Optimized Synthesis of Fe/N/C Cathode Catalysts for PEM Fuel Cells: A Matter of Iron-Ligand Coordination Strength

It's all in the detail: Highly active Fe/N/C catalysts for the oxygen‐reduction reaction in polymer‐electrolyte‐membrane (PEM) fuel cells can be obtained from a precursor constructed from the zeolitic imidazolate framework ZIF‐8 and an iron–ligand complex if, and only if, the displacement of Zn...

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Published in:Angewandte Chemie International Edition 2013-07, Vol.52 (27), p.6867-6870
Main Authors: Tian, Juan, Morozan, Adina, Sougrati, Moulay Tahar, Lefèvre, Michel, Chenitz, Régis, Dodelet, Jean-Pol, Jones, Deborah, Jaouen, Frédéric
Format: Article
Language:English
Subjects:
Catalysis
Catalysts
chelates
Chemical Sciences
Construction
Displacement
Fuel cells
Iron
Precursors
Synthesis
UV/Vis spectroscopy
zeolites
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cited_by cdi_FETCH-LOGICAL-c5815-3bb0af4bdcd97ecef52e9c6c8a8a58ada2cb6713ca85498acdc2c571a36e89283
cites cdi_FETCH-LOGICAL-c5815-3bb0af4bdcd97ecef52e9c6c8a8a58ada2cb6713ca85498acdc2c571a36e89283
container_end_page 6870
container_issue 27
container_start_page 6867
container_title Angewandte Chemie International Edition
container_volume 52
creator Tian, Juan
Morozan, Adina
Sougrati, Moulay Tahar
Lefèvre, Michel
Chenitz, Régis
Dodelet, Jean-Pol
Jones, Deborah
Jaouen, Frédéric
description It's all in the detail: Highly active Fe/N/C catalysts for the oxygen‐reduction reaction in polymer‐electrolyte‐membrane (PEM) fuel cells can be obtained from a precursor constructed from the zeolitic imidazolate framework ZIF‐8 and an iron–ligand complex if, and only if, the displacement of ZnII ions from ZIF‐8 by FeII ions is restricted (see picture; TPTZ=2,4,6‐tris(2‐pyridyl)‐s‐triazine).
doi_str_mv 10.1002/anie.201303025
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subjects Catalysis
Catalysts
chelates
Chemical Sciences
Construction
Displacement
Fuel cells
Iron
Precursors
Synthesis
UV/Vis spectroscopy
zeolites
title Optimized Synthesis of Fe/N/C Cathode Catalysts for PEM Fuel Cells: A Matter of Iron-Ligand Coordination Strength
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