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Volatile organic compound emissions from solvent- and water-borne coatings – compositional differences and tracer compound identifications
The emissions of volatile organic compounds (VOCs) from volatile chemical products (VCPs) – specifically personal care products, cleaning agents, coatings, adhesives, and pesticides – are emerging as the largest source of petroleum-derived organic carbon in US cities. Previous work has shown that th...
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| Published in: | Atmospheric chemistry and physics 2021-04, Vol.21 (8), p.6005-6022 |
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| container_title | Atmospheric chemistry and physics |
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| creator | Stockwell, Chelsea E Coggon, Matthew M Gkatzelis, Georgios I Ortega, John McDonald, Brian C Peischl, Jeff Aikin, Kenneth Gilman, Jessica B Trainer, Michael Warneke, Carsten |
| description | The emissions of volatile organic compounds (VOCs) from
volatile chemical products (VCPs) – specifically personal care products,
cleaning agents, coatings, adhesives, and pesticides – are emerging as the
largest source of petroleum-derived organic carbon in US cities. Previous
work has shown that the ambient concentration of markers for most VCP
categories correlates strongly with population density, except for VOCs
predominantly originating from solvent- and water-borne coatings (e.g.,
parachlorobenzotrifluoride (PCBTF) and Texanol®, respectively). Instead, these enhancements were dominated by distinct emission events likely driven by industrial usage patterns, such as
construction activity. In this work, the headspace of a variety of coating
products was analyzed using a proton-transfer-reaction time-of-flight mass
spectrometer (PTR-ToF-MS) and a gas chromatography (GC) preseparation
front end to identify composition differences for various coating types
(e.g., paints, primers, sealers, and stains). Evaporation experiments of
several products showed high initial VOC emission rates, and for the length
of these experiments, the majority of the VOC mass was emitted during the
first few hours following application. The percentage of mass emitted as
measured VOCs ( |
| doi_str_mv | 10.5194/acp-21-6005-2021 |
| format | article |
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volatile chemical products (VCPs) – specifically personal care products,
cleaning agents, coatings, adhesives, and pesticides – are emerging as the
largest source of petroleum-derived organic carbon in US cities. Previous
work has shown that the ambient concentration of markers for most VCP
categories correlates strongly with population density, except for VOCs
predominantly originating from solvent- and water-borne coatings (e.g.,
parachlorobenzotrifluoride (PCBTF) and Texanol®, respectively). Instead, these enhancements were dominated by distinct emission events likely driven by industrial usage patterns, such as
construction activity. In this work, the headspace of a variety of coating
products was analyzed using a proton-transfer-reaction time-of-flight mass
spectrometer (PTR-ToF-MS) and a gas chromatography (GC) preseparation
front end to identify composition differences for various coating types
(e.g., paints, primers, sealers, and stains). Evaporation experiments of
several products showed high initial VOC emission rates, and for the length
of these experiments, the majority of the VOC mass was emitted during the
first few hours following application. The percentage of mass emitted as
measured VOCs (<1 % to 83 %) mirrored the VOC content reported by
the manufacturer (<5 to 550 g L−1). Ambient and laboratory
measurements, usage trends, and ingredients compiled from architectural
coatings surveys show that both PCBTF and Texanol account for ∼10 % of the total VOC ingredient sales and, therefore, can be useful tracers for solvent- and water-borne coatings.</description><identifier>ISSN: 1680-7324</identifier><identifier>ISSN: 1680-7316</identifier><identifier>EISSN: 1680-7324</identifier><identifier>DOI: 10.5194/acp-21-6005-2021</identifier><language>eng</language><publisher>Katlenburg-Lindau: Copernicus GmbH</publisher><subject>Carbon ; Chemical compounds ; Cleaning ; Cleaning agents ; Coatings ; Consumer products ; Emission ; Emissions ; Environmental aspects ; Evaporation ; Evaporation rate ; Experiments ; Gas chromatography ; Headspace ; Hydrocarbons ; Industrial applications ; Laboratories ; Mass ; Mass spectrometry ; Molecular weight ; Organic carbon ; Organic compounds ; Personal grooming ; Pesticides ; Petroleum ; Population density ; Primers ; Primers (coatings) ; Protective coatings ; Reaction time ; Sealers ; Solvents ; Surveys ; Toiletries ; Tracers ; Tracers (Biology) ; Trends ; Urban areas ; VOCs ; Volatile organic compound emissions ; Volatile organic compounds ; Volatility</subject><ispartof>Atmospheric chemistry and physics, 2021-04, Vol.21 (8), p.6005-6022</ispartof><rights>COPYRIGHT 2021 Copernicus GmbH</rights><rights>2021. This work is published under https://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c546t-d77bfa63402e096b95a9d89db43aee40f75fbe347c382e99eb16436873c294df3</citedby><cites>FETCH-LOGICAL-c546t-d77bfa63402e096b95a9d89db43aee40f75fbe347c382e99eb16436873c294df3</cites><orcidid>0000-0002-9320-7101 ; 0000-0002-4608-3695 ; 0000-0003-3462-2126</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/2515691663/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2515691663?pq-origsite=primo$$EHTML$$P50$$Gproquest$$Hfree_for_read</linktohtml><link.rule.ids>314,780,784,864,2102,25753,27924,27925,37012,44590,75126</link.rule.ids></links><search><creatorcontrib>Stockwell, Chelsea E</creatorcontrib><creatorcontrib>Coggon, Matthew M</creatorcontrib><creatorcontrib>Gkatzelis, Georgios I</creatorcontrib><creatorcontrib>Ortega, John</creatorcontrib><creatorcontrib>McDonald, Brian C</creatorcontrib><creatorcontrib>Peischl, Jeff</creatorcontrib><creatorcontrib>Aikin, Kenneth</creatorcontrib><creatorcontrib>Gilman, Jessica B</creatorcontrib><creatorcontrib>Trainer, Michael</creatorcontrib><creatorcontrib>Warneke, Carsten</creatorcontrib><title>Volatile organic compound emissions from solvent- and water-borne coatings – compositional differences and tracer compound identifications</title><title>Atmospheric chemistry and physics</title><description>The emissions of volatile organic compounds (VOCs) from
volatile chemical products (VCPs) – specifically personal care products,
cleaning agents, coatings, adhesives, and pesticides – are emerging as the
largest source of petroleum-derived organic carbon in US cities. Previous
work has shown that the ambient concentration of markers for most VCP
categories correlates strongly with population density, except for VOCs
predominantly originating from solvent- and water-borne coatings (e.g.,
parachlorobenzotrifluoride (PCBTF) and Texanol®, respectively). Instead, these enhancements were dominated by distinct emission events likely driven by industrial usage patterns, such as
construction activity. In this work, the headspace of a variety of coating
products was analyzed using a proton-transfer-reaction time-of-flight mass
spectrometer (PTR-ToF-MS) and a gas chromatography (GC) preseparation
front end to identify composition differences for various coating types
(e.g., paints, primers, sealers, and stains). Evaporation experiments of
several products showed high initial VOC emission rates, and for the length
of these experiments, the majority of the VOC mass was emitted during the
first few hours following application. The percentage of mass emitted as
measured VOCs (<1 % to 83 %) mirrored the VOC content reported by
the manufacturer (<5 to 550 g L−1). Ambient and laboratory
measurements, usage trends, and ingredients compiled from architectural
coatings surveys show that both PCBTF and Texanol account for ∼10 % of the total VOC ingredient sales and, therefore, can be useful tracers for solvent- and water-borne coatings.</description><subject>Carbon</subject><subject>Chemical compounds</subject><subject>Cleaning</subject><subject>Cleaning agents</subject><subject>Coatings</subject><subject>Consumer products</subject><subject>Emission</subject><subject>Emissions</subject><subject>Environmental aspects</subject><subject>Evaporation</subject><subject>Evaporation rate</subject><subject>Experiments</subject><subject>Gas chromatography</subject><subject>Headspace</subject><subject>Hydrocarbons</subject><subject>Industrial applications</subject><subject>Laboratories</subject><subject>Mass</subject><subject>Mass spectrometry</subject><subject>Molecular weight</subject><subject>Organic carbon</subject><subject>Organic compounds</subject><subject>Personal grooming</subject><subject>Pesticides</subject><subject>Petroleum</subject><subject>Population density</subject><subject>Primers</subject><subject>Primers (coatings)</subject><subject>Protective coatings</subject><subject>Reaction time</subject><subject>Sealers</subject><subject>Solvents</subject><subject>Surveys</subject><subject>Toiletries</subject><subject>Tracers</subject><subject>Tracers (Biology)</subject><subject>Trends</subject><subject>Urban areas</subject><subject>VOCs</subject><subject>Volatile organic compound emissions</subject><subject>Volatile organic 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organic compound emissions from solvent- and water-borne coatings – compositional differences and tracer compound identifications</title><author>Stockwell, Chelsea E ; Coggon, Matthew M ; Gkatzelis, Georgios I ; Ortega, John ; McDonald, Brian C ; Peischl, Jeff ; Aikin, Kenneth ; Gilman, Jessica B ; Trainer, Michael ; Warneke, Carsten</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c546t-d77bfa63402e096b95a9d89db43aee40f75fbe347c382e99eb16436873c294df3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Carbon</topic><topic>Chemical compounds</topic><topic>Cleaning</topic><topic>Cleaning agents</topic><topic>Coatings</topic><topic>Consumer products</topic><topic>Emission</topic><topic>Emissions</topic><topic>Environmental aspects</topic><topic>Evaporation</topic><topic>Evaporation rate</topic><topic>Experiments</topic><topic>Gas 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E</au><au>Coggon, Matthew M</au><au>Gkatzelis, Georgios I</au><au>Ortega, John</au><au>McDonald, Brian C</au><au>Peischl, Jeff</au><au>Aikin, Kenneth</au><au>Gilman, Jessica B</au><au>Trainer, Michael</au><au>Warneke, Carsten</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Volatile organic compound emissions from solvent- and water-borne coatings – compositional differences and tracer compound identifications</atitle><jtitle>Atmospheric chemistry and physics</jtitle><date>2021-04-21</date><risdate>2021</risdate><volume>21</volume><issue>8</issue><spage>6005</spage><epage>6022</epage><pages>6005-6022</pages><issn>1680-7324</issn><issn>1680-7316</issn><eissn>1680-7324</eissn><abstract>The emissions of volatile organic compounds (VOCs) from
volatile chemical products (VCPs) – specifically personal care products,
cleaning agents, coatings, adhesives, and pesticides – are emerging as the
largest source of petroleum-derived organic carbon in US cities. Previous
work has shown that the ambient concentration of markers for most VCP
categories correlates strongly with population density, except for VOCs
predominantly originating from solvent- and water-borne coatings (e.g.,
parachlorobenzotrifluoride (PCBTF) and Texanol®, respectively). Instead, these enhancements were dominated by distinct emission events likely driven by industrial usage patterns, such as
construction activity. In this work, the headspace of a variety of coating
products was analyzed using a proton-transfer-reaction time-of-flight mass
spectrometer (PTR-ToF-MS) and a gas chromatography (GC) preseparation
front end to identify composition differences for various coating types
(e.g., paints, primers, sealers, and stains). Evaporation experiments of
several products showed high initial VOC emission rates, and for the length
of these experiments, the majority of the VOC mass was emitted during the
first few hours following application. The percentage of mass emitted as
measured VOCs (<1 % to 83 %) mirrored the VOC content reported by
the manufacturer (<5 to 550 g L−1). Ambient and laboratory
measurements, usage trends, and ingredients compiled from architectural
coatings surveys show that both PCBTF and Texanol account for ∼10 % of the total VOC ingredient sales and, therefore, can be useful tracers for solvent- and water-borne coatings.</abstract><cop>Katlenburg-Lindau</cop><pub>Copernicus GmbH</pub><doi>10.5194/acp-21-6005-2021</doi><tpages>18</tpages><orcidid>https://orcid.org/0000-0002-9320-7101</orcidid><orcidid>https://orcid.org/0000-0002-4608-3695</orcidid><orcidid>https://orcid.org/0000-0003-3462-2126</orcidid><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1680-7324 |
| ispartof | Atmospheric chemistry and physics, 2021-04, Vol.21 (8), p.6005-6022 |
| issn | 1680-7324 1680-7316 1680-7324 |
| language | eng |
| recordid | cdi_doaj_primary_oai_doaj_org_article_41ab602a22d84352a56402125f25fd2d |
| source | Publicly Available Content Database; DOAJ Directory of Open Access Journals; Alma/SFX Local Collection |
| subjects | Carbon Chemical compounds Cleaning Cleaning agents Coatings Consumer products Emission Emissions Environmental aspects Evaporation Evaporation rate Experiments Gas chromatography Headspace Hydrocarbons Industrial applications Laboratories Mass Mass spectrometry Molecular weight Organic carbon Organic compounds Personal grooming Pesticides Petroleum Population density Primers Primers (coatings) Protective coatings Reaction time Sealers Solvents Surveys Toiletries Tracers Tracers (Biology) Trends Urban areas VOCs Volatile organic compound emissions Volatile organic compounds Volatility |
| title | Volatile organic compound emissions from solvent- and water-borne coatings – compositional differences and tracer compound identifications |
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