Loading…
Microstructure and Corrosion Characterization of a MgO/Hydroxyapatite Bilayer Coating by Plasma Electrolytic Oxidation Coupled with Flame Spraying on a Mg Alloy
Thermally sprayed hydroxyapatite coatings are one of the main strategies to improve the bioactivation of metal implants. However, the naturally low corrosion resistance of these coatings is the main challenge for their use. In this study, plasma electrolytic oxidation (PEO) was used to create an int...
Saved in:
Published in: | ACS omega 2020-09, Vol.5 (38), p.24186-24194 |
---|---|
Main Authors: | , , , , , , |
Format: | Article |
Language: | English |
Citations: | Items that this one cites Items that cite this one |
Online Access: | Get full text |
Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
cited_by | cdi_FETCH-LOGICAL-a476t-35a60465fe77d8c3d669ffabf89463879cf2c7068fa1657af8800e983ffd25f53 |
---|---|
cites | cdi_FETCH-LOGICAL-a476t-35a60465fe77d8c3d669ffabf89463879cf2c7068fa1657af8800e983ffd25f53 |
container_end_page | 24194 |
container_issue | 38 |
container_start_page | 24186 |
container_title | ACS omega |
container_volume | 5 |
creator | Mardali, Marzieh Salimijazi, Hamidreza Karimzadeh, Fathallah Blawert, Carsten Luthringer-Feyerabend, Bérengère J. C Fazel, Mohammad Safarbali, Babak |
description | Thermally sprayed hydroxyapatite coatings are one of the main strategies to improve the bioactivation of metal implants. However, the naturally low corrosion resistance of these coatings is the main challenge for their use. In this study, plasma electrolytic oxidation (PEO) was used to create an intermediate layer. The anodization process was used for comparison. According to the polarization curves, the PEO layer was more effective than the anodized layer in reducing the corrosion current density (I corr of 0.05 × 10–9 A/cm2 vs I corr of 0.05 A/cm2). The results of electrochemical impedance spectroscopy showed higher resistance of the sample with a PEO interlayer than that of the sample with an anodized interlayer. The results of the hydrogen evolution test revealed that the PEO layer as a middle layer served as the main barrier for reducing the magnesium corrosion rate, especially during the initial immersion time. |
doi_str_mv | 10.1021/acsomega.0c01574 |
format | article |
fullrecord | <record><control><sourceid>proquest_doaj_</sourceid><recordid>TN_cdi_doaj_primary_oai_doaj_org_article_85ee9f7a51864503b2d7b0a29aad022e</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><doaj_id>oai_doaj_org_article_85ee9f7a51864503b2d7b0a29aad022e</doaj_id><sourcerecordid>2448635544</sourcerecordid><originalsourceid>FETCH-LOGICAL-a476t-35a60465fe77d8c3d669ffabf89463879cf2c7068fa1657af8800e983ffd25f53</originalsourceid><addsrcrecordid>eNp1kktv1DAUhSMEolXpnqWXLJjW8TsbpDJqaaVWgwSsrTt-zGTkxIPjQMOv4afiMAOiC1a2z7nnu7J9q-p1jS9qTOpLMEPs3AYusME1l-xZdUqYxIuaMvr8n_1JdT4MO4xxLRRRRLysTigtCUbZafXzoTUpDjmNJo_JIegtWsZUpDb2aLmFBCa71P6APAvRI0APm9Xl7WRTfJxgX_Ts0Ps2wORSiZZzv0HrCX0MMHSAroMzOcUw5dag1WNrD6BlHPfBWfS9zVt0E6Bz6NM-wTSHiz03QVchxOlV9cJDGNz5cT2rvtxcf17eLu5XH-6WV_cLYFLkBeUgMBPcOymtMtQK0XgPa68aJqiSjfHESCyUh1pwCV4pjF2jqPeWcM_pWXV34NoIO71PbQdp0hFa_VuIaaMhlTsEpxV3rvESeK0E45iuiZVrDKQBsJgQV1jvDqz9uO6cNa7PCcIT6FOnb7d6E79pyYmqJSmAN0dAil9HN2TdtYNxIUDv4jhowpgSlHPGSik-lM7fOCTn_7apsZ7nRP-ZE32ckxJ5e4gUR-_imPrysP8v_wUtjMN2</addsrcrecordid><sourcetype>Open Website</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2448635544</pqid></control><display><type>article</type><title>Microstructure and Corrosion Characterization of a MgO/Hydroxyapatite Bilayer Coating by Plasma Electrolytic Oxidation Coupled with Flame Spraying on a Mg Alloy</title><source>PubMed Central(OpenAccess)</source><source>American Chemical Society (ACS) Open Access</source><creator>Mardali, Marzieh ; Salimijazi, Hamidreza ; Karimzadeh, Fathallah ; Blawert, Carsten ; Luthringer-Feyerabend, Bérengère J. C ; Fazel, Mohammad ; Safarbali, Babak</creator><creatorcontrib>Mardali, Marzieh ; Salimijazi, Hamidreza ; Karimzadeh, Fathallah ; Blawert, Carsten ; Luthringer-Feyerabend, Bérengère J. C ; Fazel, Mohammad ; Safarbali, Babak</creatorcontrib><description>Thermally sprayed hydroxyapatite coatings are one of the main strategies to improve the bioactivation of metal implants. However, the naturally low corrosion resistance of these coatings is the main challenge for their use. In this study, plasma electrolytic oxidation (PEO) was used to create an intermediate layer. The anodization process was used for comparison. According to the polarization curves, the PEO layer was more effective than the anodized layer in reducing the corrosion current density (I corr of 0.05 × 10–9 A/cm2 vs I corr of 0.05 A/cm2). The results of electrochemical impedance spectroscopy showed higher resistance of the sample with a PEO interlayer than that of the sample with an anodized interlayer. The results of the hydrogen evolution test revealed that the PEO layer as a middle layer served as the main barrier for reducing the magnesium corrosion rate, especially during the initial immersion time.</description><identifier>ISSN: 2470-1343</identifier><identifier>EISSN: 2470-1343</identifier><identifier>DOI: 10.1021/acsomega.0c01574</identifier><identifier>PMID: 33015434</identifier><language>eng</language><publisher>American Chemical Society</publisher><ispartof>ACS omega, 2020-09, Vol.5 (38), p.24186-24194</ispartof><rights>2020 American Chemical Society</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a476t-35a60465fe77d8c3d669ffabf89463879cf2c7068fa1657af8800e983ffd25f53</citedby><cites>FETCH-LOGICAL-a476t-35a60465fe77d8c3d669ffabf89463879cf2c7068fa1657af8800e983ffd25f53</cites><orcidid>0000-0002-3269-8584 ; 0000-0003-4629-3008</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acsomega.0c01574$$EPDF$$P50$$Gacs$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acsomega.0c01574$$EHTML$$P50$$Gacs$$Hfree_for_read</linktohtml><link.rule.ids>230,314,727,780,784,885,27080,27924,27925,53791,53793,56762,56812</link.rule.ids></links><search><creatorcontrib>Mardali, Marzieh</creatorcontrib><creatorcontrib>Salimijazi, Hamidreza</creatorcontrib><creatorcontrib>Karimzadeh, Fathallah</creatorcontrib><creatorcontrib>Blawert, Carsten</creatorcontrib><creatorcontrib>Luthringer-Feyerabend, Bérengère J. C</creatorcontrib><creatorcontrib>Fazel, Mohammad</creatorcontrib><creatorcontrib>Safarbali, Babak</creatorcontrib><title>Microstructure and Corrosion Characterization of a MgO/Hydroxyapatite Bilayer Coating by Plasma Electrolytic Oxidation Coupled with Flame Spraying on a Mg Alloy</title><title>ACS omega</title><addtitle>ACS Omega</addtitle><description>Thermally sprayed hydroxyapatite coatings are one of the main strategies to improve the bioactivation of metal implants. However, the naturally low corrosion resistance of these coatings is the main challenge for their use. In this study, plasma electrolytic oxidation (PEO) was used to create an intermediate layer. The anodization process was used for comparison. According to the polarization curves, the PEO layer was more effective than the anodized layer in reducing the corrosion current density (I corr of 0.05 × 10–9 A/cm2 vs I corr of 0.05 A/cm2). The results of electrochemical impedance spectroscopy showed higher resistance of the sample with a PEO interlayer than that of the sample with an anodized interlayer. The results of the hydrogen evolution test revealed that the PEO layer as a middle layer served as the main barrier for reducing the magnesium corrosion rate, especially during the initial immersion time.</description><issn>2470-1343</issn><issn>2470-1343</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>N~.</sourceid><sourceid>DOA</sourceid><recordid>eNp1kktv1DAUhSMEolXpnqWXLJjW8TsbpDJqaaVWgwSsrTt-zGTkxIPjQMOv4afiMAOiC1a2z7nnu7J9q-p1jS9qTOpLMEPs3AYusME1l-xZdUqYxIuaMvr8n_1JdT4MO4xxLRRRRLysTigtCUbZafXzoTUpDjmNJo_JIegtWsZUpDb2aLmFBCa71P6APAvRI0APm9Xl7WRTfJxgX_Ts0Ps2wORSiZZzv0HrCX0MMHSAroMzOcUw5dag1WNrD6BlHPfBWfS9zVt0E6Bz6NM-wTSHiz03QVchxOlV9cJDGNz5cT2rvtxcf17eLu5XH-6WV_cLYFLkBeUgMBPcOymtMtQK0XgPa68aJqiSjfHESCyUh1pwCV4pjF2jqPeWcM_pWXV34NoIO71PbQdp0hFa_VuIaaMhlTsEpxV3rvESeK0E45iuiZVrDKQBsJgQV1jvDqz9uO6cNa7PCcIT6FOnb7d6E79pyYmqJSmAN0dAil9HN2TdtYNxIUDv4jhowpgSlHPGSik-lM7fOCTn_7apsZ7nRP-ZE32ckxJ5e4gUR-_imPrysP8v_wUtjMN2</recordid><startdate>20200929</startdate><enddate>20200929</enddate><creator>Mardali, Marzieh</creator><creator>Salimijazi, Hamidreza</creator><creator>Karimzadeh, Fathallah</creator><creator>Blawert, Carsten</creator><creator>Luthringer-Feyerabend, Bérengère J. C</creator><creator>Fazel, Mohammad</creator><creator>Safarbali, Babak</creator><general>American Chemical Society</general><scope>N~.</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>5PM</scope><scope>DOA</scope><orcidid>https://orcid.org/0000-0002-3269-8584</orcidid><orcidid>https://orcid.org/0000-0003-4629-3008</orcidid></search><sort><creationdate>20200929</creationdate><title>Microstructure and Corrosion Characterization of a MgO/Hydroxyapatite Bilayer Coating by Plasma Electrolytic Oxidation Coupled with Flame Spraying on a Mg Alloy</title><author>Mardali, Marzieh ; Salimijazi, Hamidreza ; Karimzadeh, Fathallah ; Blawert, Carsten ; Luthringer-Feyerabend, Bérengère J. C ; Fazel, Mohammad ; Safarbali, Babak</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a476t-35a60465fe77d8c3d669ffabf89463879cf2c7068fa1657af8800e983ffd25f53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Mardali, Marzieh</creatorcontrib><creatorcontrib>Salimijazi, Hamidreza</creatorcontrib><creatorcontrib>Karimzadeh, Fathallah</creatorcontrib><creatorcontrib>Blawert, Carsten</creatorcontrib><creatorcontrib>Luthringer-Feyerabend, Bérengère J. C</creatorcontrib><creatorcontrib>Fazel, Mohammad</creatorcontrib><creatorcontrib>Safarbali, Babak</creatorcontrib><collection>American Chemical Society (ACS) Open Access</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>PubMed Central (Full Participant titles)</collection><collection>DOAJ Directory of Open Access Journals</collection><jtitle>ACS omega</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Mardali, Marzieh</au><au>Salimijazi, Hamidreza</au><au>Karimzadeh, Fathallah</au><au>Blawert, Carsten</au><au>Luthringer-Feyerabend, Bérengère J. C</au><au>Fazel, Mohammad</au><au>Safarbali, Babak</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Microstructure and Corrosion Characterization of a MgO/Hydroxyapatite Bilayer Coating by Plasma Electrolytic Oxidation Coupled with Flame Spraying on a Mg Alloy</atitle><jtitle>ACS omega</jtitle><addtitle>ACS Omega</addtitle><date>2020-09-29</date><risdate>2020</risdate><volume>5</volume><issue>38</issue><spage>24186</spage><epage>24194</epage><pages>24186-24194</pages><issn>2470-1343</issn><eissn>2470-1343</eissn><abstract>Thermally sprayed hydroxyapatite coatings are one of the main strategies to improve the bioactivation of metal implants. However, the naturally low corrosion resistance of these coatings is the main challenge for their use. In this study, plasma electrolytic oxidation (PEO) was used to create an intermediate layer. The anodization process was used for comparison. According to the polarization curves, the PEO layer was more effective than the anodized layer in reducing the corrosion current density (I corr of 0.05 × 10–9 A/cm2 vs I corr of 0.05 A/cm2). The results of electrochemical impedance spectroscopy showed higher resistance of the sample with a PEO interlayer than that of the sample with an anodized interlayer. The results of the hydrogen evolution test revealed that the PEO layer as a middle layer served as the main barrier for reducing the magnesium corrosion rate, especially during the initial immersion time.</abstract><pub>American Chemical Society</pub><pmid>33015434</pmid><doi>10.1021/acsomega.0c01574</doi><tpages>9</tpages><orcidid>https://orcid.org/0000-0002-3269-8584</orcidid><orcidid>https://orcid.org/0000-0003-4629-3008</orcidid><oa>free_for_read</oa></addata></record> |
fulltext | fulltext |
identifier | ISSN: 2470-1343 |
ispartof | ACS omega, 2020-09, Vol.5 (38), p.24186-24194 |
issn | 2470-1343 2470-1343 |
language | eng |
recordid | cdi_doaj_primary_oai_doaj_org_article_85ee9f7a51864503b2d7b0a29aad022e |
source | PubMed Central(OpenAccess); American Chemical Society (ACS) Open Access |
title | Microstructure and Corrosion Characterization of a MgO/Hydroxyapatite Bilayer Coating by Plasma Electrolytic Oxidation Coupled with Flame Spraying on a Mg Alloy |
url | http://sfxeu10.hosted.exlibrisgroup.com/loughborough?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-29T13%3A44%3A10IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_doaj_&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Microstructure%20and%20Corrosion%20Characterization%20of%20a%20MgO/Hydroxyapatite%20Bilayer%20Coating%20by%20Plasma%20Electrolytic%20Oxidation%20Coupled%20with%20Flame%20Spraying%20on%20a%20Mg%20Alloy&rft.jtitle=ACS%20omega&rft.au=Mardali,%20Marzieh&rft.date=2020-09-29&rft.volume=5&rft.issue=38&rft.spage=24186&rft.epage=24194&rft.pages=24186-24194&rft.issn=2470-1343&rft.eissn=2470-1343&rft_id=info:doi/10.1021/acsomega.0c01574&rft_dat=%3Cproquest_doaj_%3E2448635544%3C/proquest_doaj_%3E%3Cgrp_id%3Ecdi_FETCH-LOGICAL-a476t-35a60465fe77d8c3d669ffabf89463879cf2c7068fa1657af8800e983ffd25f53%3C/grp_id%3E%3Coa%3E%3C/oa%3E%3Curl%3E%3C/url%3E&rft_id=info:oai/&rft_pqid=2448635544&rft_id=info:pmid/33015434&rfr_iscdi=true |