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Ternary MOF-on-MOF heterostructures with controllable architectural and compositional complexity via multiple selective assembly
Assembly of different metal-organic framework (MOF) building blocks into hybrid MOF-on-MOF heterostructures is promising in chemistry and materials science, however the development of ternary MOF-on-MOF heterostructures with controllable architectural and compositional complexity is challenging. Her...
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Published in: | Nature communications 2020-10, Vol.11 (1), p.4971-4971, Article 4971 |
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description | Assembly of different metal-organic framework (MOF) building blocks into hybrid MOF-on-MOF heterostructures is promising in chemistry and materials science, however the development of ternary MOF-on-MOF heterostructures with controllable architectural and compositional complexity is challenging. Here we report the synthesis of three types of ternary MOF-on-MOF heterostructures via a multiple selective assembly strategy. This strategy relies on the choice of one host MOF with more than one facet that can arrange the growth of a guest MOF, where the arrangement is site-selective without homogenous growth of guest MOF or homogenous coating of guest on host MOF. The growth of guest MOF on a selected site of host MOF in each step provides the opportunity to further vary the combinations of arrangements in multiple steps, leading to ternary MOF-on-MOF heterostructures with tunable complexity. The developed strategy paves the way towards the rational design of intricate and unprecedented MOF-based superstructures for various applications.
Assembly of MOF-on-MOF hybrids with complex structures and properties is of interest, but achieving sophisticated ternary heterostructures is challenging. Here, the authors synthesize three types of ternary MOF-on-MOF heterostructures with tunable complexity via a multiple selective assembly strategy. |
doi_str_mv | 10.1038/s41467-020-18776-z |
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Assembly of MOF-on-MOF hybrids with complex structures and properties is of interest, but achieving sophisticated ternary heterostructures is challenging. Here, the authors synthesize three types of ternary MOF-on-MOF heterostructures with tunable complexity via a multiple selective assembly strategy.</description><identifier>ISSN: 2041-1723</identifier><identifier>EISSN: 2041-1723</identifier><identifier>DOI: 10.1038/s41467-020-18776-z</identifier><identifier>PMID: 33009408</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>147/135 ; 147/143 ; 639/301 ; 639/638 ; 639/925 ; Architecture ; Assembly ; Complexity ; Heterostructures ; Humanities and Social Sciences ; Hybrids ; Materials science ; Metal-organic frameworks ; Microscopy ; Morphology ; multidisciplinary ; Nanocrystals ; Science ; Science (multidisciplinary) ; Strategy ; Superstructures</subject><ispartof>Nature communications, 2020-10, Vol.11 (1), p.4971-4971, Article 4971</ispartof><rights>The Author(s) 2020</rights><rights>The Author(s) 2020. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c540t-2c2a9889e7444a99ed9c3d94793161e735817985f7a09deaf87b52da13d2c5033</citedby><cites>FETCH-LOGICAL-c540t-2c2a9889e7444a99ed9c3d94793161e735817985f7a09deaf87b52da13d2c5033</cites><orcidid>0000-0001-9435-8043 ; 0000-0003-3707-0785</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/2449451240/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2449451240?pq-origsite=primo$$EHTML$$P50$$Gproquest$$Hfree_for_read</linktohtml><link.rule.ids>230,314,727,780,784,885,25753,27924,27925,37012,37013,44590,53791,53793,75126</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/33009408$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Liu, Chao</creatorcontrib><creatorcontrib>Sun, Qiang</creatorcontrib><creatorcontrib>Lin, Lina</creatorcontrib><creatorcontrib>Wang, Jing</creatorcontrib><creatorcontrib>Zhang, Chaoqi</creatorcontrib><creatorcontrib>Xia, Chunhong</creatorcontrib><creatorcontrib>Bao, Tong</creatorcontrib><creatorcontrib>Wan, Jingjing</creatorcontrib><creatorcontrib>Huang, Rong</creatorcontrib><creatorcontrib>Zou, Jin</creatorcontrib><creatorcontrib>Yu, Chengzhong</creatorcontrib><title>Ternary MOF-on-MOF heterostructures with controllable architectural and compositional complexity via multiple selective assembly</title><title>Nature communications</title><addtitle>Nat Commun</addtitle><addtitle>Nat Commun</addtitle><description>Assembly of different metal-organic framework (MOF) building blocks into hybrid MOF-on-MOF heterostructures is promising in chemistry and materials science, however the development of ternary MOF-on-MOF heterostructures with controllable architectural and compositional complexity is challenging. Here we report the synthesis of three types of ternary MOF-on-MOF heterostructures via a multiple selective assembly strategy. This strategy relies on the choice of one host MOF with more than one facet that can arrange the growth of a guest MOF, where the arrangement is site-selective without homogenous growth of guest MOF or homogenous coating of guest on host MOF. The growth of guest MOF on a selected site of host MOF in each step provides the opportunity to further vary the combinations of arrangements in multiple steps, leading to ternary MOF-on-MOF heterostructures with tunable complexity. The developed strategy paves the way towards the rational design of intricate and unprecedented MOF-based superstructures for various applications.
Assembly of MOF-on-MOF hybrids with complex structures and properties is of interest, but achieving sophisticated ternary heterostructures is challenging. 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Commun</addtitle><date>2020-10-02</date><risdate>2020</risdate><volume>11</volume><issue>1</issue><spage>4971</spage><epage>4971</epage><pages>4971-4971</pages><artnum>4971</artnum><issn>2041-1723</issn><eissn>2041-1723</eissn><abstract>Assembly of different metal-organic framework (MOF) building blocks into hybrid MOF-on-MOF heterostructures is promising in chemistry and materials science, however the development of ternary MOF-on-MOF heterostructures with controllable architectural and compositional complexity is challenging. Here we report the synthesis of three types of ternary MOF-on-MOF heterostructures via a multiple selective assembly strategy. This strategy relies on the choice of one host MOF with more than one facet that can arrange the growth of a guest MOF, where the arrangement is site-selective without homogenous growth of guest MOF or homogenous coating of guest on host MOF. The growth of guest MOF on a selected site of host MOF in each step provides the opportunity to further vary the combinations of arrangements in multiple steps, leading to ternary MOF-on-MOF heterostructures with tunable complexity. The developed strategy paves the way towards the rational design of intricate and unprecedented MOF-based superstructures for various applications.
Assembly of MOF-on-MOF hybrids with complex structures and properties is of interest, but achieving sophisticated ternary heterostructures is challenging. Here, the authors synthesize three types of ternary MOF-on-MOF heterostructures with tunable complexity via a multiple selective assembly strategy.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>33009408</pmid><doi>10.1038/s41467-020-18776-z</doi><tpages>1</tpages><orcidid>https://orcid.org/0000-0001-9435-8043</orcidid><orcidid>https://orcid.org/0000-0003-3707-0785</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | 147/135 147/143 639/301 639/638 639/925 Architecture Assembly Complexity Heterostructures Humanities and Social Sciences Hybrids Materials science Metal-organic frameworks Microscopy Morphology multidisciplinary Nanocrystals Science Science (multidisciplinary) Strategy Superstructures |
title | Ternary MOF-on-MOF heterostructures with controllable architectural and compositional complexity via multiple selective assembly |
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