Light-induced dimension crossover dictated by excitonic correlations

• Published in: Nature communications 2022-02, Vol.13 (1), p.963-7, Article 963
• Main Authors: Cheng, Yun, Zong, Alfred, Li, Jun, Xia, Wei, Duan, Shaofeng, Zhao, Wenxuan, Li, Yidian, Qi, Fengfeng, Wu, Jun, Zhao, Lingrong, Zhu, Pengfei, Zou, Xiao, Jiang, Tao, Guo, Yanfeng, Yang, Lexian, Qian, Dong, Zhang, Wentao, Kogar, Anshul, Zuerch, Michael W., Xiang, Dao, Zhang, Jie
• Format: Article
• Language: English
• Subjects: 639/766/119/2795; 639/766/119/995; Adiabatic; Astronomy; Charge density waves; Correlation; Crossovers; Electron-hole interaction; Equilibrium; Excitons; Holes (electron deficiencies); Humanities and Social Sciences; Laboratories; Lasers; Light effects; multidisciplinary; Phase coherence; Phase transitions; Photoexcitation; Physics; Science; Science & Technology - Other Topics; Science (multidisciplinary); Symmetry
• ISSN: 2041-1723; 2041-1723
• DOI: 10.1038/s41467-022-28309-5

In low-dimensional systems with strong electronic correlations, the application of an ultrashort laser pulse often yields novel phases that are otherwise inaccessible. The central challenge in understanding such phenomena is to determine how dimensionality and many-body correlations together govern the pathway of a non-adiabatic transition. To this end, we examine a layered compound, 1 T -TiSe 2 , whose three-dimensional charge-density-wave (3D CDW) state also features exciton condensation due to strong electron-hole interactions. We find that photoexcitation suppresses the equilibrium 3D CDW while creating a nonequilibrium 2D CDW. Remarkably, the dimension reduction does not occur unless bound electron-hole pairs are broken. This relation suggests that excitonic correlations maintain the out-of-plane CDW coherence, settling a long-standing debate over their role in the CDW transition. Our findings demonstrate how optical manipulation of electronic interaction enables one to control the dimensionality of a broken-symmetry order, paving the way for realizing other emergent states in strongly correlated systems. The relationship between the charge density wave and excitonic correlations in a layered compound 1 T -TiSe 2 has remained controversial. Here, the authors observe a photo-induced dimensional crossover of the charge density wave and conclude that excitonic correlations are responsible for its out-of-plane phase coherence.