Effect of thermal annealing on the magnetization reversal and spin dynamics in ferrimagnetic TbCo thin films

• Published in: Journal of magnetism and magnetic materials 2023-12, Vol.587, p.171363, Article 171363
• Main Authors: Pradhan, Jhantu, Devapriya, M.S., Mondal, Rohiteswar, Manoj, Talluri, Murapaka, Chandrasekhar, Haldar, Arabinda
• Format: Article
• Language: English
• Subjects: Ferrimagnetic thin film; Ferromagnetic resonance; Magnetic anisotropy; Magnetization dynamics; TbCo thin film
• ISSN: 0304-8853
• DOI: 10.1016/j.jmmm.2023.171363

•Ferromagnetic resonance (FMR) spectra is observed in ferrimagnetic Tb10Co90 thin film.•A significantly large reduction in inhomogeneous linewidth broadening and anisotropy is found upon post-annealing.•Annealed films are magnetically softer than as-deposited films.•Gilbert damping constant is observed to decrease upon annealing.•The damping constant of the annealed films is comparable with some of the well-known low-damping magnetic materials.•The observed results are closely related to improvement in crystallinity of the film due to annealing. “Ferrimagnetic rare earth-transition metal alloys are promising materials for high-speed and low-power spintronic device applications due to their wide tunability in magnetic properties as a function of temperature and composition. Here, we report the influence of thermal annealing on the magnetization reversal and spin dynamics of ferrimagnetic Tb10Co90 thin films. We have used the co-sputtering technique for the deposition of two different thicknesses (20 nm and 25 nm) of the TbCo films. Annealing of the samples has been carried out in the vacuum at 350 °C for 1 h. The magnetization reversal and dynamic properties of the as-deposited and annealed films are studied using the magneto-optical Kerr effect and broadband ferromagnetic resonance measurements at room temperature, respectively. The hysteresis loops reveal an anisotropic reversal process. The anisotropy field reduces from 66 Oe to 38 Oe for 20-nm-thick films and 98 Oe to 31 Oe for 25-nm-thick films upon annealing. Consequently, thermal annealing has led to a large reduction (∼70 %) in inhomogeneous linewidth broadening of the ferromagnetic resonance modes. Gilbert damping constant is found to decrease from 0.027 to 0.021 for 20-nm-thick films, whereas it decreases from 0.043 to 0.019 for 25-nm-thick films. The results have been attributed to the enhanced crystallinity of the films as observed in the structural analysis using grazing incidence X-ray diffraction.”