Effect of inserted baffles on hydrogen heterogeneous reaction in planar catalytic micro combustor

• Published in: International journal of hydrogen energy 2023-05, Vol.48 (41), p.15722-15735
• Main Authors: Lu, Qingbo, Wang, Yunchao, Zhang, Yi, Fan, Baowei, Wang, Yu, Quaye, Evans K., Pan, Jianfeng
• Format: Article
• Language: English
• Subjects: Baffle; Heterogeneous reaction; Hydrogen; Micro combustion; Numerical simulation
• ISSN: 0360-3199; 1879-3487
• DOI: 10.1016/j.ijhydene.2023.01.004

Heterogeneous reaction characteristics of premixed H2/Air mixture are numerically investigated in micro combustor with coating platinum (Pt) catalyst on the inner wall. The well-designed combustor with the inserted baffle is committed to improving the transport of bulk species on the catalytic surface, therefore enhancing the fuel conversion ratio. A two-dimensional numerical model with detailed heterogeneous reaction mechanism is developed and verified. In this work, the numerical results reveal that the heterogeneous reaction rate and fuel conversion ratio are significantly improved in the combustor with inserted baffle. The velocity of gaseous mixture swiftly increases between the baffle and catalytic surface, resulting in the increasing adsorption-desorption of bulk species on the catalytic surface. The main influencing factors of inserted baffle body comprise of slit width between two ribs in the same row (W), rib length (L), distance between adjacent baffles row (D), number of baffle row (n) which are studied to obtain a set of optimized parameters of baffle in the well-designed combustor. The optimized parameters of the baffle are W = 0 mm, L = 0.4 mm, D = 4 mm and n = 4, which are employed in the combustor to obtain a high hydrogen conversion ratio. Moreover, the effect of different inlet velocities and equivalent ratios of the mixture on the heterogeneous reaction characteristics are carried out in the designed combustor. As the designed combustor performs well, and the improvement effect of the optimized baffle gradually increases together with the inlet velocity, particularly for high inlet velocity (7 m/s). The promotion effects of baffle in the designed combustor are presented when the rich and lean fuel are adopted at inlet velocity of 7 m/s. Finally, the relative parameters of this work can serve as a reference and guidance for the design of micro scale combustor. •A digital model for a catalytic micro combustor with baffles is established.•Optimization of baffle parameters is found to improve the combustor performance.•Effect of varying inlet conditions on the well-designed combustor performance is investigated.•The principle of enhanced heterogeneous reaction in a micro combustor is explored.