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On the temperature dependence of the lifetime of thermally isolated metastable clusters
The temperature dependence of the lifetime of the thermally isolated metastable N 8 cubane up to its decay into N 2 molecules has been calculated by the molecular dynamics method. It has been demonstrated that this dependence significantly deviates from the Arrhenius law. The applicability of the fi...
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Published in: | Physics of the solid state 2010, Vol.52 (1), p.201-205 |
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container_issue | 1 |
container_start_page | 201 |
container_title | Physics of the solid state |
container_volume | 52 |
creator | Openov, L. A. Lobanov, D. A. Podlivaev, A. I. |
description | The temperature dependence of the lifetime of the thermally isolated metastable N
8
cubane up to its decay into N
2
molecules has been calculated by the molecular dynamics method. It has been demonstrated that this dependence significantly deviates from the Arrhenius law. The applicability of the finite heat bath theory to the description of thermally isolated atomic clusters has been proved using statistical analysis of the results obtained. |
doi_str_mv | 10.1134/S1063783410010348 |
format | article |
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8
cubane up to its decay into N
2
molecules has been calculated by the molecular dynamics method. It has been demonstrated that this dependence significantly deviates from the Arrhenius law. The applicability of the finite heat bath theory to the description of thermally isolated atomic clusters has been proved using statistical analysis of the results obtained.</description><identifier>ISSN: 1063-7834</identifier><identifier>EISSN: 1090-6460</identifier><identifier>DOI: 10.1134/S1063783410010348</identifier><language>eng</language><publisher>Dordrecht: SP MAIK Nauka/Interperiodica</publisher><subject>Fullerenes and Atomic Clusters ; Physics ; Physics and Astronomy ; Solid State Physics</subject><ispartof>Physics of the solid state, 2010, Vol.52 (1), p.201-205</ispartof><rights>Pleiades Publishing, Ltd. 2010</rights><rights>COPYRIGHT 2010 Springer</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c361t-abb39be389d08e4edf946a002f7d0e007a227b0bfbe4c54586b4293936f477323</citedby><cites>FETCH-LOGICAL-c361t-abb39be389d08e4edf946a002f7d0e007a227b0bfbe4c54586b4293936f477323</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27903,27904</link.rule.ids></links><search><creatorcontrib>Openov, L. A.</creatorcontrib><creatorcontrib>Lobanov, D. A.</creatorcontrib><creatorcontrib>Podlivaev, A. I.</creatorcontrib><title>On the temperature dependence of the lifetime of thermally isolated metastable clusters</title><title>Physics of the solid state</title><addtitle>Phys. Solid State</addtitle><description>The temperature dependence of the lifetime of the thermally isolated metastable N
8
cubane up to its decay into N
2
molecules has been calculated by the molecular dynamics method. It has been demonstrated that this dependence significantly deviates from the Arrhenius law. The applicability of the finite heat bath theory to the description of thermally isolated atomic clusters has been proved using statistical analysis of the results obtained.</description><subject>Fullerenes and Atomic Clusters</subject><subject>Physics</subject><subject>Physics and Astronomy</subject><subject>Solid State Physics</subject><issn>1063-7834</issn><issn>1090-6460</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2010</creationdate><recordtype>article</recordtype><recordid>eNp9kM9LwzAUx4MoOKd_gLdePXS-NGnaHsfwx2AwcIrHkrQvsyNtR5KC--9NnR6GIDm85L3P5wW-hNxSmFHK-P2GgmBZzjgFoMB4fkYmFAqIBRdwPt4Fi8f5JblybhcgStNiQt7XXeQ_MPLY7tFKP1iMatxjV2NXYdTr76lpNPqm_X3bVhpziBrXG-mxjlr00nmpDEaVGZxH667JhZbG4c1PnZK3x4fXxXO8Wj8tF_NVXDFBfSyVYoVClhc15Mix1gUXEiDRWQ0IkMkkyRQorZBXKU9zoXhSsIIJzbOMJWxKZse9W2mwbDrdeyurcGpsm6rvUDehPw-fJZxySINwdyIExuOn38rBuXK5eTll6ZGtbO-cRV3ubdNKeygplGPs5Z_Yg5McHRfYbou23PWD7UIG_0hfLhKDlg</recordid><startdate>2010</startdate><enddate>2010</enddate><creator>Openov, L. A.</creator><creator>Lobanov, D. A.</creator><creator>Podlivaev, A. I.</creator><general>SP MAIK Nauka/Interperiodica</general><general>Springer</general><scope>AAYXX</scope><scope>CITATION</scope><scope>ISR</scope></search><sort><creationdate>2010</creationdate><title>On the temperature dependence of the lifetime of thermally isolated metastable clusters</title><author>Openov, L. A. ; Lobanov, D. A. ; Podlivaev, A. I.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c361t-abb39be389d08e4edf946a002f7d0e007a227b0bfbe4c54586b4293936f477323</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2010</creationdate><topic>Fullerenes and Atomic Clusters</topic><topic>Physics</topic><topic>Physics and Astronomy</topic><topic>Solid State Physics</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Openov, L. A.</creatorcontrib><creatorcontrib>Lobanov, D. A.</creatorcontrib><creatorcontrib>Podlivaev, A. I.</creatorcontrib><collection>CrossRef</collection><collection>Gale In Context: Science</collection><jtitle>Physics of the solid state</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Openov, L. A.</au><au>Lobanov, D. A.</au><au>Podlivaev, A. I.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>On the temperature dependence of the lifetime of thermally isolated metastable clusters</atitle><jtitle>Physics of the solid state</jtitle><stitle>Phys. Solid State</stitle><date>2010</date><risdate>2010</risdate><volume>52</volume><issue>1</issue><spage>201</spage><epage>205</epage><pages>201-205</pages><issn>1063-7834</issn><eissn>1090-6460</eissn><abstract>The temperature dependence of the lifetime of the thermally isolated metastable N
8
cubane up to its decay into N
2
molecules has been calculated by the molecular dynamics method. It has been demonstrated that this dependence significantly deviates from the Arrhenius law. The applicability of the finite heat bath theory to the description of thermally isolated atomic clusters has been proved using statistical analysis of the results obtained.</abstract><cop>Dordrecht</cop><pub>SP MAIK Nauka/Interperiodica</pub><doi>10.1134/S1063783410010348</doi><tpages>5</tpages></addata></record> |
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ispartof | Physics of the solid state, 2010, Vol.52 (1), p.201-205 |
issn | 1063-7834 1090-6460 |
language | eng |
recordid | cdi_gale_infotracacademiconefile_A361241405 |
source | Springer Link |
subjects | Fullerenes and Atomic Clusters Physics Physics and Astronomy Solid State Physics |
title | On the temperature dependence of the lifetime of thermally isolated metastable clusters |
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