Solution Processed CH 3 NH 3 PbI 3-x Cl x Perovskite Based Self-Powered Ozone Sensing Element Operated at Room Temperature

Hybrid lead halide spin coated perovskite films have been successfully tested as portable, flexible, operated at room temperature, self-powered, and ultrasensitive ozone sensing elements. The electrical resistance of the hybrid lead mixed halide perovskite (CH NH PbI Cl ) sensing element, was immedi...

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Bibliographic Details
Published in:ACS sensors 2018-01, Vol.3 (1), p.135-142
Main Authors: Kakavelakis, George, Gagaoudakis, Emmanouil, Petridis, Konstantinos, Petromichelaki, Valia, Binas, Vassilis, Kiriakidis, George, Kymakis, Emmanuel
Format: Article
Language:English
Subjects:
Calcium Compounds - chemistry
Electric Conductivity
Electric Impedance
Lead
Oxides - chemistry
Ozone - analysis
Reproducibility of Results
Semiconductors
Sensitivity and Specificity
Temperature
Titanium - chemistry
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Summary:Hybrid lead halide spin coated perovskite films have been successfully tested as portable, flexible, operated at room temperature, self-powered, and ultrasensitive ozone sensing elements. The electrical resistance of the hybrid lead mixed halide perovskite (CH NH PbI Cl ) sensing element, was immediately decreased when exposed to an ozone (O ) environment and manage to recover its pristine electrical conductivity values within few seconds after the complete removal of ozone gas. The sensing measurements showed different response times at different gas concentrations, good repeatability, ultrahigh sensitivity and fast recovery time. To the best of our knowledge, this is the first time that a lead halide perovskite semiconductor material is demonstrating its sensing properties in an ozone environment. This work shows the potential of hybrid lead halide based perovskites as reliable sensing elements, serving the objectives of environmental control, with important socioeconomic impact.
ISSN:2379-3694
2379-3694
DOI:10.1021/acssensors.7b00761