Spatial Self-Phase Modulation of Optical Vortex Beams in Liquid Suspensions of Semiconducting, Semimetallic, and Metallic 2D Nanoflakes due to a Kerr-like Nonlinearity

Optical vortex beam (OVB) propagation through liquid suspensions of semiconducting, semimetallic, and metallic 2D nanoflakes, MoS2, NbS2, and WTe2, respectively, was studied under different excitation conditions regarding the optical absorption region. It is demonstrated that the OVB generated using...

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Published in:Journal of physical chemistry. C 2024-01, Vol.128 (3), p.1350-1356
Main Authors: Campos, Cecília L. A. V., Bautista, Jessica E. Q., Amaral, Anderson M., de Araújo, Cid B., Jawaid, Ali M., Busch, Robert, Vaia, Richard A., Gomes, Anderson S. L.
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C: Physical Properties of Materials and Interfaces
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container_issue 3
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container_title Journal of physical chemistry. C
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creator Campos, Cecília L. A. V.
Bautista, Jessica E. Q.
Amaral, Anderson M.
de Araújo, Cid B.
Jawaid, Ali M.
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Vaia, Richard A.
Gomes, Anderson S. L.
description Optical vortex beam (OVB) propagation through liquid suspensions of semiconducting, semimetallic, and metallic 2D nanoflakes, MoS2, NbS2, and WTe2, respectively, was studied under different excitation conditions regarding the optical absorption region. It is demonstrated that the OVB generated using a spatial light modulator propagates under intensity-dependent refraction originating from thermal nonlinearity. Besides the nanomaterial’s suspensions, measurements were also performed with pristine solvents to corroborate the thermally induced intensity dependence arising from light absorption in the studied media.
doi_str_mv 10.1021/acs.jpcc.3c06636
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title Spatial Self-Phase Modulation of Optical Vortex Beams in Liquid Suspensions of Semiconducting, Semimetallic, and Metallic 2D Nanoflakes due to a Kerr-like Nonlinearity
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