Vibrational energy redistribution and relaxation in the photoisomerization of cis-stilbene

Trans-stilbene photoproduces appearing from the photoisomerization of cis-stilbene within 150 fs are observed to be vibrationally hot, but with a nonthermal population distribution. The product electronic spectrum depends on the incident photon energy. Clearly, intramolecular vibrational energy redi...

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Published in:The Journal of chemical physics 1992-10, Vol.97 (7), p.5239-5242
Main Authors: SENSION, R. J, SZARKA, A. Z, HOCHSTRASSER, R. M
Format: Article
Language:English
Subjects:
Chemistry
Exact sciences and technology
General and physical chemistry
Photochemistry
Physical chemistry of induced reactions (with radiations, particles and ultrasonics)
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description Trans-stilbene photoproduces appearing from the photoisomerization of cis-stilbene within 150 fs are observed to be vibrationally hot, but with a nonthermal population distribution. The product electronic spectrum depends on the incident photon energy. Clearly, intramolecular vibrational energy redistribution is not ultrafast.
doi_str_mv 10.1063/1.463822
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subjects Chemistry
Exact sciences and technology
General and physical chemistry
Photochemistry
Physical chemistry of induced reactions (with radiations, particles and ultrasonics)
title Vibrational energy redistribution and relaxation in the photoisomerization of cis-stilbene
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