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A nona-vacant Keggin-type tricarbonyl rhenium derivative {[PMo 3 O 16 ][Re(CO) 3 ] 4 } 5− and its catalytic performance for CO 2 cycloaddition reactions
A nona-vacant Keggin-type tricarbonyl rhenium derivative [(NH 4 ) 5 ]{[PMo 3 O 16 ][Re(CO) 3 ] 4 }·1.5H 2 O was obtained and characterized. Its frontier orbitals were computed by density functional theory (DFT) calculations. Furthermore, it could act as a Lewis acid catalyst and promote the conversi...
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| Published in: | RSC advances 2015, Vol.5 (84), p.69006-69009 |
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| Main Authors: | , , , , , , , , |
| Format: | Article |
| Language: | English |
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| cited_by | cdi_FETCH-LOGICAL-c76F-7abd4d43e13a48665e3b010be8dfb0ab82555964e70a5f2878f4793562eb59383 |
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| cites | cdi_FETCH-LOGICAL-c76F-7abd4d43e13a48665e3b010be8dfb0ab82555964e70a5f2878f4793562eb59383 |
| container_end_page | 69009 |
| container_issue | 84 |
| container_start_page | 69006 |
| container_title | RSC advances |
| container_volume | 5 |
| creator | Huo, Zhiyuan Guo, Jipeng Lu, Jingkun Xu, Qiaofei Ma, Pengtao Zhao, Juan Zhang, Dongdi Niu, Jingyang Wang, Jingping |
| description | A nona-vacant Keggin-type tricarbonyl rhenium derivative [(NH
4
)
5
]{[PMo
3
O
16
][Re(CO)
3
]
4
}·1.5H
2
O was obtained and characterized. Its frontier orbitals were computed by density functional theory (DFT) calculations. Furthermore, it could act as a Lewis acid catalyst and promote the conversion of CO
2
to cyclic carbonate under mild reaction conditions with pyrrolidinium bromide as a co-catalyst. |
| doi_str_mv | 10.1039/C5RA14201F |
| format | article |
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)
5
]{[PMo
3
O
16
][Re(CO)
3
]
4
}·1.5H
2
O was obtained and characterized. Its frontier orbitals were computed by density functional theory (DFT) calculations. Furthermore, it could act as a Lewis acid catalyst and promote the conversion of CO
2
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4
)
5
]{[PMo
3
O
16
][Re(CO)
3
]
4
}·1.5H
2
O was obtained and characterized. Its frontier orbitals were computed by density functional theory (DFT) calculations. Furthermore, it could act as a Lewis acid catalyst and promote the conversion of CO
2
to cyclic carbonate under mild reaction conditions with pyrrolidinium bromide as a co-catalyst.</description><issn>2046-2069</issn><issn>2046-2069</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNpNkEFLwzAYhoMoOOYu_oLvqEI1aZq0PY7iVJxUxm5jlK9pOiNdOtI4KOLds0d_nr_EDQV9L-_zXt7DQ8gpo5eM8vQqE7Mxi0LKJgdkENJIBiGV6eE_Piajrnumu0jBQskG5HMMtrUYbFGh9XCvVytjA99vNHhnFLqytX0D7klb87KGSjuzRW-2Gl4Xjw8tcMiBSVguZvosy893ewkRvIH4ev8AtBUY34FCj03vjYKNdnXr1miVhh1AlkMIqldNi1VlvGktOI1qD90JOaqx6fTot4dkPrmeZ7fBNL-5y8bTQMVyEsRYVlEVcc04RomUQvOSMlrqpKpLimUSCiFSGemYoqjDJE7qKE65kKEuRcoTPiQXP7fKtV3ndF1snFmj6wtGi73X4s8r_wYqY2oI</recordid><startdate>2015</startdate><enddate>2015</enddate><creator>Huo, Zhiyuan</creator><creator>Guo, Jipeng</creator><creator>Lu, Jingkun</creator><creator>Xu, Qiaofei</creator><creator>Ma, Pengtao</creator><creator>Zhao, Juan</creator><creator>Zhang, Dongdi</creator><creator>Niu, Jingyang</creator><creator>Wang, Jingping</creator><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>2015</creationdate><title>A nona-vacant Keggin-type tricarbonyl rhenium derivative {[PMo 3 O 16 ][Re(CO) 3 ] 4 } 5− and its catalytic performance for CO 2 cycloaddition reactions</title><author>Huo, Zhiyuan ; Guo, Jipeng ; Lu, Jingkun ; Xu, Qiaofei ; Ma, Pengtao ; Zhao, Juan ; Zhang, Dongdi ; Niu, Jingyang ; Wang, Jingping</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c76F-7abd4d43e13a48665e3b010be8dfb0ab82555964e70a5f2878f4793562eb59383</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Huo, Zhiyuan</creatorcontrib><creatorcontrib>Guo, Jipeng</creatorcontrib><creatorcontrib>Lu, Jingkun</creatorcontrib><creatorcontrib>Xu, Qiaofei</creatorcontrib><creatorcontrib>Ma, Pengtao</creatorcontrib><creatorcontrib>Zhao, Juan</creatorcontrib><creatorcontrib>Zhang, Dongdi</creatorcontrib><creatorcontrib>Niu, Jingyang</creatorcontrib><creatorcontrib>Wang, Jingping</creatorcontrib><collection>CrossRef</collection><jtitle>RSC advances</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Huo, Zhiyuan</au><au>Guo, Jipeng</au><au>Lu, Jingkun</au><au>Xu, Qiaofei</au><au>Ma, Pengtao</au><au>Zhao, Juan</au><au>Zhang, Dongdi</au><au>Niu, Jingyang</au><au>Wang, Jingping</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>A nona-vacant Keggin-type tricarbonyl rhenium derivative {[PMo 3 O 16 ][Re(CO) 3 ] 4 } 5− and its catalytic performance for CO 2 cycloaddition reactions</atitle><jtitle>RSC advances</jtitle><date>2015</date><risdate>2015</risdate><volume>5</volume><issue>84</issue><spage>69006</spage><epage>69009</epage><pages>69006-69009</pages><issn>2046-2069</issn><eissn>2046-2069</eissn><abstract>A nona-vacant Keggin-type tricarbonyl rhenium derivative [(NH
4
)
5
]{[PMo
3
O
16
][Re(CO)
3
]
4
}·1.5H
2
O was obtained and characterized. Its frontier orbitals were computed by density functional theory (DFT) calculations. Furthermore, it could act as a Lewis acid catalyst and promote the conversion of CO
2
to cyclic carbonate under mild reaction conditions with pyrrolidinium bromide as a co-catalyst.</abstract><doi>10.1039/C5RA14201F</doi><tpages>4</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 2046-2069 |
| ispartof | RSC advances, 2015, Vol.5 (84), p.69006-69009 |
| issn | 2046-2069 2046-2069 |
| language | eng |
| recordid | cdi_crossref_primary_10_1039_C5RA14201F |
| source | Royal Society of Chemistry |
| title | A nona-vacant Keggin-type tricarbonyl rhenium derivative {[PMo 3 O 16 ][Re(CO) 3 ] 4 } 5− and its catalytic performance for CO 2 cycloaddition reactions |
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