High-Performance OTFTs Using Surface-Modified Alumina Dielectrics

We show novel and selective means to modify the dielectric surfaces in organic TFTs. Modification schemes include alkylphosphonic acid monolayers that have a strong affinity for alumina surfaces. Monolayers form robust, extremely uniform thin films and are deposited through simple spin-coating with...

Full description

Saved in:
Bibliographic Details
Published in:The journal of physical chemistry. B 2003-06, Vol.107 (24), p.5877-5881
Main Authors: Kelley, Tommie Wilson, Boardman, Larry D, Dunbar, Timothy D, Muyres, Dawn V, Pellerite, Mark J, Smith, Terry P
Format: Article
Language:English
Citations: Items that this one cites
Items that cite this one
Online Access:Get full text
Tags: Add Tag
No Tags, Be the first to tag this record!
cited_by cdi_FETCH-LOGICAL-a361t-98a597361ea8548ba931675984f4f593b6242d552dde7e330a22e3bb09f7cfa13
cites cdi_FETCH-LOGICAL-a361t-98a597361ea8548ba931675984f4f593b6242d552dde7e330a22e3bb09f7cfa13
container_end_page 5881
container_issue 24
container_start_page 5877
container_title The journal of physical chemistry. B
container_volume 107
creator Kelley, Tommie Wilson
Boardman, Larry D
Dunbar, Timothy D
Muyres, Dawn V
Pellerite, Mark J
Smith, Terry P
description We show novel and selective means to modify the dielectric surfaces in organic TFTs. Modification schemes include alkylphosphonic acid monolayers that have a strong affinity for alumina surfaces. Monolayers form robust, extremely uniform thin films and are deposited through simple spin-coating with a dilute solution of the monolayer precursor in solvent. Adding monolayers to organic TFTs has resulted in polycrystalline devices with mobilities nearly equal to single-crystal values while maintaining acceptable values of other device parameters (for example, the threshold voltage, on/off ratio, and subthreshold slope) required for fully functional integrated circuits.
doi_str_mv 10.1021/jp034352e
format article
fullrecord <record><control><sourceid>istex_cross</sourceid><recordid>TN_cdi_crossref_primary_10_1021_jp034352e</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>ark_67375_TPS_2FJ160R6_J</sourcerecordid><originalsourceid>FETCH-LOGICAL-a361t-98a597361ea8548ba931675984f4f593b6242d552dde7e330a22e3bb09f7cfa13</originalsourceid><addsrcrecordid>eNptj09PwjAchhujiYge_Aa7ePBQ7Z-13Y4EHUgwEBnnput-xSJspIVEv70zEE4e3rzv4cmbPAjdU_JECaPP6x3hKRcMLlCPCkZwF3V52pISeY1uYlwTwgTLZA8Nxn71iecQXBu2prGQzMqijMky-maVLA7BGQv4va2981Ang81h6xuTvHjYgN0Hb-MtunJmE-Hu1H20LF7L4RhPZ6O34WCKDZd0j_PMiFx1E0wm0qwyOadSiTxLXepEzivJUlYLweoaFHBODGPAq4rkTllnKO-jx-OvDW2MAZzeBb814UdTov_c9dm9Y_GR9XEP32fQhC8tFVdCl_OFZsWESvIh9aTjH468sVGv20NoOpN_fn8BtxdlpQ</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>High-Performance OTFTs Using Surface-Modified Alumina Dielectrics</title><source>American Chemical Society:Jisc Collections:American Chemical Society Read &amp; Publish Agreement 2022-2024 (Reading list)</source><creator>Kelley, Tommie Wilson ; Boardman, Larry D ; Dunbar, Timothy D ; Muyres, Dawn V ; Pellerite, Mark J ; Smith, Terry P</creator><creatorcontrib>Kelley, Tommie Wilson ; Boardman, Larry D ; Dunbar, Timothy D ; Muyres, Dawn V ; Pellerite, Mark J ; Smith, Terry P</creatorcontrib><description>We show novel and selective means to modify the dielectric surfaces in organic TFTs. Modification schemes include alkylphosphonic acid monolayers that have a strong affinity for alumina surfaces. Monolayers form robust, extremely uniform thin films and are deposited through simple spin-coating with a dilute solution of the monolayer precursor in solvent. Adding monolayers to organic TFTs has resulted in polycrystalline devices with mobilities nearly equal to single-crystal values while maintaining acceptable values of other device parameters (for example, the threshold voltage, on/off ratio, and subthreshold slope) required for fully functional integrated circuits.</description><identifier>ISSN: 1520-6106</identifier><identifier>EISSN: 1520-5207</identifier><identifier>DOI: 10.1021/jp034352e</identifier><language>eng</language><publisher>American Chemical Society</publisher><ispartof>The journal of physical chemistry. B, 2003-06, Vol.107 (24), p.5877-5881</ispartof><rights>Copyright © 2003 American Chemical Society</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a361t-98a597361ea8548ba931675984f4f593b6242d552dde7e330a22e3bb09f7cfa13</citedby><cites>FETCH-LOGICAL-a361t-98a597361ea8548ba931675984f4f593b6242d552dde7e330a22e3bb09f7cfa13</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids></links><search><creatorcontrib>Kelley, Tommie Wilson</creatorcontrib><creatorcontrib>Boardman, Larry D</creatorcontrib><creatorcontrib>Dunbar, Timothy D</creatorcontrib><creatorcontrib>Muyres, Dawn V</creatorcontrib><creatorcontrib>Pellerite, Mark J</creatorcontrib><creatorcontrib>Smith, Terry P</creatorcontrib><title>High-Performance OTFTs Using Surface-Modified Alumina Dielectrics</title><title>The journal of physical chemistry. B</title><addtitle>J. Phys. Chem. B</addtitle><description>We show novel and selective means to modify the dielectric surfaces in organic TFTs. Modification schemes include alkylphosphonic acid monolayers that have a strong affinity for alumina surfaces. Monolayers form robust, extremely uniform thin films and are deposited through simple spin-coating with a dilute solution of the monolayer precursor in solvent. Adding monolayers to organic TFTs has resulted in polycrystalline devices with mobilities nearly equal to single-crystal values while maintaining acceptable values of other device parameters (for example, the threshold voltage, on/off ratio, and subthreshold slope) required for fully functional integrated circuits.</description><issn>1520-6106</issn><issn>1520-5207</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2003</creationdate><recordtype>article</recordtype><recordid>eNptj09PwjAchhujiYge_Aa7ePBQ7Z-13Y4EHUgwEBnnput-xSJspIVEv70zEE4e3rzv4cmbPAjdU_JECaPP6x3hKRcMLlCPCkZwF3V52pISeY1uYlwTwgTLZA8Nxn71iecQXBu2prGQzMqijMky-maVLA7BGQv4va2981Ang81h6xuTvHjYgN0Hb-MtunJmE-Hu1H20LF7L4RhPZ6O34WCKDZd0j_PMiFx1E0wm0qwyOadSiTxLXepEzivJUlYLweoaFHBODGPAq4rkTllnKO-jx-OvDW2MAZzeBb814UdTov_c9dm9Y_GR9XEP32fQhC8tFVdCl_OFZsWESvIh9aTjH468sVGv20NoOpN_fn8BtxdlpQ</recordid><startdate>20030619</startdate><enddate>20030619</enddate><creator>Kelley, Tommie Wilson</creator><creator>Boardman, Larry D</creator><creator>Dunbar, Timothy D</creator><creator>Muyres, Dawn V</creator><creator>Pellerite, Mark J</creator><creator>Smith, Terry P</creator><general>American Chemical Society</general><scope>BSCLL</scope><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20030619</creationdate><title>High-Performance OTFTs Using Surface-Modified Alumina Dielectrics</title><author>Kelley, Tommie Wilson ; Boardman, Larry D ; Dunbar, Timothy D ; Muyres, Dawn V ; Pellerite, Mark J ; Smith, Terry P</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a361t-98a597361ea8548ba931675984f4f593b6242d552dde7e330a22e3bb09f7cfa13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2003</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Kelley, Tommie Wilson</creatorcontrib><creatorcontrib>Boardman, Larry D</creatorcontrib><creatorcontrib>Dunbar, Timothy D</creatorcontrib><creatorcontrib>Muyres, Dawn V</creatorcontrib><creatorcontrib>Pellerite, Mark J</creatorcontrib><creatorcontrib>Smith, Terry P</creatorcontrib><collection>Istex</collection><collection>CrossRef</collection><jtitle>The journal of physical chemistry. B</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Kelley, Tommie Wilson</au><au>Boardman, Larry D</au><au>Dunbar, Timothy D</au><au>Muyres, Dawn V</au><au>Pellerite, Mark J</au><au>Smith, Terry P</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>High-Performance OTFTs Using Surface-Modified Alumina Dielectrics</atitle><jtitle>The journal of physical chemistry. B</jtitle><addtitle>J. Phys. Chem. B</addtitle><date>2003-06-19</date><risdate>2003</risdate><volume>107</volume><issue>24</issue><spage>5877</spage><epage>5881</epage><pages>5877-5881</pages><issn>1520-6106</issn><eissn>1520-5207</eissn><abstract>We show novel and selective means to modify the dielectric surfaces in organic TFTs. Modification schemes include alkylphosphonic acid monolayers that have a strong affinity for alumina surfaces. Monolayers form robust, extremely uniform thin films and are deposited through simple spin-coating with a dilute solution of the monolayer precursor in solvent. Adding monolayers to organic TFTs has resulted in polycrystalline devices with mobilities nearly equal to single-crystal values while maintaining acceptable values of other device parameters (for example, the threshold voltage, on/off ratio, and subthreshold slope) required for fully functional integrated circuits.</abstract><pub>American Chemical Society</pub><doi>10.1021/jp034352e</doi><tpages>5</tpages></addata></record>
fulltext fulltext
identifier ISSN: 1520-6106
ispartof The journal of physical chemistry. B, 2003-06, Vol.107 (24), p.5877-5881
issn 1520-6106
1520-5207
language eng
recordid cdi_crossref_primary_10_1021_jp034352e
source American Chemical Society:Jisc Collections:American Chemical Society Read & Publish Agreement 2022-2024 (Reading list)
title High-Performance OTFTs Using Surface-Modified Alumina Dielectrics
url http://sfxeu10.hosted.exlibrisgroup.com/loughborough?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-25T16%3A33%3A53IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-istex_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=High-Performance%20OTFTs%20Using%20Surface-Modified%20Alumina%20Dielectrics&rft.jtitle=The%20journal%20of%20physical%20chemistry.%20B&rft.au=Kelley,%20Tommie%20Wilson&rft.date=2003-06-19&rft.volume=107&rft.issue=24&rft.spage=5877&rft.epage=5881&rft.pages=5877-5881&rft.issn=1520-6106&rft.eissn=1520-5207&rft_id=info:doi/10.1021/jp034352e&rft_dat=%3Cistex_cross%3Eark_67375_TPS_2FJ160R6_J%3C/istex_cross%3E%3Cgrp_id%3Ecdi_FETCH-LOGICAL-a361t-98a597361ea8548ba931675984f4f593b6242d552dde7e330a22e3bb09f7cfa13%3C/grp_id%3E%3Coa%3E%3C/oa%3E%3Curl%3E%3C/url%3E&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true