Dephasing and resonance electronic Raman scattering

The intensity of the resonance electronic Raman spectrum of terbium aluminum garnet is discussed in terms of radiative, non-radiative and pure electronic dephasing processes which govern the width of the resonating excited electronic state. As a result of fast electronic dephasing in comparison to t...

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Bibliographic Details
Published in:Chemical physics letters 1988-05, Vol.146 (6), p.576-581
Main Author: Koningstein, J.A.
Format: Article
Language:English
Subjects:
Condensed matter: electronic structure, electrical, magnetic, and optical properties
Exact sciences and technology
Infrared and raman spectra and scattering
Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation
Physics
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Summary:The intensity of the resonance electronic Raman spectrum of terbium aluminum garnet is discussed in terms of radiative, non-radiative and pure electronic dephasing processes which govern the width of the resonating excited electronic state. As a result of fast electronic dephasing in comparison to the other processes, the enhancement of the intensity of the electronic Raman band of the terbium ion is suppressed.
ISSN:0009-2614
1873-4448
DOI:10.1016/0009-2614(88)87505-5