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Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry
A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution ef...
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Published in: | Journal of radioanalytical and nuclear chemistry 2015-02, Vol.303 (2), p.1317-1320 |
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creator | Ooe, K. Attallah, M. F. Asai, M. Goto, N. Gupta, N. S. Haba, H. Huang, M. Kanaya, J. Kaneya, Y. Kasamatsu, Y. Kitatsuji, Y. Kitayama, Y. Koga, K. Komori, Y. Koyama, T. Kratz, J. V. Lerum, H. V. Miyashita, S. Oshimi, Y. Pershina, V. Sato, D. Sato, T. K. Shigekawa, Y. Shinohara, A. Tanaka, A. Toyoshima, A. Tsukada, K. Tsuto, S. Yokokita, T. Yokoyama, A. Omtvedt, J. P. Nagame, Y. Schädel, M. |
description | A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution efficiencies of short-lived radionuclides of
91m,93m
Mo and
176
W were measured. Yields of more than 80 % were observed for short-lived radionuclides at aqueous-phase flow rates of 0.1–0.4 mL/s. The gas flow-rate had no influence on the dissolution efficiency within the studied flow range of 1.0–2.0 L/min. These results show that this technique is applicable for on-line chemical studies of SHEs in the liquid phase. |
doi_str_mv | 10.1007/s10967-014-3469-3 |
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91m,93m
Mo and
176
W were measured. Yields of more than 80 % were observed for short-lived radionuclides at aqueous-phase flow rates of 0.1–0.4 mL/s. The gas flow-rate had no influence on the dissolution efficiency within the studied flow range of 1.0–2.0 L/min. These results show that this technique is applicable for on-line chemical studies of SHEs in the liquid phase.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-014-3469-3</identifier><language>eng</language><publisher>Dordrecht: Springer Netherlands</publisher><subject>Chemistry ; Chemistry and Materials Science ; Diagnostic Radiology ; Hadrons ; Heavy Ions ; Inorganic Chemistry ; Nuclear Chemistry ; Nuclear Physics ; Physical Chemistry</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2015-02, Vol.303 (2), p.1317-1320</ispartof><rights>Akadémiai Kiadó, Budapest, Hungary 2014</rights><rights>COPYRIGHT 2015 Springer</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c467t-ee92db9b31ce79915be6373623b412eb070e48861dba052979cfcf79f14684f53</citedby><cites>FETCH-LOGICAL-c467t-ee92db9b31ce79915be6373623b412eb070e48861dba052979cfcf79f14684f53</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27898,27899</link.rule.ids></links><search><creatorcontrib>Ooe, K.</creatorcontrib><creatorcontrib>Attallah, M. F.</creatorcontrib><creatorcontrib>Asai, M.</creatorcontrib><creatorcontrib>Goto, N.</creatorcontrib><creatorcontrib>Gupta, N. S.</creatorcontrib><creatorcontrib>Haba, H.</creatorcontrib><creatorcontrib>Huang, M.</creatorcontrib><creatorcontrib>Kanaya, J.</creatorcontrib><creatorcontrib>Kaneya, Y.</creatorcontrib><creatorcontrib>Kasamatsu, Y.</creatorcontrib><creatorcontrib>Kitatsuji, Y.</creatorcontrib><creatorcontrib>Kitayama, Y.</creatorcontrib><creatorcontrib>Koga, K.</creatorcontrib><creatorcontrib>Komori, Y.</creatorcontrib><creatorcontrib>Koyama, T.</creatorcontrib><creatorcontrib>Kratz, J. V.</creatorcontrib><creatorcontrib>Lerum, H. V.</creatorcontrib><creatorcontrib>Miyashita, S.</creatorcontrib><creatorcontrib>Oshimi, Y.</creatorcontrib><creatorcontrib>Pershina, V.</creatorcontrib><creatorcontrib>Sato, D.</creatorcontrib><creatorcontrib>Sato, T. K.</creatorcontrib><creatorcontrib>Shigekawa, Y.</creatorcontrib><creatorcontrib>Shinohara, A.</creatorcontrib><creatorcontrib>Tanaka, A.</creatorcontrib><creatorcontrib>Toyoshima, A.</creatorcontrib><creatorcontrib>Tsukada, K.</creatorcontrib><creatorcontrib>Tsuto, S.</creatorcontrib><creatorcontrib>Yokokita, T.</creatorcontrib><creatorcontrib>Yokoyama, A.</creatorcontrib><creatorcontrib>Omtvedt, J. P.</creatorcontrib><creatorcontrib>Nagame, Y.</creatorcontrib><creatorcontrib>Schädel, M.</creatorcontrib><title>Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution efficiencies of short-lived radionuclides of
91m,93m
Mo and
176
W were measured. Yields of more than 80 % were observed for short-lived radionuclides at aqueous-phase flow rates of 0.1–0.4 mL/s. The gas flow-rate had no influence on the dissolution efficiency within the studied flow range of 1.0–2.0 L/min. These results show that this technique is applicable for on-line chemical studies of SHEs in the liquid phase.</description><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Diagnostic Radiology</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Inorganic Chemistry</subject><subject>Nuclear Chemistry</subject><subject>Nuclear Physics</subject><subject>Physical Chemistry</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNp9kM1uwyAQhFHVSk1_HqA3XsApGBvMsUp_pUi9tGeE8VJT2WCBnShvX9L0XO1hpdV8o51B6I6SNSVE3CdKJBcFoVXBKi4LdoZWtG6aohQNOUcrUjJe1ILRS3SV0jchRDYNW6H4CDsYwjSCn3GwWGMPe2yCn51fwpJw51IKwzK74LGeJh31nK97N_dZ2x-6GKY-tM7gEcY2ag_YhojTMkHsQe8OGAb4NTc9jC7N8XCDLqweEtz-7Wv0-fz0sXkttu8vb5uHbWEqLuYCQJZdK1tGDQgpad0CZ4LxkrUVLaElgkDVNJx2rSZ1KYU01lghLa14U9maXaP1yfdLD6Cct2GO2uTp8iM5IViX7w8VEZzLUhwBegJMDClFsGqKbtTxoChRx5bVqWWVW1bHlhXLTHliUtb6L4jqOyzR51z_QD80UIKC</recordid><startdate>20150201</startdate><enddate>20150201</enddate><creator>Ooe, K.</creator><creator>Attallah, M. F.</creator><creator>Asai, M.</creator><creator>Goto, N.</creator><creator>Gupta, N. S.</creator><creator>Haba, H.</creator><creator>Huang, M.</creator><creator>Kanaya, J.</creator><creator>Kaneya, Y.</creator><creator>Kasamatsu, Y.</creator><creator>Kitatsuji, Y.</creator><creator>Kitayama, Y.</creator><creator>Koga, K.</creator><creator>Komori, Y.</creator><creator>Koyama, T.</creator><creator>Kratz, J. V.</creator><creator>Lerum, H. V.</creator><creator>Miyashita, S.</creator><creator>Oshimi, Y.</creator><creator>Pershina, V.</creator><creator>Sato, D.</creator><creator>Sato, T. K.</creator><creator>Shigekawa, Y.</creator><creator>Shinohara, A.</creator><creator>Tanaka, A.</creator><creator>Toyoshima, A.</creator><creator>Tsukada, K.</creator><creator>Tsuto, S.</creator><creator>Yokokita, T.</creator><creator>Yokoyama, A.</creator><creator>Omtvedt, J. P.</creator><creator>Nagame, Y.</creator><creator>Schädel, M.</creator><general>Springer Netherlands</general><general>Springer</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20150201</creationdate><title>Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry</title><author>Ooe, K. ; Attallah, M. F. ; Asai, M. ; Goto, N. ; Gupta, N. S. ; Haba, H. ; Huang, M. ; Kanaya, J. ; Kaneya, Y. ; Kasamatsu, Y. ; Kitatsuji, Y. ; Kitayama, Y. ; Koga, K. ; Komori, Y. ; Koyama, T. ; Kratz, J. V. ; Lerum, H. V. ; Miyashita, S. ; Oshimi, Y. ; Pershina, V. ; Sato, D. ; Sato, T. K. ; Shigekawa, Y. ; Shinohara, A. ; Tanaka, A. ; Toyoshima, A. ; Tsukada, K. ; Tsuto, S. ; Yokokita, T. ; Yokoyama, A. ; Omtvedt, J. 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S.</au><au>Haba, H.</au><au>Huang, M.</au><au>Kanaya, J.</au><au>Kaneya, Y.</au><au>Kasamatsu, Y.</au><au>Kitatsuji, Y.</au><au>Kitayama, Y.</au><au>Koga, K.</au><au>Komori, Y.</au><au>Koyama, T.</au><au>Kratz, J. V.</au><au>Lerum, H. V.</au><au>Miyashita, S.</au><au>Oshimi, Y.</au><au>Pershina, V.</au><au>Sato, D.</au><au>Sato, T. K.</au><au>Shigekawa, Y.</au><au>Shinohara, A.</au><au>Tanaka, A.</au><au>Toyoshima, A.</au><au>Tsukada, K.</au><au>Tsuto, S.</au><au>Yokokita, T.</au><au>Yokoyama, A.</au><au>Omtvedt, J. P.</au><au>Nagame, Y.</au><au>Schädel, M.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry</atitle><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle><stitle>J Radioanal Nucl Chem</stitle><date>2015-02-01</date><risdate>2015</risdate><volume>303</volume><issue>2</issue><spage>1317</spage><epage>1320</epage><pages>1317-1320</pages><issn>0236-5731</issn><eissn>1588-2780</eissn><abstract>A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution efficiencies of short-lived radionuclides of
91m,93m
Mo and
176
W were measured. Yields of more than 80 % were observed for short-lived radionuclides at aqueous-phase flow rates of 0.1–0.4 mL/s. The gas flow-rate had no influence on the dissolution efficiency within the studied flow range of 1.0–2.0 L/min. These results show that this technique is applicable for on-line chemical studies of SHEs in the liquid phase.</abstract><cop>Dordrecht</cop><pub>Springer Netherlands</pub><doi>10.1007/s10967-014-3469-3</doi><tpages>4</tpages></addata></record> |
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subjects | Chemistry Chemistry and Materials Science Diagnostic Radiology Hadrons Heavy Ions Inorganic Chemistry Nuclear Chemistry Nuclear Physics Physical Chemistry |
title | Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry |
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