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A Self‐Healing Flexible Quasi‐Solid Zinc‐Ion Battery Using All‐In‐One Electrodes

Self‐healing and flexibility are significant for many emerging applications of secondary batteries, which have attracted broad attention. Herein, a self‐healing flexible quasi‐solid Zn‐ion battery composing of flexible all‐in‐one cathode (VS2 nanosheets growing on carbon cloth) and anode (electroche...

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Bibliographic Details
Published in:Advanced science 2021-04, Vol.8 (8), p.2004689-n/a
Main Authors: Liu, Jinyun, Long, Jiawei, Shen, Zihan, Jin, Xing, Han, Tianli, Si, Ting, Zhang, Huigang
Format: Article
Language:English
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Summary:Self‐healing and flexibility are significant for many emerging applications of secondary batteries, which have attracted broad attention. Herein, a self‐healing flexible quasi‐solid Zn‐ion battery composing of flexible all‐in‐one cathode (VS2 nanosheets growing on carbon cloth) and anode (electrochemically deposited Zn nanowires), and a self‐healing hydrogel electrolyte, is presented. The free‐standing all‐in‐one electrodes enable a high capacity and robust structure during flexible transformation of the battery, and the hydrogel electrolyte possesses a good self‐healing performance. The presented battery remains as a high retention potential even after healing from being cut into six pieces. When bending at 60°, 90°, and 180°, the battery capacities remain 124, 125, and 114 mAh g−1, respectively, cycling at a current density of 50 mA g−1. Moreover, after cutting and healing twice, the battery still delivers a stable capacity, indicating a potential use of self‐healing and wearable electronics. A self‐healing flexible quasi‐solid Zn‐ion battery composes of all‐in‐one cathode and anode, and a self‐healing hydrogel electrolyte. The free‐standing all‐in‐one electrodes enable a high capacity and flexible transformation of the battery, while the hydrogel electrolyte possesses a self‐healing performance. Under bending at different angles, and cutting/healing many times, the batteries remain very stable, indicating a promising potential for broad applications.
ISSN:2198-3844
2198-3844
DOI:10.1002/advs.202004689