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A topological kagome magnet in high entropy form
Topological kagome magnets RMn 6 Sn 6 (R = rare earth element) attract numerous interests due to their non-trivial band topology and room-temperature magnetism. Here, we report a high entropy version of kagome magnet, (Gd 0.38 Tb 0.27 Dy 0.20 Ho 0.15 )Mn 6 Sn 6 . Such a high entropy material exhibit...
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Published in: | Communications physics 2022-03, Vol.5 (1), p.1-7, Article 63 |
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container_title | Communications physics |
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creator | Min, Lujin Sretenovic, Milos Heitmann, Thomas W. Valentine, Tyler W. Zu, Rui Gopalan, Venkatraman Rost, Christina M. Ke, Xianglin Mao, Zhiqiang |
description | Topological kagome magnets RMn
6
Sn
6
(R = rare earth element) attract numerous interests due to their non-trivial band topology and room-temperature magnetism. Here, we report a high entropy version of kagome magnet, (Gd
0.38
Tb
0.27
Dy
0.20
Ho
0.15
)Mn
6
Sn
6
. Such a high entropy material exhibits multiple spin reorientation transitions, which is not seen in all the related parent compounds and can be understood in terms of competing magnetic interactions enabled by high entropy. Furthermore, we also observed an intrinsic anomalous Hall effect, indicating that the high entropy phase preserves the non-trivial band topology. These results suggest that high entropy may provide a route to engineer the magnetic structure and expand the horizon of topological materials.
Kagome materials have recently attracted significant attention due to their ability to house both topological and magnetic phases. Here, the authors report a high-entropy Kagome magnet that exhibits an anomalous Hall effect, indicating the nontrivial topological properties for the high entropy phase remain. |
doi_str_mv | 10.1038/s42005-022-00842-1 |
format | article |
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6
Sn
6
(R = rare earth element) attract numerous interests due to their non-trivial band topology and room-temperature magnetism. Here, we report a high entropy version of kagome magnet, (Gd
0.38
Tb
0.27
Dy
0.20
Ho
0.15
)Mn
6
Sn
6
. Such a high entropy material exhibits multiple spin reorientation transitions, which is not seen in all the related parent compounds and can be understood in terms of competing magnetic interactions enabled by high entropy. Furthermore, we also observed an intrinsic anomalous Hall effect, indicating that the high entropy phase preserves the non-trivial band topology. These results suggest that high entropy may provide a route to engineer the magnetic structure and expand the horizon of topological materials.
Kagome materials have recently attracted significant attention due to their ability to house both topological and magnetic phases. Here, the authors report a high-entropy Kagome magnet that exhibits an anomalous Hall effect, indicating the nontrivial topological properties for the high entropy phase remain.</description><identifier>ISSN: 2399-3650</identifier><identifier>EISSN: 2399-3650</identifier><identifier>DOI: 10.1038/s42005-022-00842-1</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/301/119/2792 ; 639/766/119/2792 ; Electromagnetism ; Hall effect ; Magnetic properties ; Magnetic structure ; Magnets ; Physics ; Physics and Astronomy ; Rare earth elements ; Room temperature ; Topology</subject><ispartof>Communications physics, 2022-03, Vol.5 (1), p.1-7, Article 63</ispartof><rights>The Author(s) 2022</rights><rights>The Author(s) 2022. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c456t-aabee418df3eb58e6a01087230dd9f15fecc9fdbc0dd1996d676fd109444c9823</citedby><cites>FETCH-LOGICAL-c456t-aabee418df3eb58e6a01087230dd9f15fecc9fdbc0dd1996d676fd109444c9823</cites><orcidid>0000-0003-1882-9039 ; 0000-0003-3666-4661 ; 0000-0001-6866-3677 ; 0000-0002-4920-3293 ; 0000-0002-5540-6011 ; 0000000318829039 ; 0000000168663677 ; 0000000255406011 ; 0000000249203293 ; 0000000336664661</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.proquest.com/docview/2640630105?pq-origsite=primo$$EHTML$$P50$$Gproquest$$Hfree_for_read</linktohtml><link.rule.ids>230,314,776,780,881,25731,27901,27902,36989,44566</link.rule.ids><backlink>$$Uhttps://www.osti.gov/biblio/1855867$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Min, Lujin</creatorcontrib><creatorcontrib>Sretenovic, Milos</creatorcontrib><creatorcontrib>Heitmann, Thomas W.</creatorcontrib><creatorcontrib>Valentine, Tyler W.</creatorcontrib><creatorcontrib>Zu, Rui</creatorcontrib><creatorcontrib>Gopalan, Venkatraman</creatorcontrib><creatorcontrib>Rost, Christina M.</creatorcontrib><creatorcontrib>Ke, Xianglin</creatorcontrib><creatorcontrib>Mao, Zhiqiang</creatorcontrib><title>A topological kagome magnet in high entropy form</title><title>Communications physics</title><addtitle>Commun Phys</addtitle><description>Topological kagome magnets RMn
6
Sn
6
(R = rare earth element) attract numerous interests due to their non-trivial band topology and room-temperature magnetism. Here, we report a high entropy version of kagome magnet, (Gd
0.38
Tb
0.27
Dy
0.20
Ho
0.15
)Mn
6
Sn
6
. Such a high entropy material exhibits multiple spin reorientation transitions, which is not seen in all the related parent compounds and can be understood in terms of competing magnetic interactions enabled by high entropy. Furthermore, we also observed an intrinsic anomalous Hall effect, indicating that the high entropy phase preserves the non-trivial band topology. These results suggest that high entropy may provide a route to engineer the magnetic structure and expand the horizon of topological materials.
Kagome materials have recently attracted significant attention due to their ability to house both topological and magnetic phases. Here, the authors report a high-entropy Kagome magnet that exhibits an anomalous Hall effect, indicating the nontrivial topological properties for the high entropy phase remain.</description><subject>639/301/119/2792</subject><subject>639/766/119/2792</subject><subject>Electromagnetism</subject><subject>Hall effect</subject><subject>Magnetic properties</subject><subject>Magnetic structure</subject><subject>Magnets</subject><subject>Physics</subject><subject>Physics and Astronomy</subject><subject>Rare earth elements</subject><subject>Room temperature</subject><subject>Topology</subject><issn>2399-3650</issn><issn>2399-3650</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>PIMPY</sourceid><sourceid>DOA</sourceid><recordid>eNp9kTtPxDAQhCMEEgjuD1BFUAfWz9glQrwkJBqoLcdZ53LcxYdtCv495oKAisrr1Tdjj6aqTglcEGDqMnEKIBqgtAFQnDZkrzqiTOuGSQH7f-bDapHSCgAo4dAyeVTBVZ3DNqzDMDq7rl_tEDZYb-wwYa7HqV6Ow7LGKcew_ah9iJuT6sDbdcLF93lcvdzePF_fN49Pdw_XV4-N40LmxtoOkRPVe4adUCgtEFAtZdD32hPh0Tnt-86VO9Fa9rKVviegOedOK8qOq4fZtw92ZbZx3Nj4YYIdzW4R4mBszKNbo4FWA4rOKiQlvRPa81Zr25ZHhJXCFq-z2SukPJrkxoxu6cI0ocuGKCGUbAt0PkPbGN7eMWWzCu9xKhkNlRwkKwFEoehMuRhSiuh_vkbAfLVh5jZMacPs2jCkiNgsSgWeBoy_1v-oPgEBNopW</recordid><startdate>20220318</startdate><enddate>20220318</enddate><creator>Min, Lujin</creator><creator>Sretenovic, Milos</creator><creator>Heitmann, Thomas W.</creator><creator>Valentine, Tyler W.</creator><creator>Zu, Rui</creator><creator>Gopalan, Venkatraman</creator><creator>Rost, Christina M.</creator><creator>Ke, Xianglin</creator><creator>Mao, Zhiqiang</creator><general>Nature Publishing Group UK</general><general>Nature Publishing Group</general><general>Nature Portfolio</general><scope>C6C</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7XB</scope><scope>88I</scope><scope>8FE</scope><scope>8FG</scope><scope>8FK</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>L6V</scope><scope>M2P</scope><scope>M7S</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope><scope>Q9U</scope><scope>OTOTI</scope><scope>DOA</scope><orcidid>https://orcid.org/0000-0003-1882-9039</orcidid><orcidid>https://orcid.org/0000-0003-3666-4661</orcidid><orcidid>https://orcid.org/0000-0001-6866-3677</orcidid><orcidid>https://orcid.org/0000-0002-4920-3293</orcidid><orcidid>https://orcid.org/0000-0002-5540-6011</orcidid><orcidid>https://orcid.org/0000000318829039</orcidid><orcidid>https://orcid.org/0000000168663677</orcidid><orcidid>https://orcid.org/0000000255406011</orcidid><orcidid>https://orcid.org/0000000249203293</orcidid><orcidid>https://orcid.org/0000000336664661</orcidid></search><sort><creationdate>20220318</creationdate><title>A topological kagome magnet in high entropy form</title><author>Min, Lujin ; Sretenovic, Milos ; Heitmann, Thomas W. ; Valentine, Tyler W. ; Zu, Rui ; Gopalan, Venkatraman ; Rost, Christina M. ; Ke, Xianglin ; Mao, Zhiqiang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c456t-aabee418df3eb58e6a01087230dd9f15fecc9fdbc0dd1996d676fd109444c9823</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>639/301/119/2792</topic><topic>639/766/119/2792</topic><topic>Electromagnetism</topic><topic>Hall effect</topic><topic>Magnetic properties</topic><topic>Magnetic structure</topic><topic>Magnets</topic><topic>Physics</topic><topic>Physics and Astronomy</topic><topic>Rare earth elements</topic><topic>Room temperature</topic><topic>Topology</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Min, Lujin</creatorcontrib><creatorcontrib>Sretenovic, Milos</creatorcontrib><creatorcontrib>Heitmann, Thomas W.</creatorcontrib><creatorcontrib>Valentine, Tyler W.</creatorcontrib><creatorcontrib>Zu, Rui</creatorcontrib><creatorcontrib>Gopalan, Venkatraman</creatorcontrib><creatorcontrib>Rost, Christina M.</creatorcontrib><creatorcontrib>Ke, Xianglin</creatorcontrib><creatorcontrib>Mao, Zhiqiang</creatorcontrib><collection>SpringerOpen</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni)</collection><collection>ProQuest Central</collection><collection>ProQuest Central Essentials</collection><collection>AUTh Library subscriptions: ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Engineering Collection</collection><collection>ProQuest Science Journals</collection><collection>Engineering Database</collection><collection>Publicly Available Content Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering collection</collection><collection>ProQuest Central Basic</collection><collection>OSTI.GOV</collection><collection>DOAJ Directory of Open Access Journals</collection><jtitle>Communications physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Min, Lujin</au><au>Sretenovic, Milos</au><au>Heitmann, Thomas W.</au><au>Valentine, Tyler W.</au><au>Zu, Rui</au><au>Gopalan, Venkatraman</au><au>Rost, Christina M.</au><au>Ke, Xianglin</au><au>Mao, Zhiqiang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>A topological kagome magnet in high entropy form</atitle><jtitle>Communications physics</jtitle><stitle>Commun Phys</stitle><date>2022-03-18</date><risdate>2022</risdate><volume>5</volume><issue>1</issue><spage>1</spage><epage>7</epage><pages>1-7</pages><artnum>63</artnum><issn>2399-3650</issn><eissn>2399-3650</eissn><abstract>Topological kagome magnets RMn
6
Sn
6
(R = rare earth element) attract numerous interests due to their non-trivial band topology and room-temperature magnetism. Here, we report a high entropy version of kagome magnet, (Gd
0.38
Tb
0.27
Dy
0.20
Ho
0.15
)Mn
6
Sn
6
. Such a high entropy material exhibits multiple spin reorientation transitions, which is not seen in all the related parent compounds and can be understood in terms of competing magnetic interactions enabled by high entropy. Furthermore, we also observed an intrinsic anomalous Hall effect, indicating that the high entropy phase preserves the non-trivial band topology. These results suggest that high entropy may provide a route to engineer the magnetic structure and expand the horizon of topological materials.
Kagome materials have recently attracted significant attention due to their ability to house both topological and magnetic phases. Here, the authors report a high-entropy Kagome magnet that exhibits an anomalous Hall effect, indicating the nontrivial topological properties for the high entropy phase remain.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><doi>10.1038/s42005-022-00842-1</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0003-1882-9039</orcidid><orcidid>https://orcid.org/0000-0003-3666-4661</orcidid><orcidid>https://orcid.org/0000-0001-6866-3677</orcidid><orcidid>https://orcid.org/0000-0002-4920-3293</orcidid><orcidid>https://orcid.org/0000-0002-5540-6011</orcidid><orcidid>https://orcid.org/0000000318829039</orcidid><orcidid>https://orcid.org/0000000168663677</orcidid><orcidid>https://orcid.org/0000000255406011</orcidid><orcidid>https://orcid.org/0000000249203293</orcidid><orcidid>https://orcid.org/0000000336664661</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | 639/301/119/2792 639/766/119/2792 Electromagnetism Hall effect Magnetic properties Magnetic structure Magnets Physics Physics and Astronomy Rare earth elements Room temperature Topology |
title | A topological kagome magnet in high entropy form |
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