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Catalytic gasification of biomass (Miscanthus) enhanced by CO2 sorption
The main objective of this work concerns the coupling of biomass gasification reaction and CO 2 sorption. The study shows the feasibility to promote biomass steam gasification in a dense fluidized bed reactor with CO 2 sorption to enhance tar removal and hydrogen production. It also proves the effic...
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Published in: | Environmental science and pollution research international 2016-11, Vol.23 (22), p.22253-22266 |
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creator | Zamboni, I. Debal, M. Matt, M. Girods, P. Kiennemann, A. Rogaume, Y. Courson, C. |
description | The main objective of this work concerns the coupling of biomass gasification reaction and CO
2
sorption. The study shows the feasibility to promote biomass steam gasification in a dense fluidized bed reactor with CO
2
sorption to enhance tar removal and hydrogen production. It also proves the efficiency of CaO-Ca
12
Al
14
O
33
/olivine bi-functional materials to reduce heavy tar production. Experiments have been carried out in a fluidized bed gasifier using steam as the fluidizing medium to improve hydrogen production. Bed materials consisting of CaO-based oxide for CO
2
sorption (CaO-Ca
12
Al
14
O
33
) deposited on olivine for tar reduction were synthesized, their structural and textural properties were characterized by Brunauer–Emmett–Teller (BET), X-ray diffraction (XRD), and temperature-programmed reduction (TPR) methods, and the determination of their sorption capacity and stability analyzed by thermogravimetric analysis (TGA). It appears that this CaO-Ca
12
Al
14
O
33
/olivine sorbent/catalyst presents a good CO
2
sorption stability (for seven cycles of carbonation/decarbonation). Compared to olivine and Fe/olivine in a fixed bed reactor for steam reforming of toluene chosen as tar model compound, it shows a better hydrogen production rate and a lower CO
2
selectivity due to its sorption on the CaO phase. In the biomass steam gasification, the use of CaO-Ca
12
Al
14
O
33
/olivine as bed material at 700 °C leads to a higher H
2
production than olivine at 800 °C thanks to CO
2
sorption. Similar tar concentration and lighter tar production (analyzed by HPLC/UV) are observed. At 700 °C, sorbent addition allows to halve tar content and to eliminate the heaviest tars. |
doi_str_mv | 10.1007/s11356-016-6444-4 |
format | article |
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2
sorption. The study shows the feasibility to promote biomass steam gasification in a dense fluidized bed reactor with CO
2
sorption to enhance tar removal and hydrogen production. It also proves the efficiency of CaO-Ca
12
Al
14
O
33
/olivine bi-functional materials to reduce heavy tar production. Experiments have been carried out in a fluidized bed gasifier using steam as the fluidizing medium to improve hydrogen production. Bed materials consisting of CaO-based oxide for CO
2
sorption (CaO-Ca
12
Al
14
O
33
) deposited on olivine for tar reduction were synthesized, their structural and textural properties were characterized by Brunauer–Emmett–Teller (BET), X-ray diffraction (XRD), and temperature-programmed reduction (TPR) methods, and the determination of their sorption capacity and stability analyzed by thermogravimetric analysis (TGA). It appears that this CaO-Ca
12
Al
14
O
33
/olivine sorbent/catalyst presents a good CO
2
sorption stability (for seven cycles of carbonation/decarbonation). Compared to olivine and Fe/olivine in a fixed bed reactor for steam reforming of toluene chosen as tar model compound, it shows a better hydrogen production rate and a lower CO
2
selectivity due to its sorption on the CaO phase. In the biomass steam gasification, the use of CaO-Ca
12
Al
14
O
33
/olivine as bed material at 700 °C leads to a higher H
2
production than olivine at 800 °C thanks to CO
2
sorption. Similar tar concentration and lighter tar production (analyzed by HPLC/UV) are observed. At 700 °C, sorbent addition allows to halve tar content and to eliminate the heaviest tars.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-016-6444-4</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Biomass ; Carbon dioxide ; Catalysis ; Condensed Matter ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Fixed bed reactors ; Fluidized bed reactors ; Fluidized beds ; Gases ; Gasification ; Hydrocarbons ; Hydrogen ; Hydrogen production ; Liquid chromatography ; Materials Science ; Physics ; Reactors ; Sorption ; Steam ; Studies ; Synthesis gas ; Tar ; Technoeconomic Perspectives on Sustainable CO2 Capture and Utilization ; Thermogravimetric analysis ; Toluene ; Waste Water Technology ; Water Management ; Water Pollution Control ; X-ray diffraction</subject><ispartof>Environmental science and pollution research international, 2016-11, Vol.23 (22), p.22253-22266</ispartof><rights>Springer-Verlag Berlin Heidelberg 2016</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, 2016.</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c420t-be56734f3d21585885ea5ae1834f336f4e9d72d06c530df0b27ef6148157e0de3</citedby><cites>FETCH-LOGICAL-c420t-be56734f3d21585885ea5ae1834f336f4e9d72d06c530df0b27ef6148157e0de3</cites><orcidid>0000-0002-6818-4155 ; 0000-0001-8229-2219</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/1860882697/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/1860882697?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>230,314,780,784,885,11688,27924,27925,36060,36061,44363,74895</link.rule.ids><backlink>$$Uhttps://hal.univ-lorraine.fr/hal-01518102$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Zamboni, I.</creatorcontrib><creatorcontrib>Debal, M.</creatorcontrib><creatorcontrib>Matt, M.</creatorcontrib><creatorcontrib>Girods, P.</creatorcontrib><creatorcontrib>Kiennemann, A.</creatorcontrib><creatorcontrib>Rogaume, Y.</creatorcontrib><creatorcontrib>Courson, C.</creatorcontrib><title>Catalytic gasification of biomass (Miscanthus) enhanced by CO2 sorption</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><description>The main objective of this work concerns the coupling of biomass gasification reaction and CO
2
sorption. The study shows the feasibility to promote biomass steam gasification in a dense fluidized bed reactor with CO
2
sorption to enhance tar removal and hydrogen production. It also proves the efficiency of CaO-Ca
12
Al
14
O
33
/olivine bi-functional materials to reduce heavy tar production. Experiments have been carried out in a fluidized bed gasifier using steam as the fluidizing medium to improve hydrogen production. Bed materials consisting of CaO-based oxide for CO
2
sorption (CaO-Ca
12
Al
14
O
33
) deposited on olivine for tar reduction were synthesized, their structural and textural properties were characterized by Brunauer–Emmett–Teller (BET), X-ray diffraction (XRD), and temperature-programmed reduction (TPR) methods, and the determination of their sorption capacity and stability analyzed by thermogravimetric analysis (TGA). It appears that this CaO-Ca
12
Al
14
O
33
/olivine sorbent/catalyst presents a good CO
2
sorption stability (for seven cycles of carbonation/decarbonation). Compared to olivine and Fe/olivine in a fixed bed reactor for steam reforming of toluene chosen as tar model compound, it shows a better hydrogen production rate and a lower CO
2
selectivity due to its sorption on the CaO phase. In the biomass steam gasification, the use of CaO-Ca
12
Al
14
O
33
/olivine as bed material at 700 °C leads to a higher H
2
production than olivine at 800 °C thanks to CO
2
sorption. Similar tar concentration and lighter tar production (analyzed by HPLC/UV) are observed. At 700 °C, sorbent addition allows to halve tar content and to eliminate the heaviest tars.</description><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Biomass</subject><subject>Carbon dioxide</subject><subject>Catalysis</subject><subject>Condensed Matter</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Fixed bed reactors</subject><subject>Fluidized bed reactors</subject><subject>Fluidized beds</subject><subject>Gases</subject><subject>Gasification</subject><subject>Hydrocarbons</subject><subject>Hydrogen</subject><subject>Hydrogen production</subject><subject>Liquid chromatography</subject><subject>Materials Science</subject><subject>Physics</subject><subject>Reactors</subject><subject>Sorption</subject><subject>Steam</subject><subject>Studies</subject><subject>Synthesis gas</subject><subject>Tar</subject><subject>Technoeconomic Perspectives on Sustainable CO2 Capture and Utilization</subject><subject>Thermogravimetric analysis</subject><subject>Toluene</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><subject>X-ray 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gasification of biomass (Miscanthus) enhanced by CO2 sorption</title><author>Zamboni, I. ; Debal, M. ; Matt, M. ; Girods, P. ; Kiennemann, A. ; Rogaume, Y. ; Courson, C.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c420t-be56734f3d21585885ea5ae1834f336f4e9d72d06c530df0b27ef6148157e0de3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Biomass</topic><topic>Carbon dioxide</topic><topic>Catalysis</topic><topic>Condensed Matter</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental science</topic><topic>Fixed bed reactors</topic><topic>Fluidized bed reactors</topic><topic>Fluidized 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Res</stitle><date>2016-11-01</date><risdate>2016</risdate><volume>23</volume><issue>22</issue><spage>22253</spage><epage>22266</epage><pages>22253-22266</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>The main objective of this work concerns the coupling of biomass gasification reaction and CO
2
sorption. The study shows the feasibility to promote biomass steam gasification in a dense fluidized bed reactor with CO
2
sorption to enhance tar removal and hydrogen production. It also proves the efficiency of CaO-Ca
12
Al
14
O
33
/olivine bi-functional materials to reduce heavy tar production. Experiments have been carried out in a fluidized bed gasifier using steam as the fluidizing medium to improve hydrogen production. Bed materials consisting of CaO-based oxide for CO
2
sorption (CaO-Ca
12
Al
14
O
33
) deposited on olivine for tar reduction were synthesized, their structural and textural properties were characterized by Brunauer–Emmett–Teller (BET), X-ray diffraction (XRD), and temperature-programmed reduction (TPR) methods, and the determination of their sorption capacity and stability analyzed by thermogravimetric analysis (TGA). It appears that this CaO-Ca
12
Al
14
O
33
/olivine sorbent/catalyst presents a good CO
2
sorption stability (for seven cycles of carbonation/decarbonation). Compared to olivine and Fe/olivine in a fixed bed reactor for steam reforming of toluene chosen as tar model compound, it shows a better hydrogen production rate and a lower CO
2
selectivity due to its sorption on the CaO phase. In the biomass steam gasification, the use of CaO-Ca
12
Al
14
O
33
/olivine as bed material at 700 °C leads to a higher H
2
production than olivine at 800 °C thanks to CO
2
sorption. Similar tar concentration and lighter tar production (analyzed by HPLC/UV) are observed. At 700 °C, sorbent addition allows to halve tar content and to eliminate the heaviest tars.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s11356-016-6444-4</doi><tpages>14</tpages><orcidid>https://orcid.org/0000-0002-6818-4155</orcidid><orcidid>https://orcid.org/0000-0001-8229-2219</orcidid></addata></record> |
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ispartof | Environmental science and pollution research international, 2016-11, Vol.23 (22), p.22253-22266 |
issn | 0944-1344 1614-7499 |
language | eng |
recordid | cdi_hal_primary_oai_HAL_hal_01518102v1 |
source | ABI/INFORM Global; Springer Link |
subjects | Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Biomass Carbon dioxide Catalysis Condensed Matter Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Fixed bed reactors Fluidized bed reactors Fluidized beds Gases Gasification Hydrocarbons Hydrogen Hydrogen production Liquid chromatography Materials Science Physics Reactors Sorption Steam Studies Synthesis gas Tar Technoeconomic Perspectives on Sustainable CO2 Capture and Utilization Thermogravimetric analysis Toluene Waste Water Technology Water Management Water Pollution Control X-ray diffraction |
title | Catalytic gasification of biomass (Miscanthus) enhanced by CO2 sorption |
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