Smart Materials for Environmental Remediation Based on Two-Component Gels: Room-Temperature-Phase-Selective Gelation for the Removal of Organic Pollutants Including Nitrobenzene/O-Dichlorobenzene, and Dye Molecules from the Wastewater

Novel two-component gel systems based on aliphatic acid–hydroxy/base interaction were developed as smart materials for environmental remediation. The G1-A16 gelator could be used directly as a powder form to selectively gel aromatic solvents (nitrobenzene and o-dichlorobenzene) from their mixtures w...

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Published in:Nanoscale research letters 2019-02, Vol.14 (1), p.42-10, Article 42
Main Authors: Zhang, Jing, Liu, Jiahui, Tong, Ciqing, Chen, Shipeng, Zhang, Baohao, Zhang, Bao, Song, Jian
Format: Article
Language:English
Subjects:
Aliphatic compounds
Aqueous solutions
Chemistry and Materials Science
Color removal
Dichlorobenzene
Dye removal
Dyes
Environmental cleanup
Environmental restoration
Gelation
Gels
Industrial applications
Industrial pollution
Materials Science
Molecular Medicine
Nano Express
Nanochemistry
Nanoscale Science and Technology
Nanotechnology
Nanotechnology and Microengineering
Nitrobenzene
NMR
Nuclear magnetic resonance
o-Dichlorobenzene
Pollutant removal
Pollutants
Powder
Remediation
Room temperature
Room-phase-selective-gelator (RPSG)
Self-healing
Shaking
Smart materials
Sodium
Sodium nitrate
Sodium sulfate
Solvents
Wastewater
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Zhang, Bao
Song, Jian
description Novel two-component gel systems based on aliphatic acid–hydroxy/base interaction were developed as smart materials for environmental remediation. The G1-A16 gelator could be used directly as a powder form to selectively gel aromatic solvents (nitrobenzene and o-dichlorobenzene) from their mixtures with wastewater (containing 0.5 M sodium nitrate and 0.5 M sodium sulfate) via a simple shaking strategy at room temperature without employing co-solvents and a heating–cooling process. Meanwhile, the two-component gel system can efficiently remove the toxic dyes from the aqueous solution. The dominant factors that drive gelation in the case of the gelator and nitrobenzene or water have been studied using FT-IR, 1 H NMR, and XRD. Overall, our research provides an efficient two-component approach for facilely tuning the properties of one-component gel for the realization of high-performance functionalities of gels. At the same time, our study demonstrates potential industrial application prospect in removing pollutants efficiently (such as aromatic solvents and toxic dye removal).
doi_str_mv 10.1186/s11671-019-2865-6
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subjects Aliphatic compounds
Aqueous solutions
Chemistry and Materials Science
Color removal
Dichlorobenzene
Dye removal
Dyes
Environmental cleanup
Environmental restoration
Gelation
Gels
Industrial applications
Industrial pollution
Materials Science
Molecular Medicine
Nano Express
Nanochemistry
Nanoscale Science and Technology
Nanotechnology
Nanotechnology and Microengineering
Nitrobenzene
NMR
Nuclear magnetic resonance
o-Dichlorobenzene
Pollutant removal
Pollutants
Powder
Remediation
Room temperature
Room-phase-selective-gelator (RPSG)
Self-healing
Shaking
Smart materials
Sodium
Sodium nitrate
Sodium sulfate
Solvents
Wastewater
title Smart Materials for Environmental Remediation Based on Two-Component Gels: Room-Temperature-Phase-Selective Gelation for the Removal of Organic Pollutants Including Nitrobenzene/O-Dichlorobenzene, and Dye Molecules from the Wastewater
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