Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet

• Published in: Nature communications 2024-08, Vol.15 (1), p.7264-10
• Main Authors: Park, Pyeongjae, Ghioldi, E. A., May, Andrew F., Kolopus, James A., Podlesnyak, Andrey A., Calder, Stuart, Paddison, Joseph A. M., Trumper, A. E., Manuel, L. O., Batista, Cristian D., Stone, Matthew B., Halász, Gábor B., Christianson, Andrew D.
• Format: Article
• Language: English
• Subjects: 639/301/119/997; 639/766/119/997; Anisotropy; Antiferromagnetism; Carbon dioxide; Cobalt; Excitation spectra; Frustrated magnetism; High temperature; Humanities and Social Sciences; Inelastic scattering; Lattice vibration; Magnetism; Magnons; Melting point; Melting points; multidisciplinary; Neutron scattering; Science; Science (multidisciplinary); Singularities; Spin dynamics; Spin liquid
• ISSN: 2041-1723; 2041-1723
• DOI: 10.1038/s41467-024-51618-w

The S  = 1/2 triangular lattice antiferromagnet (TLAF) is a paradigmatic example of frustrated quantum magnetism. An ongoing challenge involves understanding the influence of exchange anisotropy on the collective behavior within such systems. Using inelastic neutron scattering (INS) and advanced calculation techniques, we have studied the low and high-temperature spin dynamics of Ba 2 La 2 CoTe 2 O 12 (BLCTO): a Co 2+ -based J eff  = 1/2 TLAF that exhibits 120° order below T N  = 3.26 K. We determined the spin Hamiltonian by fitting the energy-resolved paramagnetic excitations measured at T  >  T N , revealing exceptionally strong easy-plane XXZ anisotropy. Below T N , the excitation spectrum exhibits a high energy continuum having a larger spectral weight than the single-magnon modes, suggesting a scenario characterized by a spinon confinement length that markedly exceeds the lattice spacing. We conjecture that this phenomenon arises from the proximity to a quantum melting point, even under strong easy-plane XXZ anisotropy. Finally, we highlight characteristic flat features in the excitation spectrum, which are connected to higher-order van Hove singularities in the magnon dispersion directly induced by easy-plane XXZ anisotropy. Our results provide a rare experimental insight into the nature of highly anisotropic S  = 1/2 TLAFs between the Heisenberg and XY limits. A TLAF is an archetypal geometrically frustrated magnetic system, which serves as the foundation for many exotic states, including quantum spin-liquids. Here, Park et al perform INS measurements on BLCTO, which, combined with theoretical calculations, reveal distinctive fingerprints of spinon excitations, thereby suggesting proximity to a spin liquid even in the presence of strong XXZ anisotropy.