Ionic Liquid@Metal-Organic Framework as a Solid Electrolyte in a Lithium-Ion Battery: Current Performance and Perspective at Molecular Level

Searching for a suitable electrolyte in a lithium-ion battery is a challenging task. The electrolyte must not only be chemically and mechanically stable, but also be able to transport lithium ions efficiently. Ionic liquid incorporated into a metal-organic framework (IL@MOF) has currently emerged as...

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Bibliographic Details
Published in:Nanomaterials (Basel, Switzerland) Switzerland), 2022-03, Vol.12 (7), p.1076
Main Authors: Majid, Mohd Faridzuan, Mohd Zaid, Hayyiratul Fatimah, Kait, Chong Fai, Ahmad, Azizan, Jumbri, Khairulazhar
Format: Article
Language:English
Subjects:
Batteries
Computer applications
Electrochemical analysis
Electrochemistry
Electrodes
Electrolytes
ionic conductivity
ionic liquid
Ionic liquids
Lithium
Lithium-ion batteries
lithium-ion battery
metal-organic framework
Metal-organic frameworks
Phosphates
Polymers
Rechargeable batteries
Review
Solid electrolytes
solid-state electrolyte
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Summary:Searching for a suitable electrolyte in a lithium-ion battery is a challenging task. The electrolyte must not only be chemically and mechanically stable, but also be able to transport lithium ions efficiently. Ionic liquid incorporated into a metal-organic framework (IL@MOF) has currently emerged as an interesting class of hybrid material that could offer excellent electrochemical properties. However, the understanding of the mechanism and factors that govern its fast ionic conduction is crucial as well. In this review, the characteristics and potential use of IL@MOF as an electrolyte in a lithium-ion battery are highlighted. The importance of computational methods is emphasized as a comprehensive tool to investigate the atomistic behavior of IL@MOF and its interaction in electrochemical environments.
ISSN:2079-4991
2079-4991
DOI:10.3390/nano12071076