Influence of continental outflow on aerosol chemical characteristics over the Arabian Sea during winter

The chemical composition of aerosol over the Arabian Sea was investigated during December 2007. Elemental Carbon (EC), Organic Carbon (OC), water soluble organic and inorganic constituents and crustal elements (Al, Fe, Ca, and Mg) were measured in total suspended particulate samples (TSP) collected...

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Bibliographic Details
Published in:Atmospheric environment (1994) 2012-04, Vol.50, p.182-191
Main Authors: Kumar, Ashwini, Sudheer, A.K., Goswami, Vineet, Bhushan, Ravi
Format: Article
Language:English
Subjects:
Aerosol composition
aerosols
air
aluminum
Arabian Sea
atmospheric chemistry
biogeochemistry
biomass
burning
calcium
carbon
chemical composition
Elemental and organic carbon
iron
magnesium
Marine aerosol
potassium
winter
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Summary:The chemical composition of aerosol over the Arabian Sea was investigated during December 2007. Elemental Carbon (EC), Organic Carbon (OC), water soluble organic and inorganic constituents and crustal elements (Al, Fe, Ca, and Mg) were measured in total suspended particulate samples (TSP) collected from marine boundary layer of the Arabian Sea when the oceanic region is influenced by continental outflow. Anthropogenic and natural mineral aerosol originating from continental regions dominates the aerosol composition contributing ∼88% of total aerosol mass. The sea-salt aerosol comprises only ∼12% of TSP. The carbonaceous aerosol exhibits spatial trend similar to that of K+ suggesting major source could be biomass burning. Secondary organic aerosol (SOA) contribution estimated by EC-tracer method suggests that up to 67% of OC can be of secondary origin. Average water soluble organic carbon to OC ratio is ∼0.9, indicates significant formation of SOA during transport of continental air masses. These results demonstrate the dominance of continental aerosol over the Arabian Sea during wintertime where deposition may have major impact on surface ocean biogeochemistry. ► Aerosol characteristics were studied over Arabian Sea during continental outflow. ► Continental aerosol dominates total measured aerosol mass (∼88%). ► The sea-salt aerosol comprises only ∼12%. ► Secondary organic carbon estimated up to 67% of total organic carbon.
ISSN:1352-2310
1873-2844
DOI:10.1016/j.atmosenv.2011.12.040