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γ-BaFe2O4: a fresh playground for room temperature multiferroicity
Multiferroics, showing the coexistence of two or more ferroic orderings at room temperature, could harness a revolution in multifunctional devices. However, most of the multiferroic compounds known to date are not magnetically and electrically ordered at ambient conditions, so the discovery of new m...
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| Published in: | Nature communications 2022-12, Vol.13 (1), p.7968-10, Article 7968 |
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| creator | Orlandi, Fabio Delmonte, Davide Calestani, Gianluca Cavalli, Enrico Gilioli, Edmondo Shvartsman, Vladimir V. Graziosi, Patrizio Rampino, Stefano Spaggiari, Giulia Liu, Chao Ren, Wei Picozzi, Silvia Solzi, Massimo Casappa, Michele Mezzadri, Francesco |
| description | Multiferroics, showing the coexistence of two or more ferroic orderings at room temperature, could harness a revolution in multifunctional devices. However, most of the multiferroic compounds known to date are not magnetically and electrically ordered at ambient conditions, so the discovery of new materials is pivotal to allow the development of the field. In this work, we show that BaFe
2
O
4
is a previously unrecognized room temperature multiferroic. X-ray and neutron diffraction allowed to reveal the polar crystal structure of the compound as well as its antiferromagnetic behavior, confirmed by bulk magnetometry characterizations. Piezo force microscopy and electrical measurements show the polarization to be switchable by the application of an external field, while symmetry analysis and calculations based on density functional theory reveal the improper nature of the ferroelectric component. Considering the present findings, we propose BaFe
2
O
4
as a Bi- and Pb-free model for the search of new advanced multiferroic materials.
The application of multiferroics is often limited by low ordering temperatures. Here, the authors show that BaFe2O
4
is a room temperature antiferromagnet with improper ferroelectricity, suggesting it as a playground for the study of multiferroicity. |
| doi_str_mv | 10.1038/s41467-022-35669-5 |
| format | article |
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2
O
4
is a previously unrecognized room temperature multiferroic. X-ray and neutron diffraction allowed to reveal the polar crystal structure of the compound as well as its antiferromagnetic behavior, confirmed by bulk magnetometry characterizations. Piezo force microscopy and electrical measurements show the polarization to be switchable by the application of an external field, while symmetry analysis and calculations based on density functional theory reveal the improper nature of the ferroelectric component. Considering the present findings, we propose BaFe
2
O
4
as a Bi- and Pb-free model for the search of new advanced multiferroic materials.
The application of multiferroics is often limited by low ordering temperatures. Here, the authors show that BaFe2O
4
is a room temperature antiferromagnet with improper ferroelectricity, suggesting it as a playground for the study of multiferroicity.</description><identifier>ISSN: 2041-1723</identifier><identifier>EISSN: 2041-1723</identifier><identifier>DOI: 10.1038/s41467-022-35669-5</identifier><identifier>PMID: 36575166</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>119/118 ; 140/133 ; 147/3 ; 639/301/1005/1007 ; 639/301/1005/1008 ; Antiferromagnetism ; Coexistence ; Crystal structure ; Density functional theory ; Electrical measurement ; Ferroelectricity ; Humanities and Social Sciences ; Lead free ; Magnetic measurement ; multidisciplinary ; Multiferroic materials ; Neutron diffraction ; Playgrounds ; Room temperature ; Science ; Science (multidisciplinary) ; Temperature</subject><ispartof>Nature communications, 2022-12, Vol.13 (1), p.7968-10, Article 7968</ispartof><rights>The Author(s) 2022</rights><rights>The Author(s) 2022. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>2022. The Author(s).</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c517t-27c2918e321bcfcee9512e4e1678fd19d8028f1cf5dd07629671ff0fc92fa5cf3</citedby><cites>FETCH-LOGICAL-c517t-27c2918e321bcfcee9512e4e1678fd19d8028f1cf5dd07629671ff0fc92fa5cf3</cites><orcidid>0000-0001-7317-3867 ; 0000-0001-9505-1457 ; 0000-0001-9185-5925 ; 0000-0001-8402-412X ; 0000-0001-5367-527X ; 0000-0001-6333-521X ; 0000-0002-7155-2473 ; 0000-0002-9912-4534</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/2758459506/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2758459506?pq-origsite=primo$$EHTML$$P50$$Gproquest$$Hfree_for_read</linktohtml><link.rule.ids>230,314,727,780,784,885,25753,27924,27925,37012,37013,44590,53791,53793,75126</link.rule.ids></links><search><creatorcontrib>Orlandi, Fabio</creatorcontrib><creatorcontrib>Delmonte, Davide</creatorcontrib><creatorcontrib>Calestani, Gianluca</creatorcontrib><creatorcontrib>Cavalli, Enrico</creatorcontrib><creatorcontrib>Gilioli, Edmondo</creatorcontrib><creatorcontrib>Shvartsman, Vladimir V.</creatorcontrib><creatorcontrib>Graziosi, Patrizio</creatorcontrib><creatorcontrib>Rampino, Stefano</creatorcontrib><creatorcontrib>Spaggiari, Giulia</creatorcontrib><creatorcontrib>Liu, Chao</creatorcontrib><creatorcontrib>Ren, Wei</creatorcontrib><creatorcontrib>Picozzi, Silvia</creatorcontrib><creatorcontrib>Solzi, Massimo</creatorcontrib><creatorcontrib>Casappa, Michele</creatorcontrib><creatorcontrib>Mezzadri, Francesco</creatorcontrib><title>γ-BaFe2O4: a fresh playground for room temperature multiferroicity</title><title>Nature communications</title><addtitle>Nat Commun</addtitle><description>Multiferroics, showing the coexistence of two or more ferroic orderings at room temperature, could harness a revolution in multifunctional devices. However, most of the multiferroic compounds known to date are not magnetically and electrically ordered at ambient conditions, so the discovery of new materials is pivotal to allow the development of the field. In this work, we show that BaFe
2
O
4
is a previously unrecognized room temperature multiferroic. X-ray and neutron diffraction allowed to reveal the polar crystal structure of the compound as well as its antiferromagnetic behavior, confirmed by bulk magnetometry characterizations. Piezo force microscopy and electrical measurements show the polarization to be switchable by the application of an external field, while symmetry analysis and calculations based on density functional theory reveal the improper nature of the ferroelectric component. Considering the present findings, we propose BaFe
2
O
4
as a Bi- and Pb-free model for the search of new advanced multiferroic materials.
The application of multiferroics is often limited by low ordering temperatures. Here, the authors show that BaFe2O
4
is a room temperature antiferromagnet with improper ferroelectricity, suggesting it as a playground for the study of multiferroicity.</description><subject>119/118</subject><subject>140/133</subject><subject>147/3</subject><subject>639/301/1005/1007</subject><subject>639/301/1005/1008</subject><subject>Antiferromagnetism</subject><subject>Coexistence</subject><subject>Crystal structure</subject><subject>Density functional theory</subject><subject>Electrical measurement</subject><subject>Ferroelectricity</subject><subject>Humanities and Social Sciences</subject><subject>Lead free</subject><subject>Magnetic measurement</subject><subject>multidisciplinary</subject><subject>Multiferroic materials</subject><subject>Neutron diffraction</subject><subject>Playgrounds</subject><subject>Room temperature</subject><subject>Science</subject><subject>Science 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Francesco</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>γ-BaFe2O4: a fresh playground for room temperature multiferroicity</atitle><jtitle>Nature communications</jtitle><stitle>Nat Commun</stitle><date>2022-12-27</date><risdate>2022</risdate><volume>13</volume><issue>1</issue><spage>7968</spage><epage>10</epage><pages>7968-10</pages><artnum>7968</artnum><issn>2041-1723</issn><eissn>2041-1723</eissn><abstract>Multiferroics, showing the coexistence of two or more ferroic orderings at room temperature, could harness a revolution in multifunctional devices. However, most of the multiferroic compounds known to date are not magnetically and electrically ordered at ambient conditions, so the discovery of new materials is pivotal to allow the development of the field. In this work, we show that BaFe
2
O
4
is a previously unrecognized room temperature multiferroic. X-ray and neutron diffraction allowed to reveal the polar crystal structure of the compound as well as its antiferromagnetic behavior, confirmed by bulk magnetometry characterizations. Piezo force microscopy and electrical measurements show the polarization to be switchable by the application of an external field, while symmetry analysis and calculations based on density functional theory reveal the improper nature of the ferroelectric component. Considering the present findings, we propose BaFe
2
O
4
as a Bi- and Pb-free model for the search of new advanced multiferroic materials.
The application of multiferroics is often limited by low ordering temperatures. Here, the authors show that BaFe2O
4
is a room temperature antiferromagnet with improper ferroelectricity, suggesting it as a playground for the study of multiferroicity.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>36575166</pmid><doi>10.1038/s41467-022-35669-5</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0001-7317-3867</orcidid><orcidid>https://orcid.org/0000-0001-9505-1457</orcidid><orcidid>https://orcid.org/0000-0001-9185-5925</orcidid><orcidid>https://orcid.org/0000-0001-8402-412X</orcidid><orcidid>https://orcid.org/0000-0001-5367-527X</orcidid><orcidid>https://orcid.org/0000-0001-6333-521X</orcidid><orcidid>https://orcid.org/0000-0002-7155-2473</orcidid><orcidid>https://orcid.org/0000-0002-9912-4534</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | 119/118 140/133 147/3 639/301/1005/1007 639/301/1005/1008 Antiferromagnetism Coexistence Crystal structure Density functional theory Electrical measurement Ferroelectricity Humanities and Social Sciences Lead free Magnetic measurement multidisciplinary Multiferroic materials Neutron diffraction Playgrounds Room temperature Science Science (multidisciplinary) Temperature |
| title | γ-BaFe2O4: a fresh playground for room temperature multiferroicity |
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