Characterization of a Continuous Muon Source for the Non-Destructive and Depth-Selective Elemental Composition Analysis by Muon Induced X- and Gamma-rays

• Published in: Applied sciences 2022-03, Vol.12 (5), p.2541
• Main Authors: Biswas, Sayani, Gerchow, Lars, Luetkens, Hubertus, Prokscha, Thomas, Antognini, Aldo, Berger, Niklaus, Cocolios, Thomas Elias, Dressler, Rugard, Indelicato, Paul, Jungmann, Klaus, Kirch, Klaus, Knecht, Andreas, Papa, Angela, Pohl, Randolf, Pospelov, Maxim, Rapisarda, Elisa, Reiter, Peter, Ritjoho, Narongrit, Roccia, Stephanie, Severijns, Nathal, Skawran, Alexander, Vogiatzi, Stergiani Marina, Wauters, Frederik, Willmann, Lorenz, Amato, Alex
• Format: Article
• Language: English
• Subjects: Chemical analysis; Chemical composition; Composition; Continuous beams; continuous muon beam; Data points; depth-dependent elemental analysis; Energy; Gamma rays; Muons; negative muon induced X-ray emission; non-destructive technique; Nuclear capture; Nuclear Theory; Particle beams; Physics; Probability; sandwich sample; Scientific imaging; Signal to noise ratio; Statistical methods; X-rays
• ISSN: 2076-3417; 2076-3417
• DOI: 10.3390/app12052541

The toolbox for material characterization has never been richer than today. Great progress with all kinds of particles and interaction methods provide access to nearly all properties of an object under study. However, a tomographic analysis of the subsurface region remains still a challenge today. In this regard, the Muon Induced X-ray Emission (MIXE) technique has seen rebirth fueled by the availability of high intensity muon beams. We report here a study conducted at the Paul Scherrer Institute (PSI). It demonstrates that the absence of any beam time-structure leads to low pile-up events and a high signal-to-noise ratio (SNR) with less than one hour acquisition time per sample or data point. This performance creates the perspective to open this technique to a wider audience for the routine investigation of non-destructive and depth-sensitive elemental compositions, for example in rare and precious samples. Using a hetero-structured sample of known elements and thicknesses, we successfully detected the characteristic muonic X-rays, emitted during the capture of a negative muon by an atom, and the gamma-rays resulting from the nuclear capture of the muon, characterizing the capabilities of MIXE at PSI. This sample emphasizes the quality of a continuous beam, and the exceptional SNR at high rates. Such sensitivity will enable totally new statistically intense aspects in the field of MIXE, e.g., elemental 3D-tomography and chemical analysis. Therefore, we are currently advancing our proof-of-concept experiments with the goal of creating a full fledged permanently operated user station to make MIXE available to the wider scientific community as well as industry.