Exploring the capture and desorption of CO2 on graphene oxide foams supported by computational calculations

In the last decade, the highest levels of greenhouse gases (GHG) in the atmosphere have been recorded, with carbon dioxide (CO 2 ) being one of the GHGs that most concerns mankind due to the rate at which it is generated on the planet. Given its long time of permanence in the atmosphere (between 100...

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Bibliographic Details
Published in:Scientific reports 2023-09, Vol.13 (1), p.14476-14476, Article 14476
Main Authors: Arango Hoyos, Bryan E., Osorio, H. Franco, Valencia Gómez, E. K., Guerrero Sánchez, J., Del Canto Palominos, A. P., Larrain, Felipe A., Prías Barragán, J. J.
Format: Article
Language:English
Subjects:
639/301/1034
639/638
639/638/169
639/638/563
704/172
704/172/169
Adsorption
Atmosphere
Carbon dioxide
Carbon sequestration
Chemical reactions
Clean technology
Desorption
Foams
Graphene
Greenhouse gases
Humanities and Social Sciences
multidisciplinary
Science
Science (multidisciplinary)
Silica
Silica gel
Zeolites
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Summary:In the last decade, the highest levels of greenhouse gases (GHG) in the atmosphere have been recorded, with carbon dioxide (CO 2 ) being one of the GHGs that most concerns mankind due to the rate at which it is generated on the planet. Given its long time of permanence in the atmosphere (between 100 to 150 years); this has deployed research in the scientific field focused on the absorption and desorption of CO 2 in the atmosphere. This work presents the study of CO 2 adsorption employing materials based on graphene oxide (GO), such as GO foams with different oxidation percentages (3.00%, 5.25%, and 9.00%) in their structure, obtained via an environmentally friendly method. The characterization of CO 2 adsorption was carried out in a closed system, within which were placed the GO foams and other CO 2 adsorbent materials (zeolite and silica gel). Through a controlled chemical reaction, production of CO 2 was conducted to obtain CO 2 concentration curves inside the system and calculate from these the efficiency, obtained between 86.28 and 92.20%, yield between 60.10 and 99.50%, and effectiveness of CO 2 adsorption of the materials under study. The results obtained suggest that GO foams are a promising material for carbon capture and the future development of a new clean technology, given their highest CO 2 adsorption efficiency and yield.
ISSN:2045-2322
2045-2322
DOI:10.1038/s41598-023-41683-4