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Synthesis of CdS/N-rGO S-scheme heterojunction photocatalyst for efficient H2 evolution

Owing to the anticipated energy crisis, the demand for photocatalytic H2 evolution is also growing. Herein, a hydrothermal process is used to prepare an S-scheme CdS/N-rGO heterojunction system. Different characterizations reveal that robust interfacial contact and integration of CdS and N-rGO effec...

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Bibliographic Details
Published in:Materials science in semiconductor processing 2024-11, Vol.182, p.108716, Article 108716
Main Authors: Zhao, Feng, Ahmad, Irshad, AlFaify, S., M Alanezi, Khaled, Bayahia, Hossein, A. Aladsani, Ebrahim, Alshahrani, Thamraa
Format: Article
Language:English
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Summary:Owing to the anticipated energy crisis, the demand for photocatalytic H2 evolution is also growing. Herein, a hydrothermal process is used to prepare an S-scheme CdS/N-rGO heterojunction system. Different characterizations reveal that robust interfacial contact and integration of CdS and N-rGO effectively promote the surface area, photoresponse, and separation and migration of photoinduced electron-hole pairs, endowing CdS/N-rGO composite an excellent photocatalytic activity. Under visible light illumination, the CdS/N-rGO obtains a promising H2 evolution efficiency of 58.8 mmolh−1g−1, which is nearly 21-times more than that of bare CdS. The prepared composite also exhibits excellent stability in recycling experiments. This work might open up novel ways to design excellent N-rGO-based S-scheme photocatalysts for solar fuel generation.
ISSN:1369-8001
1873-4081
DOI:10.1016/j.mssp.2024.108716