Loading…

Ferromagnetism in transparent thin films of MgO

We show both theoretical and experimental evidences of the appearance of ferromagnetism in MgO thin films. First-principles calculations allow predicting the possibility of the formation of a local moment in MgO, provided the existence of Mg vacancies which create holes on acceptor levels near the O...

Full description

Saved in:
Bibliographic Details
Published in:Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2010-07, Vol.82 (2), Article 024405
Main Authors: Martínez-Boubeta, C., Beltrán, J. I., Balcells, Ll, Konstantinović, Z., Valencia, S., Schmitz, D., Arbiol, J., Estrade, S., Cornil, J., Martínez, B.
Format: Article
Language:English
Subjects:
Citations: Items that this one cites
Items that cite this one
Online Access:Get full text
Tags: Add Tag
No Tags, Be the first to tag this record!
cited_by cdi_FETCH-LOGICAL-c399t-23f74ba88c1349704e98fef5112379677b52eceb4e131532cd212dec8d4a8b33
cites cdi_FETCH-LOGICAL-c399t-23f74ba88c1349704e98fef5112379677b52eceb4e131532cd212dec8d4a8b33
container_end_page
container_issue 2
container_start_page
container_title Physical review. B, Condensed matter and materials physics
container_volume 82
creator Martínez-Boubeta, C.
Beltrán, J. I.
Balcells, Ll
Konstantinović, Z.
Valencia, S.
Schmitz, D.
Arbiol, J.
Estrade, S.
Cornil, J.
Martínez, B.
description We show both theoretical and experimental evidences of the appearance of ferromagnetism in MgO thin films. First-principles calculations allow predicting the possibility of the formation of a local moment in MgO, provided the existence of Mg vacancies which create holes on acceptor levels near the O 2p-dominated valence band. Magnetic measurements evidence of the existence of room-temperature ferromagnetism in MgO thin films. High-resolution transmission electron microscopy demonstrates the existence of cation vacancies in our samples. Finally, by applying the element specificity of the x-ray magnetic circular dichroism technique, we also demonstrate that the magnetic moments of the system arise from the spin polarization of the 2p electrons of oxygen atoms surrounding Mg vacancies.
doi_str_mv 10.1103/PhysRevB.82.024405
format article
fullrecord <record><control><sourceid>csuc_cross</sourceid><recordid>TN_cdi_csuc_recercat_oai_recercat_cat_2072_204758</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>oai_recercat_cat_2072_204758</sourcerecordid><originalsourceid>FETCH-LOGICAL-c399t-23f74ba88c1349704e98fef5112379677b52eceb4e131532cd212dec8d4a8b33</originalsourceid><addsrcrecordid>eNpFkMFKAzEQhoMoWKsv4GlfYNvMJDHJUYu1QqUiPXgL2WzSrnR3SxKFvr1bWvEwM_8M88_AR8g90AkAZdP37SF9-J-nicIJRc6puCAjEIKWyMTn5aCpViUFhGtyk9IXpcA1xxGZzn2MfWs3nc9NaoumK3K0Xdrb6Ltc5O0wCM2uTUUfirfN6pZcBbtL_u5cx2Q9f17PFuVy9fI6e1yWjmmdh69B8soq5YBxLSn3WgUfBAAyqR-krAR65yvugYFg6GoErL1TNbeqYmxM4HTWpW9n4rAanc2mt81_cwykEofEpVCDB8-e2KcUfTD72LQ2HgxQc6Rk_igZheZEif0C9KFbtw</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Ferromagnetism in transparent thin films of MgO</title><source>American Physical Society:Jisc Collections:APS Read and Publish 2023-2025 (reading list)</source><creator>Martínez-Boubeta, C. ; Beltrán, J. I. ; Balcells, Ll ; Konstantinović, Z. ; Valencia, S. ; Schmitz, D. ; Arbiol, J. ; Estrade, S. ; Cornil, J. ; Martínez, B.</creator><creatorcontrib>Martínez-Boubeta, C. ; Beltrán, J. I. ; Balcells, Ll ; Konstantinović, Z. ; Valencia, S. ; Schmitz, D. ; Arbiol, J. ; Estrade, S. ; Cornil, J. ; Martínez, B.</creatorcontrib><description>We show both theoretical and experimental evidences of the appearance of ferromagnetism in MgO thin films. First-principles calculations allow predicting the possibility of the formation of a local moment in MgO, provided the existence of Mg vacancies which create holes on acceptor levels near the O 2p-dominated valence band. Magnetic measurements evidence of the existence of room-temperature ferromagnetism in MgO thin films. High-resolution transmission electron microscopy demonstrates the existence of cation vacancies in our samples. Finally, by applying the element specificity of the x-ray magnetic circular dichroism technique, we also demonstrate that the magnetic moments of the system arise from the spin polarization of the 2p electrons of oxygen atoms surrounding Mg vacancies.</description><identifier>ISSN: 1098-0121</identifier><identifier>EISSN: 1550-235X</identifier><identifier>DOI: 10.1103/PhysRevB.82.024405</identifier><language>eng</language><publisher>American Physical Society</publisher><subject>Espintrònica ; Ferromagnetism ; Ferromagnetisme ; Magnesium oxide ; Pel·lícules fines ; Spintronics ; Thin films ; Òxid de magnesi</subject><ispartof>Physical review. B, Condensed matter and materials physics, 2010-07, Vol.82 (2), Article 024405</ispartof><rights>(c) American Physical Society, 2010 info:eu-repo/semantics/openAccess</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c399t-23f74ba88c1349704e98fef5112379677b52eceb4e131532cd212dec8d4a8b33</citedby><cites>FETCH-LOGICAL-c399t-23f74ba88c1349704e98fef5112379677b52eceb4e131532cd212dec8d4a8b33</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,784,885,27922,27923</link.rule.ids></links><search><creatorcontrib>Martínez-Boubeta, C.</creatorcontrib><creatorcontrib>Beltrán, J. I.</creatorcontrib><creatorcontrib>Balcells, Ll</creatorcontrib><creatorcontrib>Konstantinović, Z.</creatorcontrib><creatorcontrib>Valencia, S.</creatorcontrib><creatorcontrib>Schmitz, D.</creatorcontrib><creatorcontrib>Arbiol, J.</creatorcontrib><creatorcontrib>Estrade, S.</creatorcontrib><creatorcontrib>Cornil, J.</creatorcontrib><creatorcontrib>Martínez, B.</creatorcontrib><title>Ferromagnetism in transparent thin films of MgO</title><title>Physical review. B, Condensed matter and materials physics</title><description>We show both theoretical and experimental evidences of the appearance of ferromagnetism in MgO thin films. First-principles calculations allow predicting the possibility of the formation of a local moment in MgO, provided the existence of Mg vacancies which create holes on acceptor levels near the O 2p-dominated valence band. Magnetic measurements evidence of the existence of room-temperature ferromagnetism in MgO thin films. High-resolution transmission electron microscopy demonstrates the existence of cation vacancies in our samples. Finally, by applying the element specificity of the x-ray magnetic circular dichroism technique, we also demonstrate that the magnetic moments of the system arise from the spin polarization of the 2p electrons of oxygen atoms surrounding Mg vacancies.</description><subject>Espintrònica</subject><subject>Ferromagnetism</subject><subject>Ferromagnetisme</subject><subject>Magnesium oxide</subject><subject>Pel·lícules fines</subject><subject>Spintronics</subject><subject>Thin films</subject><subject>Òxid de magnesi</subject><issn>1098-0121</issn><issn>1550-235X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2010</creationdate><recordtype>article</recordtype><recordid>eNpFkMFKAzEQhoMoWKsv4GlfYNvMJDHJUYu1QqUiPXgL2WzSrnR3SxKFvr1bWvEwM_8M88_AR8g90AkAZdP37SF9-J-nicIJRc6puCAjEIKWyMTn5aCpViUFhGtyk9IXpcA1xxGZzn2MfWs3nc9NaoumK3K0Xdrb6Ltc5O0wCM2uTUUfirfN6pZcBbtL_u5cx2Q9f17PFuVy9fI6e1yWjmmdh69B8soq5YBxLSn3WgUfBAAyqR-krAR65yvugYFg6GoErL1TNbeqYmxM4HTWpW9n4rAanc2mt81_cwykEofEpVCDB8-e2KcUfTD72LQ2HgxQc6Rk_igZheZEif0C9KFbtw</recordid><startdate>20100708</startdate><enddate>20100708</enddate><creator>Martínez-Boubeta, C.</creator><creator>Beltrán, J. I.</creator><creator>Balcells, Ll</creator><creator>Konstantinović, Z.</creator><creator>Valencia, S.</creator><creator>Schmitz, D.</creator><creator>Arbiol, J.</creator><creator>Estrade, S.</creator><creator>Cornil, J.</creator><creator>Martínez, B.</creator><general>American Physical Society</general><scope>AAYXX</scope><scope>CITATION</scope><scope>XX2</scope></search><sort><creationdate>20100708</creationdate><title>Ferromagnetism in transparent thin films of MgO</title><author>Martínez-Boubeta, C. ; Beltrán, J. I. ; Balcells, Ll ; Konstantinović, Z. ; Valencia, S. ; Schmitz, D. ; Arbiol, J. ; Estrade, S. ; Cornil, J. ; Martínez, B.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c399t-23f74ba88c1349704e98fef5112379677b52eceb4e131532cd212dec8d4a8b33</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2010</creationdate><topic>Espintrònica</topic><topic>Ferromagnetism</topic><topic>Ferromagnetisme</topic><topic>Magnesium oxide</topic><topic>Pel·lícules fines</topic><topic>Spintronics</topic><topic>Thin films</topic><topic>Òxid de magnesi</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Martínez-Boubeta, C.</creatorcontrib><creatorcontrib>Beltrán, J. I.</creatorcontrib><creatorcontrib>Balcells, Ll</creatorcontrib><creatorcontrib>Konstantinović, Z.</creatorcontrib><creatorcontrib>Valencia, S.</creatorcontrib><creatorcontrib>Schmitz, D.</creatorcontrib><creatorcontrib>Arbiol, J.</creatorcontrib><creatorcontrib>Estrade, S.</creatorcontrib><creatorcontrib>Cornil, J.</creatorcontrib><creatorcontrib>Martínez, B.</creatorcontrib><collection>CrossRef</collection><collection>Recercat</collection><jtitle>Physical review. B, Condensed matter and materials physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Martínez-Boubeta, C.</au><au>Beltrán, J. I.</au><au>Balcells, Ll</au><au>Konstantinović, Z.</au><au>Valencia, S.</au><au>Schmitz, D.</au><au>Arbiol, J.</au><au>Estrade, S.</au><au>Cornil, J.</au><au>Martínez, B.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Ferromagnetism in transparent thin films of MgO</atitle><jtitle>Physical review. B, Condensed matter and materials physics</jtitle><date>2010-07-08</date><risdate>2010</risdate><volume>82</volume><issue>2</issue><artnum>024405</artnum><issn>1098-0121</issn><eissn>1550-235X</eissn><abstract>We show both theoretical and experimental evidences of the appearance of ferromagnetism in MgO thin films. First-principles calculations allow predicting the possibility of the formation of a local moment in MgO, provided the existence of Mg vacancies which create holes on acceptor levels near the O 2p-dominated valence band. Magnetic measurements evidence of the existence of room-temperature ferromagnetism in MgO thin films. High-resolution transmission electron microscopy demonstrates the existence of cation vacancies in our samples. Finally, by applying the element specificity of the x-ray magnetic circular dichroism technique, we also demonstrate that the magnetic moments of the system arise from the spin polarization of the 2p electrons of oxygen atoms surrounding Mg vacancies.</abstract><pub>American Physical Society</pub><doi>10.1103/PhysRevB.82.024405</doi><tpages>7</tpages><oa>free_for_read</oa></addata></record>
fulltext fulltext
identifier ISSN: 1098-0121
ispartof Physical review. B, Condensed matter and materials physics, 2010-07, Vol.82 (2), Article 024405
issn 1098-0121
1550-235X
language eng
recordid cdi_csuc_recercat_oai_recercat_cat_2072_204758
source American Physical Society:Jisc Collections:APS Read and Publish 2023-2025 (reading list)
subjects Espintrònica
Ferromagnetism
Ferromagnetisme
Magnesium oxide
Pel·lícules fines
Spintronics
Thin films
Òxid de magnesi
title Ferromagnetism in transparent thin films of MgO
url http://sfxeu10.hosted.exlibrisgroup.com/loughborough?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-13T13%3A17%3A56IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-csuc_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Ferromagnetism%20in%20transparent%20thin%20films%20of%20MgO&rft.jtitle=Physical%20review.%20B,%20Condensed%20matter%20and%20materials%20physics&rft.au=Mart%C3%ADnez-Boubeta,%20C.&rft.date=2010-07-08&rft.volume=82&rft.issue=2&rft.artnum=024405&rft.issn=1098-0121&rft.eissn=1550-235X&rft_id=info:doi/10.1103/PhysRevB.82.024405&rft_dat=%3Ccsuc_cross%3Eoai_recercat_cat_2072_204758%3C/csuc_cross%3E%3Cgrp_id%3Ecdi_FETCH-LOGICAL-c399t-23f74ba88c1349704e98fef5112379677b52eceb4e131532cd212dec8d4a8b33%3C/grp_id%3E%3Coa%3E%3C/oa%3E%3Curl%3E%3C/url%3E&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true