Preparation and characterisation of Fe/Fe3O4 fibres based soft magnetic composites

• Published in: Ceramics international 2021-01, Vol.47 (1), p.581-589
• Main Authors: Neamţu, B.V., Pszola, M., Vermeşan, H., Stoian, G., Grigoraş, M., Opriş, A., Cotojman, L., Marinca, T.F., Lupu, N., Chicinaş, I.
• Format: Article
• Language: English
• Subjects: Core loss separation; DC and AC magnetic Characterisation; Fe3O4 insulating layer; Fibres based soft magnetic composites
• ISSN: 0272-8842; 1873-3956
• DOI: 10.1016/j.ceramint.2020.08.165

Soft magnetic composites (FSMCs) have been prepared by using Fe fibres coated with a layer of Fe3O4, this layer playing the role of insulating material. The coating was made via blackening method by simply immersing the fibres in the blackening bath for 5, 10 and 15 min. The formation of the Fe3O4 coating on the surface of the fibres was confirmed by X-ray diffraction. The SEM investigation, used to evaluate the thickness of the coatings, has proved that increasing the coating duration leads to the increase of the coating thickness and complete coverage of the surface of the fibres. Differential scanning calorimetry and thermomagnetic measurements were used to investigate the thermal stability of the composite fibres. The fibres coated with Fe3O4 were compacted at a compaction pressure of 700 MPa to obtain toroidal magnetic cores. The obtained cores were characterised in DC and AC magnetisation regime. The analysis of the quasi-static hysteresis loops evidenced that increasing the thickness of the Fe3O4 leads to a slight deterioration of the compact's magnetic properties. However, as the thickness of the Fe3O4 layer increases, the development of eddy currents at a larger scale is hindered as proved by the AC magnetic investigations. A model for analytic separation of the core losses is proposed. By applying this model to the prepared samples, we are now able to discriminate between the occurring losses and adjust the preparation process of new samples to the targeted characteristics.