Fabrication of Loose Nanofiltration Membranes with High Rejection Selectivity between Natural Organic Matter and Salts for Drinking Water Treatment

Loose nanofiltration (LNF) membranes with a molecular weight cut-off (MWCO) of about 1000 Da and high surface negative charge density have great application potential for drinking water treatment pursuing high rejection selectivity between natural organic matter (NOM) and mineral salts. This study w...

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Published in:Membranes (Basel) 2022-09, Vol.12 (9), p.887
Main Authors: He, Zhihai, Wang, Kunpeng, Liu, Yanling, Zhang, Ting, Wang, Xiaomao
Format: Article
Language:English
Subjects:
Charge density
Drinking water
Fabrication
Humic acid
interfacial polymerization (IP)
loose nanofiltration (LNF)
Membranes
Microscopy
Molecular weight
Nanofiltration
Nanotechnology
natural organic matter (NOM)
non-solvent induced phase separation (NIPS)
Organic matter
Phase separation
Piperazine
Polyethersulfones
Polyethylene glycol
Purification
Rejection
rejection selectivity
Reluctance
Salts
Selectivity
Surface charge
Water
Water purification
Water treatment
Water treatment plants
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description Loose nanofiltration (LNF) membranes with a molecular weight cut-off (MWCO) of about 1000 Da and high surface negative charge density have great application potential for drinking water treatment pursuing high rejection selectivity between natural organic matter (NOM) and mineral salts. This study was conducted to exploit the novel method coupling non-solvent induced phase separation (NIPS) and interfacial polymerization (IP) for the preparation of high-performance LNF membranes. A number of LNF membranes were synthesized by varying the polyethersulfone (PES) and piperazine (PIP) concentrations in the cast solution for the PES support layer preparation. Results showed that these two conditions could greatly affect the membrane water permeance, MWCO and surface charge. One LNF membrane, with a water permeance as high as 23.0 ± 1.8 L/m2/h/bar, when used for the filtration of conventional process-treated natural water, demonstrated a rejection of NOM higher than 70% and a low rejection of mineral salts at about 20%. Both the mineral salts/NOM selectivity and permselectivity were superior to the currently available LNF membranes as far as the authors know. This study demonstrated the great advantage of the NIPS–IP method for the fabrication of LNF membranes, particularly for the advanced treatment of drinking water.
doi_str_mv 10.3390/membranes12090887
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subjects Charge density
Drinking water
Fabrication
Humic acid
interfacial polymerization (IP)
loose nanofiltration (LNF)
Membranes
Microscopy
Molecular weight
Nanofiltration
Nanotechnology
natural organic matter (NOM)
non-solvent induced phase separation (NIPS)
Organic matter
Phase separation
Piperazine
Polyethersulfones
Polyethylene glycol
Purification
Rejection
rejection selectivity
Reluctance
Salts
Selectivity
Surface charge
Water
Water purification
Water treatment
Water treatment plants
title Fabrication of Loose Nanofiltration Membranes with High Rejection Selectivity between Natural Organic Matter and Salts for Drinking Water Treatment
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