Radiological hazards associated with natural radioactivity in topsoil and subsoil from Osogbo, Nigeria

• Published in: Physics and chemistry of the earth. Parts A/B/C 2025-02, Vol.137, Article 103821
• Main Authors: Khalaf, Hyam, Olaoye, M.A., Mostafa, Mostafa.Y.A., Adegbola, R.B., Muniru, E.D., Mansour, Howaida
• Format: Article
• Language: English
• Subjects: Natural radioactivity; Radiation exposure; Radiological hazards; Subsoil; Topsoil
• ISSN: 1474-7065
• DOI: 10.1016/j.pce.2024.103821

The present research used gamma-ray spectrometry to assess the amount of activity concentration for radionuclides (226Ra, 232Th and 40K). That naturally exist in samples of topsoil and subsoil in Osogbo, Osun State, Nigeria, using a sodium-iodide detector and associated radiological risk factors were estimated. The activity levels of 226Ra, 232Th and 40K are, respectively, ranges from 167.03 ± 4.37 to 1187.51 ± 178.68 Bqkg−1, 18.21 ± 23.97 to 134.79 ± 60.00 Bqkg−1 and 8.67 ± 4.80 to 188.65 ± 7.33 Bqkg−1 for subsoil, and ranges from 263.64 ± 5.39 to 3303.33 ± 14.47 Bqkg−1, 23.90 ± 32.28 to 191.05 ± 72.93 Bqkg−1 and 9.90 ± 5.90 to 129.17 ± 8.94 Bqkg−1for topsoil. According to the United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR), the global average activity levels for these radionuclides are 226Ra (35 Bq/kg), 232Th (30 Bq/kg), and 40K (400 Bq/kg). In the study area, the average activity levels of these radionuclides were found to be higher in subsoil compared to topsoil. The estimated average of radiological risk factors (radium activity, the absorbed dose rate, annual gonadal dose equivalent, excess lifetime cancer risk, and representative level index) are recorded, 166.52 Bq/kg, 78.62 nGy/h, 545.23 μSv/y, 0.38 and 1.21 For subsoil respectively, but for topsoil are recorded 184.39 Bq/kg, 90.39 nGy/h, 637.92 μSv/y, 0.44 and 1.40 respectively. All radiological risk factors are much greater than those reported by UNSCEAR (2000) magnitudes of 370 Bq/kg, 59 nGy/h, 300 μSv/y, 2.9 × 10-4, and 1, respectively. The results obtained reveal a high radioactivity level in the investigated area. Therefore, it is advised that the study region have regular radiation monitoring and ecological evaluations. •Using gamma spectrometry, naturally occurring radionuclides in topsoil and subsoil were measured.•The average activity of naturally occurring radionuclides is observed to be higher in subsoil.•Radiological hazard indices were estimated with high radioactivity levels in the study area.•Regular radiation monitoring and environmental assessment are recommended in the study area.