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Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry

A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution ef...

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Published in:Journal of radioanalytical and nuclear chemistry 2015-02, Vol.303 (2), p.1317-1320
Main Authors: Ooe, K., Attallah, M. F., Asai, M., Goto, N., Gupta, N. S., Haba, H., Huang, M., Kanaya, J., Kaneya, Y., Kasamatsu, Y., Kitatsuji, Y., Kitayama, Y., Koga, K., Komori, Y., Koyama, T., Kratz, J. V., Lerum, H. V., Miyashita, S., Oshimi, Y., Pershina, V., Sato, D., Sato, T. K., Shigekawa, Y., Shinohara, A., Tanaka, A., Toyoshima, A., Tsukada, K., Tsuto, S., Yokokita, T., Yokoyama, A., Omtvedt, J. P., Nagame, Y., Schädel, M.
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cited_by cdi_FETCH-LOGICAL-c467t-ee92db9b31ce79915be6373623b412eb070e48861dba052979cfcf79f14684f53
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creator Ooe, K.
Attallah, M. F.
Asai, M.
Goto, N.
Gupta, N. S.
Haba, H.
Huang, M.
Kanaya, J.
Kaneya, Y.
Kasamatsu, Y.
Kitatsuji, Y.
Kitayama, Y.
Koga, K.
Komori, Y.
Koyama, T.
Kratz, J. V.
Lerum, H. V.
Miyashita, S.
Oshimi, Y.
Pershina, V.
Sato, D.
Sato, T. K.
Shigekawa, Y.
Shinohara, A.
Tanaka, A.
Toyoshima, A.
Tsukada, K.
Tsuto, S.
Yokokita, T.
Yokoyama, A.
Omtvedt, J. P.
Nagame, Y.
Schädel, M.
description A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution efficiencies of short-lived radionuclides of 91m,93m Mo and 176 W were measured. Yields of more than 80 % were observed for short-lived radionuclides at aqueous-phase flow rates of 0.1–0.4 mL/s. The gas flow-rate had no influence on the dissolution efficiency within the studied flow range of 1.0–2.0 L/min. These results show that this technique is applicable for on-line chemical studies of SHEs in the liquid phase.
doi_str_mv 10.1007/s10967-014-3469-3
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subjects Chemistry
Chemistry and Materials Science
Diagnostic Radiology
Hadrons
Heavy Ions
Inorganic Chemistry
Nuclear Chemistry
Nuclear Physics
Physical Chemistry
title Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry
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