Achieving stable Na metal cycling via polydopamine/multilayer graphene coating of a polypropylene separator

Sodium metal batteries are considered one of the most promising low-cost high-energy-density electrochemical energy storage systems. However, the growth of unfavourable Na metal deposition and the limited cell cycle life hamper the application of this battery system at a large scale. Here, we propos...

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Published in:Nature communications 2021-10, Vol.12 (1), p.5786-5786, Article 5786
Main Authors: Qin, Jieqiong, Shi, Haodong, Huang, Kai, Lu, Pengfei, Wen, Pengchao, Xing, Feifei, Yang, Bing, Ye, Mao, Yu, Yan, Wu, Zhong-Shuai
Format: Article
Language:English
Subjects:
147/135
147/143
147/3
639/301/299/891
639/4077/4079/891
639/638/675
639/925/357/1018
Batteries
Cell cycle
Coated electrodes
Coatings
Composite materials
Cycles
Electrochemistry
Energy storage
Graphene
Humanities and Social Sciences
Metals
multidisciplinary
Multilayers
Pollutant deposition
Polypropylene
Science
Science (multidisciplinary)
Separators
Sodium
Storage systems
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creator Qin, Jieqiong
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description Sodium metal batteries are considered one of the most promising low-cost high-energy-density electrochemical energy storage systems. However, the growth of unfavourable Na metal deposition and the limited cell cycle life hamper the application of this battery system at a large scale. Here, we propose the use of polypropylene separator coated with a composite material comprising polydopamine and multilayer graphene to tackle these issues. The oxygen- and nitrogen- containing moieties as well as the nano- and meso- porous network of the coating allow cycling of Na metal electrodes in symmetric cell configuration for over 2000 h with a stable 4 mV overpotential at 1 mA cm −2 . When tested in full Na || Na 3 V 2 (PO 4 ) 3 coin cell, the coated separator enables the delivery of a stable capacity of about 100 mAh g −1 for 500 cycles (90% capacity retention) at a specific current of 235 mA g −1 and satisfactory rate capability performances (i.e., 75 mAh g −1 at 3.5 A g −1 ). The development of future Na metal batteries relies on the cycling stability of the metallic anode. Here, the authors propose a polypropylene separator functionalized with polydopamine and multilayer graphene to enable stable and prolonged Na metal cell cycling.
doi_str_mv 10.1038/s41467-021-26032-1
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subjects 147/135
147/143
147/3
639/301/299/891
639/4077/4079/891
639/638/675
639/925/357/1018
Batteries
Cell cycle
Coated electrodes
Coatings
Composite materials
Cycles
Electrochemistry
Energy storage
Graphene
Humanities and Social Sciences
Metals
multidisciplinary
Multilayers
Pollutant deposition
Polypropylene
Science
Science (multidisciplinary)
Separators
Sodium
Storage systems
title Achieving stable Na metal cycling via polydopamine/multilayer graphene coating of a polypropylene separator
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