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Effect of end-substitutions of distyryl-oligothiophenes by hexyl chains on environmental stability in organic thin film transistors
In this study, solution and solid-state properties as well as the organic thin film transistor (OTFT) behaviour of two α,ω-hexyl-distyryl-oligothiophenes ( DH-DS nT , n = 2, 4) are presented. The optical and electrochemical properties of the oligomers in solution were investigated by UV–vis absorpti...
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Published in: | Organic electronics 2008-10, Vol.9 (5), p.591-601 |
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container_start_page | 591 |
container_title | Organic electronics |
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creator | Videlot-Ackermann, C. Brisset, H. Ackermann, J. Zhang, J. Raynal, P. Fages, F. Mehl, G.H. Tnanisawa, T. Yoshimoto, N. |
description | In this study, solution and solid-state properties as well as the organic thin film transistor (OTFT) behaviour of two α,ω-hexyl-distyryl-oligothiophenes (
DH-DS
nT
,
n
=
2, 4) are presented. The optical and electrochemical properties of the oligomers in solution were investigated by UV–vis absorption and photoluminescence spectroscopies, and cyclic voltammetry. Liquid crystal properties were studied by differential scanning calorimetry (DSC) and optical polarising microscopy (OPM). High-vacuum evaporated thin films were studied by optical absorption, X-ray diffraction and atomic force microscopy (AFM), and implemented as p-type semiconducting layers into organic thin film transistors (OTFTs). The results are investigated to study the influence of alkyl chains on the α,ω-end positions of the distyryl-oligothiophene skeleton (
DS
nT
). Furthermore, detailed shelf-live tests of hole mobility (
μ), threshold voltage (
V
t), on current (
I
ON) and off current (
I
OFF) under atmospheric conditions (air, temperature) of OTFTs based on
DS4T and
DH-DS4T show that the presence of alkyl chains in α,ω-end positions of distyryl-oligothiophenes is detrimental to the environmental stability of OTFTs over time. |
doi_str_mv | 10.1016/j.orgel.2008.03.007 |
format | article |
fullrecord | <record><control><sourceid>elsevier_hal_p</sourceid><recordid>TN_cdi_hal_primary_oai_HAL_hal_00386843v1</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><els_id>S1566119908000475</els_id><sourcerecordid>S1566119908000475</sourcerecordid><originalsourceid>FETCH-LOGICAL-c433t-115e50e90e4e78c8c69ec3f757eabef06b0368eff567173621499d21f745466b3</originalsourceid><addsrcrecordid>eNp9kUFv3CAQha2qlZKm_QW5cOmhBztgbIwPPURRmlRaKZf2jDAe4lmxsAKyqs_948XdKMeeBo3e92bmUVXXjDaMMnGzb0J8Bte0lMqG8obS4V11yeQg677n9H1590LUjI3jRfUxpT0tVMfay-rPvbVgMgmWgJ_r9DKljPklY_Bpa86Y8hpXVweHzyEvGI4LeEhkWskCv1dHzKJx0_picMIY_AF81o6krCd0mFeCnpT1tEdDioEnFt2B5Kh9KuYhpk_VB6tdgs-v9ar69f3-591jvXt6-HF3u6tNx3ku2_fQUxgpdDBII40YwXA79APoCSwVE-VCgrW9GNjARcu6cZxbZoeu74SY-FX19ey7aKeOEQ86ripoVI-3O7X1KOVSyI6fWNHys9bEkFIE-wYwqrbM1V79y1xtmSvKCzwU6suZOupktLPlRoPpDW2paKVgXdF9O-ugnHtCiCoZBG9gxlh-Q80B_zvnL9Inm1g</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Effect of end-substitutions of distyryl-oligothiophenes by hexyl chains on environmental stability in organic thin film transistors</title><source>ScienceDirect Freedom Collection 2022-2024</source><creator>Videlot-Ackermann, C. ; Brisset, H. ; Ackermann, J. ; Zhang, J. ; Raynal, P. ; Fages, F. ; Mehl, G.H. ; Tnanisawa, T. ; Yoshimoto, N.</creator><creatorcontrib>Videlot-Ackermann, C. ; Brisset, H. ; Ackermann, J. ; Zhang, J. ; Raynal, P. ; Fages, F. ; Mehl, G.H. ; Tnanisawa, T. ; Yoshimoto, N.</creatorcontrib><description>In this study, solution and solid-state properties as well as the organic thin film transistor (OTFT) behaviour of two α,ω-hexyl-distyryl-oligothiophenes (
DH-DS
nT
,
n
=
2, 4) are presented. The optical and electrochemical properties of the oligomers in solution were investigated by UV–vis absorption and photoluminescence spectroscopies, and cyclic voltammetry. Liquid crystal properties were studied by differential scanning calorimetry (DSC) and optical polarising microscopy (OPM). High-vacuum evaporated thin films were studied by optical absorption, X-ray diffraction and atomic force microscopy (AFM), and implemented as p-type semiconducting layers into organic thin film transistors (OTFTs). The results are investigated to study the influence of alkyl chains on the α,ω-end positions of the distyryl-oligothiophene skeleton (
DS
nT
). Furthermore, detailed shelf-live tests of hole mobility (
μ), threshold voltage (
V
t), on current (
I
ON) and off current (
I
OFF) under atmospheric conditions (air, temperature) of OTFTs based on
DS4T and
DH-DS4T show that the presence of alkyl chains in α,ω-end positions of distyryl-oligothiophenes is detrimental to the environmental stability of OTFTs over time.</description><identifier>ISSN: 1566-1199</identifier><identifier>EISSN: 1878-5530</identifier><identifier>DOI: 10.1016/j.orgel.2008.03.007</identifier><language>eng</language><publisher>Amsterdam: Elsevier B.V</publisher><subject>Analytical chemistry ; Applied sciences ; Chemistry ; Condensed matter: electronic structure, electrical, magnetic, and optical properties ; Electrochemical methods ; Electronics ; Exact sciences and technology ; Oligothiophene derivative ; Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation ; Organic semiconductor ; Organic thin film transistor ; Photoluminescence ; Physics ; Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices ; Stability ; Transistors</subject><ispartof>Organic electronics, 2008-10, Vol.9 (5), p.591-601</ispartof><rights>2008 Elsevier B.V.</rights><rights>2008 INIST-CNRS</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c433t-115e50e90e4e78c8c69ec3f757eabef06b0368eff567173621499d21f745466b3</citedby><cites>FETCH-LOGICAL-c433t-115e50e90e4e78c8c69ec3f757eabef06b0368eff567173621499d21f745466b3</cites><orcidid>0000-0003-2013-0710 ; 0000-0001-8240-6474 ; 0000-0003-2586-3788 ; 0000-0003-1944-8457</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,784,885,27924,27925</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=20628614$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://hal.science/hal-00386843$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Videlot-Ackermann, C.</creatorcontrib><creatorcontrib>Brisset, H.</creatorcontrib><creatorcontrib>Ackermann, J.</creatorcontrib><creatorcontrib>Zhang, J.</creatorcontrib><creatorcontrib>Raynal, P.</creatorcontrib><creatorcontrib>Fages, F.</creatorcontrib><creatorcontrib>Mehl, G.H.</creatorcontrib><creatorcontrib>Tnanisawa, T.</creatorcontrib><creatorcontrib>Yoshimoto, N.</creatorcontrib><title>Effect of end-substitutions of distyryl-oligothiophenes by hexyl chains on environmental stability in organic thin film transistors</title><title>Organic electronics</title><description>In this study, solution and solid-state properties as well as the organic thin film transistor (OTFT) behaviour of two α,ω-hexyl-distyryl-oligothiophenes (
DH-DS
nT
,
n
=
2, 4) are presented. The optical and electrochemical properties of the oligomers in solution were investigated by UV–vis absorption and photoluminescence spectroscopies, and cyclic voltammetry. Liquid crystal properties were studied by differential scanning calorimetry (DSC) and optical polarising microscopy (OPM). High-vacuum evaporated thin films were studied by optical absorption, X-ray diffraction and atomic force microscopy (AFM), and implemented as p-type semiconducting layers into organic thin film transistors (OTFTs). The results are investigated to study the influence of alkyl chains on the α,ω-end positions of the distyryl-oligothiophene skeleton (
DS
nT
). Furthermore, detailed shelf-live tests of hole mobility (
μ), threshold voltage (
V
t), on current (
I
ON) and off current (
I
OFF) under atmospheric conditions (air, temperature) of OTFTs based on
DS4T and
DH-DS4T show that the presence of alkyl chains in α,ω-end positions of distyryl-oligothiophenes is detrimental to the environmental stability of OTFTs over time.</description><subject>Analytical chemistry</subject><subject>Applied sciences</subject><subject>Chemistry</subject><subject>Condensed matter: electronic structure, electrical, magnetic, and optical properties</subject><subject>Electrochemical methods</subject><subject>Electronics</subject><subject>Exact sciences and technology</subject><subject>Oligothiophene derivative</subject><subject>Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation</subject><subject>Organic semiconductor</subject><subject>Organic thin film transistor</subject><subject>Photoluminescence</subject><subject>Physics</subject><subject>Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices</subject><subject>Stability</subject><subject>Transistors</subject><issn>1566-1199</issn><issn>1878-5530</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2008</creationdate><recordtype>article</recordtype><recordid>eNp9kUFv3CAQha2qlZKm_QW5cOmhBztgbIwPPURRmlRaKZf2jDAe4lmxsAKyqs_948XdKMeeBo3e92bmUVXXjDaMMnGzb0J8Bte0lMqG8obS4V11yeQg677n9H1590LUjI3jRfUxpT0tVMfay-rPvbVgMgmWgJ_r9DKljPklY_Bpa86Y8hpXVweHzyEvGI4LeEhkWskCv1dHzKJx0_picMIY_AF81o6krCd0mFeCnpT1tEdDioEnFt2B5Kh9KuYhpk_VB6tdgs-v9ar69f3-591jvXt6-HF3u6tNx3ku2_fQUxgpdDBII40YwXA79APoCSwVE-VCgrW9GNjARcu6cZxbZoeu74SY-FX19ey7aKeOEQ86ripoVI-3O7X1KOVSyI6fWNHys9bEkFIE-wYwqrbM1V79y1xtmSvKCzwU6suZOupktLPlRoPpDW2paKVgXdF9O-ugnHtCiCoZBG9gxlh-Q80B_zvnL9Inm1g</recordid><startdate>20081001</startdate><enddate>20081001</enddate><creator>Videlot-Ackermann, C.</creator><creator>Brisset, H.</creator><creator>Ackermann, J.</creator><creator>Zhang, J.</creator><creator>Raynal, P.</creator><creator>Fages, F.</creator><creator>Mehl, G.H.</creator><creator>Tnanisawa, T.</creator><creator>Yoshimoto, N.</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0003-2013-0710</orcidid><orcidid>https://orcid.org/0000-0001-8240-6474</orcidid><orcidid>https://orcid.org/0000-0003-2586-3788</orcidid><orcidid>https://orcid.org/0000-0003-1944-8457</orcidid></search><sort><creationdate>20081001</creationdate><title>Effect of end-substitutions of distyryl-oligothiophenes by hexyl chains on environmental stability in organic thin film transistors</title><author>Videlot-Ackermann, C. ; Brisset, H. ; Ackermann, J. ; Zhang, J. ; Raynal, P. ; Fages, F. ; Mehl, G.H. ; Tnanisawa, T. ; Yoshimoto, N.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c433t-115e50e90e4e78c8c69ec3f757eabef06b0368eff567173621499d21f745466b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2008</creationdate><topic>Analytical chemistry</topic><topic>Applied sciences</topic><topic>Chemistry</topic><topic>Condensed matter: electronic structure, electrical, magnetic, and optical properties</topic><topic>Electrochemical methods</topic><topic>Electronics</topic><topic>Exact sciences and technology</topic><topic>Oligothiophene derivative</topic><topic>Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation</topic><topic>Organic semiconductor</topic><topic>Organic thin film transistor</topic><topic>Photoluminescence</topic><topic>Physics</topic><topic>Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices</topic><topic>Stability</topic><topic>Transistors</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Videlot-Ackermann, C.</creatorcontrib><creatorcontrib>Brisset, H.</creatorcontrib><creatorcontrib>Ackermann, J.</creatorcontrib><creatorcontrib>Zhang, J.</creatorcontrib><creatorcontrib>Raynal, P.</creatorcontrib><creatorcontrib>Fages, F.</creatorcontrib><creatorcontrib>Mehl, G.H.</creatorcontrib><creatorcontrib>Tnanisawa, T.</creatorcontrib><creatorcontrib>Yoshimoto, N.</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Hyper Article en Ligne (HAL)</collection><jtitle>Organic electronics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Videlot-Ackermann, C.</au><au>Brisset, H.</au><au>Ackermann, J.</au><au>Zhang, J.</au><au>Raynal, P.</au><au>Fages, F.</au><au>Mehl, G.H.</au><au>Tnanisawa, T.</au><au>Yoshimoto, N.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effect of end-substitutions of distyryl-oligothiophenes by hexyl chains on environmental stability in organic thin film transistors</atitle><jtitle>Organic electronics</jtitle><date>2008-10-01</date><risdate>2008</risdate><volume>9</volume><issue>5</issue><spage>591</spage><epage>601</epage><pages>591-601</pages><issn>1566-1199</issn><eissn>1878-5530</eissn><abstract>In this study, solution and solid-state properties as well as the organic thin film transistor (OTFT) behaviour of two α,ω-hexyl-distyryl-oligothiophenes (
DH-DS
nT
,
n
=
2, 4) are presented. The optical and electrochemical properties of the oligomers in solution were investigated by UV–vis absorption and photoluminescence spectroscopies, and cyclic voltammetry. Liquid crystal properties were studied by differential scanning calorimetry (DSC) and optical polarising microscopy (OPM). High-vacuum evaporated thin films were studied by optical absorption, X-ray diffraction and atomic force microscopy (AFM), and implemented as p-type semiconducting layers into organic thin film transistors (OTFTs). The results are investigated to study the influence of alkyl chains on the α,ω-end positions of the distyryl-oligothiophene skeleton (
DS
nT
). Furthermore, detailed shelf-live tests of hole mobility (
μ), threshold voltage (
V
t), on current (
I
ON) and off current (
I
OFF) under atmospheric conditions (air, temperature) of OTFTs based on
DS4T and
DH-DS4T show that the presence of alkyl chains in α,ω-end positions of distyryl-oligothiophenes is detrimental to the environmental stability of OTFTs over time.</abstract><cop>Amsterdam</cop><pub>Elsevier B.V</pub><doi>10.1016/j.orgel.2008.03.007</doi><tpages>11</tpages><orcidid>https://orcid.org/0000-0003-2013-0710</orcidid><orcidid>https://orcid.org/0000-0001-8240-6474</orcidid><orcidid>https://orcid.org/0000-0003-2586-3788</orcidid><orcidid>https://orcid.org/0000-0003-1944-8457</orcidid></addata></record> |
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language | eng |
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source | ScienceDirect Freedom Collection 2022-2024 |
subjects | Analytical chemistry Applied sciences Chemistry Condensed matter: electronic structure, electrical, magnetic, and optical properties Electrochemical methods Electronics Exact sciences and technology Oligothiophene derivative Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation Organic semiconductor Organic thin film transistor Photoluminescence Physics Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices Stability Transistors |
title | Effect of end-substitutions of distyryl-oligothiophenes by hexyl chains on environmental stability in organic thin film transistors |
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