Quantum coherence controls the charge separation in a prototypical artificial light harvesting system

Ultrafast spectroscopy and quantum-dynamics simulations of an artificial sup ra mo lecu lar light-harvesting system - a supramolecular triad - provide strong evidence that the quantum-correlated wavelike motion of electrons and nuclei on a timescale of few tens of femtoseconds governs the ultrafast...

Full description

Saved in:
Bibliographic Details
Published in:EPJ Web of conferences 2013-01, Vol.41, p.8017-np
Main Authors: Falke, S.M., Rozzi, C. A., Spallanzani, N., Rubio, A., Molinari, E., Brida, D., Maiuri, M., Cerullo, G., Schramm, H., Christoffers, J., Lienau, C.
Format: Article
Language:English
Subjects:
Charge
Charge transfer
Coherence
Electronics
Femtosecond
Nuclei
Simulation
Spectroscopy
Citations: Items that this one cites
Online Access:Get full text
Tags: Add Tag
No Tags, Be the first to tag this record!
Description
Summary:Ultrafast spectroscopy and quantum-dynamics simulations of an artificial sup ra mo lecu lar light-harvesting system - a supramolecular triad - provide strong evidence that the quantum-correlated wavelike motion of electrons and nuclei on a timescale of few tens of femtoseconds governs the ultrafast electronic charge transfer.
ISSN:2100-014X
2100-014X
DOI:10.1051/epjconf/20134108017