The Effect of Surface Confined Gold Nanoparticles in Blocking the Extraction of Nitrate by PVC-Based Polymer Inclusion Membranes Containing Aliquat 336 as the Carrier

Clusters of gold nanoparticles (AuNPs) formed on the surface of PVC-based polymer inclusion membranes (PIMs) with a liquid phase containing Aliquat 336 as the carrier and in some cases 1-dodecanol or 2-nitrophenol octyl ether as plasticizers were found to inhibit the extraction of nitrate by the PIM...

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Published in:Membranes (Basel) 2018-01, Vol.8 (1), p.6
Main Authors: Bonggotgetsakul, Ya Ya N, Cattrall, Robert W, Kolev, Spas D
Format: Article
Language:English
Subjects:
Aliquat
Aliquat 336
Dodecanol
Gold
gold nanoparticles (AuNPs)
Liquid phases
Membranes
Nanoparticles
nitrate extraction
Nitrates
Nitrophenol
Plasticizers
polymer inclusion membrane (PIM)
Polymers
Polyvinyl chloride
Powder injection molding
surface morphology
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creator Bonggotgetsakul, Ya Ya N
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description Clusters of gold nanoparticles (AuNPs) formed on the surface of PVC-based polymer inclusion membranes (PIMs) with a liquid phase containing Aliquat 336 as the carrier and in some cases 1-dodecanol or 2-nitrophenol octyl ether as plasticizers were found to inhibit the extraction of nitrate by the PIMs. This observation was based on gradually increasing the mass of AuNPs on the membrane surface and testing the ability of the membrane to extract nitrate after each increase. In this way, it was possible to determine the so-called "critical AuNP masses" at which the studied membranes ceased to extract nitrate. On the basis of these results, it can be hypothesized that the surfaces of these PIMs are not homogeneous with respect to the distribution of their membrane liquid phases, which are present only at certain sites. Extraction takes place only at these sites, and at the "critical AuNP mass" of a PIM, all these extraction sites are blocked and the membrane loses its ability to extract.
doi_str_mv 10.3390/membranes8010006
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source Publicly Available Content Database; PubMed Central
subjects Aliquat
Aliquat 336
Dodecanol
Gold
gold nanoparticles (AuNPs)
Liquid phases
Membranes
Nanoparticles
nitrate extraction
Nitrates
Nitrophenol
Plasticizers
polymer inclusion membrane (PIM)
Polymers
Polyvinyl chloride
Powder injection molding
surface morphology
title The Effect of Surface Confined Gold Nanoparticles in Blocking the Extraction of Nitrate by PVC-Based Polymer Inclusion Membranes Containing Aliquat 336 as the Carrier
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