Transient Kinetic Experiments within the High Conversion Domain: The Case of Ammonia Decomposition

In the development of catalytic materials, a set of standard conditions is needed where the kinetic performance of many samples can be compared. This can be challenging when a sample set covers a broad range of activity. Precise kinetic characterization requires uniformity in the gas and catalyst be...

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Bibliographic Details
Published in:Catalysts 2019-01, Vol.9 (1), p.104
Main Authors: Wang, Yixiao, Kunz, M., Siebers, Skyler, Rollins, Harry, Gleaves, John, Yablonsky, Gregory, Fushimi, Rebecca
Format: Article
Language:English
Subjects:
Advecting differential plug flow reactor
Ammonia
ammonia decomposition
Bimetals
Catalysts
Chemical elements
Chemical reactions
Cobalt
Composition
Conversion
Decomposition
Decomposition reactions
Experiments
Hydrogen production
Iron
MATERIALS SCIENCE
Microscopy
Nitrogen
PFR
Plug flow chemical reactors
TAP
TAP reactor
temporal analysis of products
Temporal Analysis of Products Reactor
Time dependence
transient kinetics
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Summary:In the development of catalytic materials, a set of standard conditions is needed where the kinetic performance of many samples can be compared. This can be challenging when a sample set covers a broad range of activity. Precise kinetic characterization requires uniformity in the gas and catalyst bed composition. This limits the range of convecting devices to low conversion (generally
ISSN:2073-4344
2073-4344
DOI:10.3390/catal9010104