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On a singularity-free pair-polarizability anisotropy model for atomic gases
We present a collision-induced light scattering spectrum of Ne 2 and analyze it, together with an induced spectrum of Ar 2 , in terms of a model for the pair-polarizability anisotropy β of an atomic gas. This model, which is in essence a slight modification of one introduced by Ceccherini [ J. Chem....
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| Published in: | The Journal of chemical physics 2006-06, Vol.124 (23), p.234303-234303-4 |
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| Main Authors: | , , |
| Format: | Article |
| Language: | English |
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| cites | cdi_FETCH-LOGICAL-c372t-872b1349de2359eb6dab8dbfa33ea9eb0197653a2c7cb720d4aff94f81b7b4e33 |
| container_end_page | 234303-4 |
| container_issue | 23 |
| container_start_page | 234303 |
| container_title | The Journal of chemical physics |
| container_volume | 124 |
| creator | Chrysos, M. Dixneuf, S. Rachet, F. |
| description | We present a collision-induced light scattering spectrum of
Ne
2
and analyze it, together with an induced spectrum of
Ar
2
, in terms of a model for the pair-polarizability anisotropy
β
of an atomic gas. This model, which is in essence a slight modification of one introduced by
Ceccherini
[
J. Chem. Phys.
111
,
6316
(
1999
)
], is shown to describe the measured spectra much farther into the wings than does the original model. The agreement of our measurements with quantum-mechanical spectra from the most reliable, now available,
ab initio
computation methods for
β
produces evidence in support of the data and counters criticism of our experiment. |
| doi_str_mv | 10.1063/1.2210478 |
| format | article |
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Ne
2
and analyze it, together with an induced spectrum of
Ar
2
, in terms of a model for the pair-polarizability anisotropy
β
of an atomic gas. This model, which is in essence a slight modification of one introduced by
Ceccherini
[
J. Chem. Phys.
111
,
6316
(
1999
)
], is shown to describe the measured spectra much farther into the wings than does the original model. The agreement of our measurements with quantum-mechanical spectra from the most reliable, now available,
ab initio
computation methods for
β
produces evidence in support of the data and counters criticism of our experiment.</description><identifier>ISSN: 0021-9606</identifier><identifier>EISSN: 1089-7690</identifier><identifier>DOI: 10.1063/1.2210478</identifier><identifier>PMID: 16821914</identifier><identifier>CODEN: JCPSA6</identifier><language>eng</language><publisher>United States: American Institute of Physics</publisher><ispartof>The Journal of chemical physics, 2006-06, Vol.124 (23), p.234303-234303-4</ispartof><rights>2006 American Institute of Physics</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c372t-872b1349de2359eb6dab8dbfa33ea9eb0197653a2c7cb720d4aff94f81b7b4e33</citedby><cites>FETCH-LOGICAL-c372t-872b1349de2359eb6dab8dbfa33ea9eb0197653a2c7cb720d4aff94f81b7b4e33</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,782,784,795,885,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/16821914$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://hal.science/hal-00099486$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Chrysos, M.</creatorcontrib><creatorcontrib>Dixneuf, S.</creatorcontrib><creatorcontrib>Rachet, F.</creatorcontrib><title>On a singularity-free pair-polarizability anisotropy model for atomic gases</title><title>The Journal of chemical physics</title><addtitle>J Chem Phys</addtitle><description>We present a collision-induced light scattering spectrum of
Ne
2
and analyze it, together with an induced spectrum of
Ar
2
, in terms of a model for the pair-polarizability anisotropy
β
of an atomic gas. This model, which is in essence a slight modification of one introduced by
Ceccherini
[
J. Chem. Phys.
111
,
6316
(
1999
)
], is shown to describe the measured spectra much farther into the wings than does the original model. The agreement of our measurements with quantum-mechanical spectra from the most reliable, now available,
ab initio
computation methods for
β
produces evidence in support of the data and counters criticism of our experiment.</description><issn>0021-9606</issn><issn>1089-7690</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2006</creationdate><recordtype>article</recordtype><recordid>eNp1kcFKAzEQhoMoWqsHX0D2JHjYmkm2yeYiSFErFnrRc5jsZmtkd7MmW6E-vVta1IunYWY-Pph_CLkAOgEq-A1MGAOayfyAjIDmKpVC0UMyopRBqgQVJ-Q0xndKKUiWHZMTEDkDBdmIPC_bBJPo2tW6xuD6TVoFa5MOXUg7vx19oXH1sEiwddH3wXebpPGlrZPKhwR737giWWG08YwcVVhHe76vY_L6cP8ym6eL5ePT7G6RFlyyPs0lM8AzVVrGp8oaUaLJS1Mh5xaHnoKSYsqRFbIwktEyw6pSWZWDkSaznI_J9c77hrXugmswbLRHp-d3C72dDYcqleXiEwb2asd2wX-sbex142Jh6xpb69dRi1wA43T6Ky2CjzHY6scMVG9T1qD3KQ_s5V66No0tf8l9rANwuwNi4XrsnW__ty1bjfrPA_TwAP4N_teMeA</recordid><startdate>20060621</startdate><enddate>20060621</enddate><creator>Chrysos, M.</creator><creator>Dixneuf, S.</creator><creator>Rachet, F.</creator><general>American Institute of Physics</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>1XC</scope></search><sort><creationdate>20060621</creationdate><title>On a singularity-free pair-polarizability anisotropy model for atomic gases</title><author>Chrysos, M. ; Dixneuf, S. ; Rachet, F.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c372t-872b1349de2359eb6dab8dbfa33ea9eb0197653a2c7cb720d4aff94f81b7b4e33</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2006</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chrysos, M.</creatorcontrib><creatorcontrib>Dixneuf, S.</creatorcontrib><creatorcontrib>Rachet, F.</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>The Journal of chemical physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chrysos, M.</au><au>Dixneuf, S.</au><au>Rachet, F.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>On a singularity-free pair-polarizability anisotropy model for atomic gases</atitle><jtitle>The Journal of chemical physics</jtitle><addtitle>J Chem Phys</addtitle><date>2006-06-21</date><risdate>2006</risdate><volume>124</volume><issue>23</issue><spage>234303</spage><epage>234303-4</epage><pages>234303-234303-4</pages><issn>0021-9606</issn><eissn>1089-7690</eissn><coden>JCPSA6</coden><abstract>We present a collision-induced light scattering spectrum of
Ne
2
and analyze it, together with an induced spectrum of
Ar
2
, in terms of a model for the pair-polarizability anisotropy
β
of an atomic gas. This model, which is in essence a slight modification of one introduced by
Ceccherini
[
J. Chem. Phys.
111
,
6316
(
1999
)
], is shown to describe the measured spectra much farther into the wings than does the original model. The agreement of our measurements with quantum-mechanical spectra from the most reliable, now available,
ab initio
computation methods for
β
produces evidence in support of the data and counters criticism of our experiment.</abstract><cop>United States</cop><pub>American Institute of Physics</pub><pmid>16821914</pmid><doi>10.1063/1.2210478</doi><tpages>1</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0021-9606 |
| ispartof | The Journal of chemical physics, 2006-06, Vol.124 (23), p.234303-234303-4 |
| issn | 0021-9606 1089-7690 |
| language | eng |
| recordid | cdi_hal_primary_oai_HAL_hal_00099486v1 |
| source | American Institute of Physics (AIP) Publications; American Institute of Physics:Jisc Collections:Transitional Journals Agreement 2021-23 (Reading list) |
| title | On a singularity-free pair-polarizability anisotropy model for atomic gases |
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