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The Structure, Property, and Ion Irradiation Effects of Pyrochlores: A Comprehensive Review
Since the beginning of the use of nuclear energy, humans have been faced with the problem of radionuclide disposal. At present, a large amount of waste is stored in pools or dry tanks at reactor sites. With the development of the nuclear power generation industry worldwide, the high storage cost (in...
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Published in: | Crystals (Basel) 2023-01, Vol.13 (1), p.143 |
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container_title | Crystals (Basel) |
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creator | Wang, Yuhao Jing, Chong Ding, Zhao-Ying Zhang, Yun-Zhuo Wei, Tao Ouyang, Jia-Hu Liu, Zhan-Guo Wang, Yu-Jin Wang, Ya-Ming |
description | Since the beginning of the use of nuclear energy, humans have been faced with the problem of radionuclide disposal. At present, a large amount of waste is stored in pools or dry tanks at reactor sites. With the development of the nuclear power generation industry worldwide, the high storage cost (including building, maintaining, and operating storage pools) is overwhelming and serious, and urgent radionuclide disposal problems have become increasingly difficult. Safe and economical strategies are urgently needed for long-term storage and disposal of nuclear waste, which has become among the core issues in the utilization of nuclear energy. Pyrochlore ceramics are able to immobilize a variety of radionuclides and have excellent irradiation stability, so they have received extensive attention as hosts of radionuclides waste. This review summarizes the structure, composition, synthesis process, properties, and irradiation stability of pyrochlore ceramics, focusing on the ion irradiation effect of pyrochlore. In general, the cation radii ratio rA/rB is a key parameter related to various properties of pyrochlores. Zirconate pyrochlore is more easily transformed from pyrochlore to defective fluorite, and leads to better irradiation resistance. |
doi_str_mv | 10.3390/cryst13010143 |
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At present, a large amount of waste is stored in pools or dry tanks at reactor sites. With the development of the nuclear power generation industry worldwide, the high storage cost (including building, maintaining, and operating storage pools) is overwhelming and serious, and urgent radionuclide disposal problems have become increasingly difficult. Safe and economical strategies are urgently needed for long-term storage and disposal of nuclear waste, which has become among the core issues in the utilization of nuclear energy. Pyrochlore ceramics are able to immobilize a variety of radionuclides and have excellent irradiation stability, so they have received extensive attention as hosts of radionuclides waste. This review summarizes the structure, composition, synthesis process, properties, and irradiation stability of pyrochlore ceramics, focusing on the ion irradiation effect of pyrochlore. In general, the cation radii ratio rA/rB is a key parameter related to various properties of pyrochlores. Zirconate pyrochlore is more easily transformed from pyrochlore to defective fluorite, and leads to better irradiation resistance.</description><identifier>ISSN: 2073-4352</identifier><identifier>EISSN: 2073-4352</identifier><identifier>DOI: 10.3390/cryst13010143</identifier><language>eng</language><publisher>Basel: MDPI AG</publisher><subject>Ceramics ; Fluorite ; Ion irradiation ; irradiation ; Laboratories ; Nuclear electric power generation ; Nuclear energy ; Nuclear fuels ; Nuclear power plants ; Nuclear reactor components ; Nuclear reactors ; Pools ; pyrochlore ; Pyrochlores ; Radiation ; radiation effect ; radiation model ; Radioactive wastes ; Radioisotopes ; Storage tanks ; waste form</subject><ispartof>Crystals (Basel), 2023-01, Vol.13 (1), p.143</ispartof><rights>2023 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). 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Zirconate pyrochlore is more easily transformed from pyrochlore to defective fluorite, and leads to better irradiation resistance.</description><subject>Ceramics</subject><subject>Fluorite</subject><subject>Ion irradiation</subject><subject>irradiation</subject><subject>Laboratories</subject><subject>Nuclear electric power generation</subject><subject>Nuclear energy</subject><subject>Nuclear fuels</subject><subject>Nuclear power plants</subject><subject>Nuclear reactor components</subject><subject>Nuclear reactors</subject><subject>Pools</subject><subject>pyrochlore</subject><subject>Pyrochlores</subject><subject>Radiation</subject><subject>radiation effect</subject><subject>radiation model</subject><subject>Radioactive wastes</subject><subject>Radioisotopes</subject><subject>Storage tanks</subject><subject>waste form</subject><issn>2073-4352</issn><issn>2073-4352</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>PIMPY</sourceid><sourceid>DOA</sourceid><recordid>eNpVkc1LAzEQxRdRUNSj94DXriaZ7GbjTYofBUHx4-QhpNmJ3dI2dZJW-t-7WhGdyzyGx28evKI4EfwMwPBzT5uUBXDBhYKd4kByDaWCSu7-0fvFcUpT3o-uudbioHh9niB7yrTyeUU4YA8Ul0h5M2Bu0bJRXLARkWs7l7teX4WAPicWA3vYUPSTWSRMF-ySDeN8STjBRerWyB5x3eHHUbEX3Czh8c8-LF6ur56Ht-Xd_c1oeHlXetA8lyCMDAZCI3HMAaSvxi3o0HhtKgktSKh1cNoEFVxdGdNL2QppVAAMSio4LEZbbhvd1C6pmzva2Og6-32I9GYd5c7P0ArOm6AFN0I2SnBoqmrMFYZxI9sqtF-s0y1rSfF9hSnbaVzRoo9vpa61ME2tmt5Vbl2eYkqE4fer4ParDvuvDvgEJbJ7ww</recordid><startdate>20230101</startdate><enddate>20230101</enddate><creator>Wang, Yuhao</creator><creator>Jing, Chong</creator><creator>Ding, Zhao-Ying</creator><creator>Zhang, Yun-Zhuo</creator><creator>Wei, Tao</creator><creator>Ouyang, Jia-Hu</creator><creator>Liu, Zhan-Guo</creator><creator>Wang, Yu-Jin</creator><creator>Wang, Ya-Ming</creator><general>MDPI AG</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>DOA</scope><orcidid>https://orcid.org/0000-0003-1764-5676</orcidid></search><sort><creationdate>20230101</creationdate><title>The Structure, Property, and Ion Irradiation Effects of Pyrochlores: A Comprehensive Review</title><author>Wang, Yuhao ; 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subjects | Ceramics Fluorite Ion irradiation irradiation Laboratories Nuclear electric power generation Nuclear energy Nuclear fuels Nuclear power plants Nuclear reactor components Nuclear reactors Pools pyrochlore Pyrochlores Radiation radiation effect radiation model Radioactive wastes Radioisotopes Storage tanks waste form |
title | The Structure, Property, and Ion Irradiation Effects of Pyrochlores: A Comprehensive Review |
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