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Hall effect in gated single-wall carbon nanotube films
The presence of hopping carriers and grain boundaries can sometimes lead to anomalous carrier types and density overestimation in Hall-effect measurements. Previous Hall-effect studies on carbon nanotube films reported unreasonably large carrier densities without independent assessments of the carri...
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Published in: | Scientific reports 2022-01, Vol.12 (1), p.101-101, Article 101 |
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creator | Yomogida, Yohei Horiuchi, Kanako Okada, Ryotaro Kawai, Hideki Ichinose, Yota Nishidome, Hiroyuki Ueji, Kan Komatsu, Natsumi Gao, Weilu Kono, Junichiro Yanagi, Kazuhiro |
description | The presence of hopping carriers and grain boundaries can sometimes lead to anomalous carrier types and density overestimation in Hall-effect measurements. Previous Hall-effect studies on carbon nanotube films reported unreasonably large carrier densities without independent assessments of the carrier types and densities. Here, we have systematically investigated the validity of Hall-effect results for a series of metallic, semiconducting, and metal–semiconductor-mixed single-wall carbon nanotube films. With carrier densities controlled through applied gate voltages, we were able to observe the Hall effect both in the
n
- and
p
-type regions, detecting opposite signs in the Hall coefficient. By comparing the obtained carrier types and densities against values derived from simultaneous field-effect-transistor measurements, we found that, while the Hall carrier types were always correct, the Hall carrier densities were overestimated by up to four orders of magnitude. This significant overestimation indicates that thin films of one-dimensional SWCNTs are quite different from conventional hopping transport systems. |
doi_str_mv | 10.1038/s41598-021-03911-7 |
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n
- and
p
-type regions, detecting opposite signs in the Hall coefficient. By comparing the obtained carrier types and densities against values derived from simultaneous field-effect-transistor measurements, we found that, while the Hall carrier types were always correct, the Hall carrier densities were overestimated by up to four orders of magnitude. This significant overestimation indicates that thin films of one-dimensional SWCNTs are quite different from conventional hopping transport systems.</description><identifier>ISSN: 2045-2322</identifier><identifier>EISSN: 2045-2322</identifier><identifier>DOI: 10.1038/s41598-021-03911-7</identifier><identifier>PMID: 34996961</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/301/1005/1007 ; 639/925/357/73 ; Carbon ; carbon nanotubes ; Electromagnetism ; electronic devices ; ENGINEERING ; fullerenes ; Humanities and Social Sciences ; multidisciplinary ; Science ; Science (multidisciplinary) ; Thin films</subject><ispartof>Scientific reports, 2022-01, Vol.12 (1), p.101-101, Article 101</ispartof><rights>The Author(s) 2022</rights><rights>2022. The Author(s).</rights><rights>The Author(s) 2022. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c633t-42a1f1d09a0e5b3ce192ad0ef959e6cc3982c68b14b9b53180dc071b628e0c913</citedby><cites>FETCH-LOGICAL-c633t-42a1f1d09a0e5b3ce192ad0ef959e6cc3982c68b14b9b53180dc071b628e0c913</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/2619578692/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2619578692?pq-origsite=primo$$EHTML$$P50$$Gproquest$$Hfree_for_read</linktohtml><link.rule.ids>230,314,727,780,784,885,25753,27924,27925,37012,37013,44590,53791,53793,75126</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/34996961$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://www.osti.gov/servlets/purl/1904647$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Yomogida, Yohei</creatorcontrib><creatorcontrib>Horiuchi, Kanako</creatorcontrib><creatorcontrib>Okada, Ryotaro</creatorcontrib><creatorcontrib>Kawai, Hideki</creatorcontrib><creatorcontrib>Ichinose, Yota</creatorcontrib><creatorcontrib>Nishidome, Hiroyuki</creatorcontrib><creatorcontrib>Ueji, Kan</creatorcontrib><creatorcontrib>Komatsu, Natsumi</creatorcontrib><creatorcontrib>Gao, Weilu</creatorcontrib><creatorcontrib>Kono, Junichiro</creatorcontrib><creatorcontrib>Yanagi, Kazuhiro</creatorcontrib><creatorcontrib>Rice Univ., Houston, TX (United States)</creatorcontrib><title>Hall effect in gated single-wall carbon nanotube films</title><title>Scientific reports</title><addtitle>Sci Rep</addtitle><addtitle>Sci Rep</addtitle><description>The presence of hopping carriers and grain boundaries can sometimes lead to anomalous carrier types and density overestimation in Hall-effect measurements. Previous Hall-effect studies on carbon nanotube films reported unreasonably large carrier densities without independent assessments of the carrier types and densities. Here, we have systematically investigated the validity of Hall-effect results for a series of metallic, semiconducting, and metal–semiconductor-mixed single-wall carbon nanotube films. With carrier densities controlled through applied gate voltages, we were able to observe the Hall effect both in the
n
- and
p
-type regions, detecting opposite signs in the Hall coefficient. By comparing the obtained carrier types and densities against values derived from simultaneous field-effect-transistor measurements, we found that, while the Hall carrier types were always correct, the Hall carrier densities were overestimated by up to four orders of magnitude. This significant overestimation indicates that thin films of one-dimensional SWCNTs are quite different from conventional hopping transport systems.</description><subject>639/301/1005/1007</subject><subject>639/925/357/73</subject><subject>Carbon</subject><subject>carbon nanotubes</subject><subject>Electromagnetism</subject><subject>electronic devices</subject><subject>ENGINEERING</subject><subject>fullerenes</subject><subject>Humanities and Social Sciences</subject><subject>multidisciplinary</subject><subject>Science</subject><subject>Science (multidisciplinary)</subject><subject>Thin films</subject><issn>2045-2322</issn><issn>2045-2322</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>PIMPY</sourceid><sourceid>DOA</sourceid><recordid>eNp9kstu1TAQhiMEolXpC7BAEWzYBDx24ssGCVX0IlViA2vLsSepj3LsYidUvD3OSSktC7yx5fn9zcV_Vb0G8gEIkx9zC52SDaHQEKYAGvGsOqak7RrKKH3-6HxUnea8I2V1VLWgXlZHrFWKKw7HFb8001TjMKCdax_q0czo6uzDOGFzt8asSX0MdTAhzkuP9eCnfX5VvRjMlPH0fj-pvp9_-XZ22Vx_vbg6-3zdWM7Y3LTUwACOKEOw65lFUNQ4goPqFHJrmZLUctlD26u-YyCJs0RAz6lEYhWwk-pq47podvo2-b1Jv3Q0Xh8uYhq1SbO3E2oiHHVWApjWtQCid447kLwcnZCtKKxPG-t26ffoLIY5mekJ9Gkk-Bs9xp9aijI10RXA2w0Q8-x1tn5Ge2NjCGV2GhRp-SHL-_ssKf5YMM9677PFaTIB45I15SApEx2szb37R7qLSwplnqtKdUJyRYuKbiqbYs4Jh4eKgejVCnqzgi5W0Acr6LWKN497fXjy5-OLgG2CXEJhxPQ393-wvwFmDLwn</recordid><startdate>20220107</startdate><enddate>20220107</enddate><creator>Yomogida, Yohei</creator><creator>Horiuchi, Kanako</creator><creator>Okada, Ryotaro</creator><creator>Kawai, Hideki</creator><creator>Ichinose, Yota</creator><creator>Nishidome, Hiroyuki</creator><creator>Ueji, Kan</creator><creator>Komatsu, Natsumi</creator><creator>Gao, Weilu</creator><creator>Kono, Junichiro</creator><creator>Yanagi, Kazuhiro</creator><general>Nature Publishing Group UK</general><general>Nature Publishing Group</general><general>Nature Portfolio</general><scope>C6C</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7X7</scope><scope>7XB</scope><scope>88A</scope><scope>88E</scope><scope>88I</scope><scope>8FE</scope><scope>8FH</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BBNVY</scope><scope>BENPR</scope><scope>BHPHI</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FYUFA</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K9.</scope><scope>LK8</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7P</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>Q9U</scope><scope>7X8</scope><scope>OIOZB</scope><scope>OTOTI</scope><scope>5PM</scope><scope>DOA</scope></search><sort><creationdate>20220107</creationdate><title>Hall effect in gated single-wall carbon nanotube films</title><author>Yomogida, Yohei ; 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Previous Hall-effect studies on carbon nanotube films reported unreasonably large carrier densities without independent assessments of the carrier types and densities. Here, we have systematically investigated the validity of Hall-effect results for a series of metallic, semiconducting, and metal–semiconductor-mixed single-wall carbon nanotube films. With carrier densities controlled through applied gate voltages, we were able to observe the Hall effect both in the
n
- and
p
-type regions, detecting opposite signs in the Hall coefficient. By comparing the obtained carrier types and densities against values derived from simultaneous field-effect-transistor measurements, we found that, while the Hall carrier types were always correct, the Hall carrier densities were overestimated by up to four orders of magnitude. This significant overestimation indicates that thin films of one-dimensional SWCNTs are quite different from conventional hopping transport systems.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>34996961</pmid><doi>10.1038/s41598-021-03911-7</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
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subjects | 639/301/1005/1007 639/925/357/73 Carbon carbon nanotubes Electromagnetism electronic devices ENGINEERING fullerenes Humanities and Social Sciences multidisciplinary Science Science (multidisciplinary) Thin films |
title | Hall effect in gated single-wall carbon nanotube films |
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