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Gate-Switchable Arrays of Quantum Light Emitters in Contacted Monolayer MoS 2 van der Waals Heterodevices
We demonstrate electrostatic switching of individual, site-selectively generated matrices of single photon emitters (SPEs) in MoS van der Waals heterodevices. We contact monolayers of MoS in field-effect devices with graphene gates and hexagonal boron nitride as the dielectric and graphite as bottom...
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Published in: | Nano letters 2021-01, Vol.21 (2), p.1040-1046 |
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Main Authors: | , , , , , , , , , , , , , , , , , |
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container_title | Nano letters |
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creator | Hötger, Alexander Klein, Julian Barthelmi, Katja Sigl, Lukas Sigger, Florian Männer, Wolfgang Gyger, Samuel Florian, Matthias Lorke, Michael Jahnke, Frank Taniguchi, Takashi Watanabe, Kenji Jöns, Klaus D Wurstbauer, Ursula Kastl, Christoph Müller, Kai Finley, Jonathan J Holleitner, Alexander W |
description | We demonstrate electrostatic switching of individual, site-selectively generated matrices of single photon emitters (SPEs) in MoS
van der Waals heterodevices. We contact monolayers of MoS
in field-effect devices with graphene gates and hexagonal boron nitride as the dielectric and graphite as bottom gates. After the assembly of such gate-tunable heterodevices, we demonstrate how arrays of defects, that serve as quantum emitters, can be site-selectively generated in the monolayer MoS
by focused helium ion irradiation. The SPEs are sensitive to the charge carrier concentration in the MoS
and switch on and off similar to the neutral exciton in MoS
for moderate electron doping. The demonstrated scheme is a first step for producing scalable, gate-addressable, and gate-switchable arrays of quantum light emitters in MoS
heterostacks. |
doi_str_mv | 10.1021/acs.nanolett.0c04222 |
format | article |
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van der Waals heterodevices. We contact monolayers of MoS
in field-effect devices with graphene gates and hexagonal boron nitride as the dielectric and graphite as bottom gates. After the assembly of such gate-tunable heterodevices, we demonstrate how arrays of defects, that serve as quantum emitters, can be site-selectively generated in the monolayer MoS
by focused helium ion irradiation. The SPEs are sensitive to the charge carrier concentration in the MoS
and switch on and off similar to the neutral exciton in MoS
for moderate electron doping. The demonstrated scheme is a first step for producing scalable, gate-addressable, and gate-switchable arrays of quantum light emitters in MoS
heterostacks.</description><identifier>ISSN: 1530-6984</identifier><identifier>EISSN: 1530-6992</identifier><identifier>DOI: 10.1021/acs.nanolett.0c04222</identifier><identifier>PMID: 33433221</identifier><language>eng</language><publisher>United States</publisher><ispartof>Nano letters, 2021-01, Vol.21 (2), p.1040-1046</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c1191-98572dbabf140f0c32f60c03485bf513d8d645abed4e54cae77ab1c8ee4971af3</citedby><cites>FETCH-LOGICAL-c1191-98572dbabf140f0c32f60c03485bf513d8d645abed4e54cae77ab1c8ee4971af3</cites><orcidid>0000-0002-1467-3105 ; 0000-0002-8314-4397 ; 0000-0002-0873-8224 ; 0000-0001-5309-618X ; 0000-0003-3701-8119 ; 0000-0002-5814-7510</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/33433221$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Hötger, Alexander</creatorcontrib><creatorcontrib>Klein, Julian</creatorcontrib><creatorcontrib>Barthelmi, Katja</creatorcontrib><creatorcontrib>Sigl, Lukas</creatorcontrib><creatorcontrib>Sigger, Florian</creatorcontrib><creatorcontrib>Männer, Wolfgang</creatorcontrib><creatorcontrib>Gyger, Samuel</creatorcontrib><creatorcontrib>Florian, Matthias</creatorcontrib><creatorcontrib>Lorke, Michael</creatorcontrib><creatorcontrib>Jahnke, Frank</creatorcontrib><creatorcontrib>Taniguchi, Takashi</creatorcontrib><creatorcontrib>Watanabe, Kenji</creatorcontrib><creatorcontrib>Jöns, Klaus D</creatorcontrib><creatorcontrib>Wurstbauer, Ursula</creatorcontrib><creatorcontrib>Kastl, Christoph</creatorcontrib><creatorcontrib>Müller, Kai</creatorcontrib><creatorcontrib>Finley, Jonathan J</creatorcontrib><creatorcontrib>Holleitner, Alexander W</creatorcontrib><title>Gate-Switchable Arrays of Quantum Light Emitters in Contacted Monolayer MoS 2 van der Waals Heterodevices</title><title>Nano letters</title><addtitle>Nano Lett</addtitle><description>We demonstrate electrostatic switching of individual, site-selectively generated matrices of single photon emitters (SPEs) in MoS
van der Waals heterodevices. We contact monolayers of MoS
in field-effect devices with graphene gates and hexagonal boron nitride as the dielectric and graphite as bottom gates. After the assembly of such gate-tunable heterodevices, we demonstrate how arrays of defects, that serve as quantum emitters, can be site-selectively generated in the monolayer MoS
by focused helium ion irradiation. The SPEs are sensitive to the charge carrier concentration in the MoS
and switch on and off similar to the neutral exciton in MoS
for moderate electron doping. The demonstrated scheme is a first step for producing scalable, gate-addressable, and gate-switchable arrays of quantum light emitters in MoS
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van der Waals heterodevices. We contact monolayers of MoS
in field-effect devices with graphene gates and hexagonal boron nitride as the dielectric and graphite as bottom gates. After the assembly of such gate-tunable heterodevices, we demonstrate how arrays of defects, that serve as quantum emitters, can be site-selectively generated in the monolayer MoS
by focused helium ion irradiation. The SPEs are sensitive to the charge carrier concentration in the MoS
and switch on and off similar to the neutral exciton in MoS
for moderate electron doping. The demonstrated scheme is a first step for producing scalable, gate-addressable, and gate-switchable arrays of quantum light emitters in MoS
heterostacks.</abstract><cop>United States</cop><pmid>33433221</pmid><doi>10.1021/acs.nanolett.0c04222</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0002-1467-3105</orcidid><orcidid>https://orcid.org/0000-0002-8314-4397</orcidid><orcidid>https://orcid.org/0000-0002-0873-8224</orcidid><orcidid>https://orcid.org/0000-0001-5309-618X</orcidid><orcidid>https://orcid.org/0000-0003-3701-8119</orcidid><orcidid>https://orcid.org/0000-0002-5814-7510</orcidid></addata></record> |
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title | Gate-Switchable Arrays of Quantum Light Emitters in Contacted Monolayer MoS 2 van der Waals Heterodevices |
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