with more detailed insight into the often-overlooked membrane roles and requirements; thus, new methodologies for membrane evaluation during CO
2
RR may be developed. By using CO
2
-to-CO/HCOO
−
methodologies as practical baseline systems, a clear conceptualization of the merits and challenges of different systems and reasonable objectives for future research and development are presented.
Graphical Abstract |
| doi_str_mv | 10.1007/s41918-023-00183-9 |
| format | article |
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2
in membrane-based flow reactors is a promising technology for converting captured CO
2
into valuable chemicals and fuels. In recent years, substantial improvements in reactor design have significantly improved the economic viability of this technology; thus, the field has experienced a rapid increase in research interest. Among the factors related to reactor design, the ion exchange membrane (IEM) plays a prominent role in the energetic efficiency of CO
2
conversion into useful products. Reactors utilizing cation exchange, anion exchange and bipolar membranes have all been developed, each providing unique benefits and challenges that must be overcome before large-scale commercialization is feasible. Therefore, to direct advances in IEM technology specific to electrochemical CO
2
reduction reactions (CO
2
RRs), this review serves to first provide polymer scientists with a general understanding of membrane-based CO
2
RR reactors and membrane-related shortcomings and to encourage systematic synthetic approaches to develop membranes that meet the specific requirements of CO
2
RRs. Second, this review provides researchers in the fields of electrocatalysis and CO
2
RRs with more detailed insight into the often-overlooked membrane roles and requirements; thus, new methodologies for membrane evaluation during CO
2
RR may be developed. By using CO
2
-to-CO/HCOO
−
methodologies as practical baseline systems, a clear conceptualization of the merits and challenges of different systems and reasonable objectives for future research and development are presented.
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2
in membrane-based flow reactors is a promising technology for converting captured CO
2
into valuable chemicals and fuels. In recent years, substantial improvements in reactor design have significantly improved the economic viability of this technology; thus, the field has experienced a rapid increase in research interest. Among the factors related to reactor design, the ion exchange membrane (IEM) plays a prominent role in the energetic efficiency of CO
2
conversion into useful products. Reactors utilizing cation exchange, anion exchange and bipolar membranes have all been developed, each providing unique benefits and challenges that must be overcome before large-scale commercialization is feasible. Therefore, to direct advances in IEM technology specific to electrochemical CO
2
reduction reactions (CO
2
RRs), this review serves to first provide polymer scientists with a general understanding of membrane-based CO
2
RR reactors and membrane-related shortcomings and to encourage systematic synthetic approaches to develop membranes that meet the specific requirements of CO
2
RRs. Second, this review provides researchers in the fields of electrocatalysis and CO
2
RRs with more detailed insight into the often-overlooked membrane roles and requirements; thus, new methodologies for membrane evaluation during CO
2
RR may be developed. By using CO
2
-to-CO/HCOO
−
methodologies as practical baseline systems, a clear conceptualization of the merits and challenges of different systems and reasonable objectives for future research and development are presented.
Graphical Abstract</description><subject>Catalysis</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Electrochemistry</subject><subject>Industrial Chemistry/Chemical Engineering</subject><subject>Renewable and Green Energy</subject><subject>Review Article</subject><issn>2520-8489</issn><issn>2520-8136</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNp9kN1KAzEQhYMoWGpfwKt9gegk2WySy1KqFioV0euQTaZ2y_5IsgV9e6Ort17NMHO-Yc4h5JrBDQNQt6lkhmkKXFAApgU1Z2TGJQeqmajO__pSm0uySOkIkKVMVoLPyHIz9MX6wx9c_4bFI3Z1dD2mosnTFv0YB3_ArvGuLVY7XjxjOPmxycxT3mBKmK7Ixd61CRe_dU5e79Yvqwe63d1vVsst9ULIkSo0slSsVCGEGlAqWdY1V0qAcsZpdIJ5BxI5liEwg7oymF_UIDXUggcxJ3y66-OQUsS9fY9N5-KnZWC_c7BTDjabsz85WJMhMUEpi7PDaI_DKfb5z_-oL-tOX0A</recordid><startdate>20231201</startdate><enddate>20231201</enddate><creator>Habibzadeh, Faezeh</creator><creator>Mardle, Peter</creator><creator>Zhao, Nana</creator><creator>Riley, Harry D.</creator><creator>Salvatore, Danielle A.</creator><creator>Berlinguette, Curtis P.</creator><creator>Holdcroft, Steven</creator><creator>Shi, Zhiqing</creator><general>Springer Nature Singapore</general><scope>C6C</scope><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-7929-945X</orcidid></search><sort><creationdate>20231201</creationdate><title>Ion Exchange Membranes in Electrochemical CO2 Reduction Processes</title><author>Habibzadeh, Faezeh ; Mardle, Peter ; Zhao, Nana ; Riley, Harry D. ; Salvatore, Danielle A. ; Berlinguette, Curtis P. ; Holdcroft, Steven ; Shi, Zhiqing</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c335t-7e9547147dddb0e5754bb277307a9a8ea31ca05e2e4dd19e869e56380580b32d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Catalysis</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Electrochemistry</topic><topic>Industrial Chemistry/Chemical Engineering</topic><topic>Renewable and Green Energy</topic><topic>Review Article</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Habibzadeh, Faezeh</creatorcontrib><creatorcontrib>Mardle, Peter</creatorcontrib><creatorcontrib>Zhao, Nana</creatorcontrib><creatorcontrib>Riley, Harry D.</creatorcontrib><creatorcontrib>Salvatore, Danielle A.</creatorcontrib><creatorcontrib>Berlinguette, Curtis P.</creatorcontrib><creatorcontrib>Holdcroft, Steven</creatorcontrib><creatorcontrib>Shi, Zhiqing</creatorcontrib><collection>SpringerOpen</collection><collection>CrossRef</collection><jtitle>Electrochemical energy reviews</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Habibzadeh, Faezeh</au><au>Mardle, Peter</au><au>Zhao, Nana</au><au>Riley, Harry D.</au><au>Salvatore, Danielle A.</au><au>Berlinguette, Curtis P.</au><au>Holdcroft, Steven</au><au>Shi, Zhiqing</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Ion Exchange Membranes in Electrochemical CO2 Reduction Processes</atitle><jtitle>Electrochemical energy reviews</jtitle><stitle>Electrochem. Energy Rev</stitle><date>2023-12-01</date><risdate>2023</risdate><volume>6</volume><issue>1</issue><artnum>26</artnum><issn>2520-8489</issn><eissn>2520-8136</eissn><abstract>The low-temperature electrolysis of CO
2
in membrane-based flow reactors is a promising technology for converting captured CO
2
into valuable chemicals and fuels. In recent years, substantial improvements in reactor design have significantly improved the economic viability of this technology; thus, the field has experienced a rapid increase in research interest. Among the factors related to reactor design, the ion exchange membrane (IEM) plays a prominent role in the energetic efficiency of CO
2
conversion into useful products. Reactors utilizing cation exchange, anion exchange and bipolar membranes have all been developed, each providing unique benefits and challenges that must be overcome before large-scale commercialization is feasible. Therefore, to direct advances in IEM technology specific to electrochemical CO
2
reduction reactions (CO
2
RRs), this review serves to first provide polymer scientists with a general understanding of membrane-based CO
2
RR reactors and membrane-related shortcomings and to encourage systematic synthetic approaches to develop membranes that meet the specific requirements of CO
2
RRs. Second, this review provides researchers in the fields of electrocatalysis and CO
2
RRs with more detailed insight into the often-overlooked membrane roles and requirements; thus, new methodologies for membrane evaluation during CO
2
RR may be developed. By using CO
2
-to-CO/HCOO
−
methodologies as practical baseline systems, a clear conceptualization of the merits and challenges of different systems and reasonable objectives for future research and development are presented.
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| subjects | Catalysis Chemistry Chemistry and Materials Science Electrochemistry Industrial Chemistry/Chemical Engineering Renewable and Green Energy Review Article |
| title | Ion Exchange Membranes in Electrochemical CO2 Reduction Processes |
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