Measurements of K-edge and L-edge extended x-ray absorption fine structure at the national ignition facility (invited)

• Published in: Review of scientific instruments 2024-10, Vol.95 (10)
• Main Authors: Sio, H., Krygier, A., Stoupin, S., Rudd, R. E., Bonev, S. A., Braun, D. G., Coppari, F., Coleman, A. L., Bhandarkar, N., Bitter, M., Bradley, D. K., Buscho, J., Corbin, J., Dozieres, M., Efthimion, P. C., Eggert, J. H., Gao, L., Hill, K. W., Hamel, S., Hsing, W., Kozioziemski, B., Kraus, B. F., Landen, O. L., Le Galloudec, K., Lockard, T. E., Mackinnon, A., May, M., McNaney, J. M., Ose, N., Pablant, N., Park, H.-S., Riddles, J., Sharma, M., Schneider, M. B., Stan, C., Thompson, N., Thorn, D. B., Vonhof, S., Ping, Y.
• Format: Article
• Language: English
• Subjects: Bright plating; Crystal spectroscopy; Data compression; Density; Extended X-ray absorption fine structure; Fine structure; Geophysics; Ignition; Inertial confinement fusion; MATERIALS SCIENCE; Photoelectrons; X ray absorption; X ray sources; X ray spectrometers; X-ray absorption spectroscopy; Zirconium
• ISSN: 0034-6748; 1089-7623; 1089-7623
• DOI: 10.1063/5.0219575

High-energy-density laser facilities and advances in dynamic compression techniques have expanded access to material states in the Terapascal regime relevant to inertial confinement fusion, planetary science, and geophysics. However, experimentally determining the material temperature in these extreme conditions has remained a difficult challenge. Extended X-ray Absorption Fine Structure (EXAFS), referring to the modulations in x-ray absorption above an absorption edge from photoelectrons’ interactions with neighboring atoms, has proven to be a versatile and robust technique for probing material temperature and density for mid-to-high Z elements under dynamic compression. The current platform at the National Ignition Facility has developed six configurations for EXAFS measurements between 7 and 18 keV for different absorption edges (Fe K, Co K, Cu K, Ta L3, Pb L3, and Zr K) using a curved-crystal spectrometer and a bright, continuum foil x-ray source. In this work, we describe the platform geometry, x-ray source performance, spectrometer resolution and throughput, design considerations, and data in ambient and dynamic-compression conditions.