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Nanostructured CuO/Co2O4@ nitrogen doped MWCNT hybrid composite electrode for high-performance supercapacitors

Nanosheet-like structures of copper cobaltite (CuO/Co2O4) decorated on N-MWCNT electrodes were synthesized through hydrothermal process in the presence of ammonia/urea. The structural and morphological properties were characterized by Raman, XRD, XPS, SEM, SEM-EDX and FE-TEM analysis. The electroche...

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Bibliographic Details
Published in:Composites. Part B, Engineering Engineering, 2019-06, Vol.166, p.74-85
Main Authors: Ramesh, Sivalingam, Kathalingam, A., Karuppasamy, K., Kim, Hyun-Seok, Kim, Heung Soo
Format: Article
Language:English
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Summary:Nanosheet-like structures of copper cobaltite (CuO/Co2O4) decorated on N-MWCNT electrodes were synthesized through hydrothermal process in the presence of ammonia/urea. The structural and morphological properties were characterized by Raman, XRD, XPS, SEM, SEM-EDX and FE-TEM analysis. The electrochemical properties of the CuO/Co2O4@N-MWCNT hybrid electrodes were studied using cyclic voltammetry, galvanostatic charge−discharge, and electrochemical impedance analyses. The prepared CuO/Co2O4@N-MWCNT and CuO@N-MWCNT electrodes showed a specific capacitance of ∼246 F g−1 and 100 F g−1 at a current density of 0.5 A g−1 for three electrode assembly. Further, the asymmetric cells also fabricated and it delivered the highest specific capacitance of 268 F g−1 and 279 F g−1 for CuO@N-MWCNT and CuO/Co2O4@N-MWCNT electrodes respectively. These electrodes possessed very good capacitance behavior with 89% retention even after 5000 cycles at 0.5 A g−1 which overlay a way to use as promising candidates for the high-performance supercapacitors.
ISSN:1359-8368
1879-1069
DOI:10.1016/j.compositesb.2018.11.116