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Real time chemical imaging of a working catalytic membrane reactor during oxidative coupling of methane

We report the results from an operando XRD-CT study of a working catalytic membrane reactor for the oxidative coupling of methane. These results reveal the importance of the evolving solid state chemistry during catalytic reaction, particularly the chemical interaction between the catalyst and the o...

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Bibliographic Details
Published in:Chemical communications (Cambridge, England) England), 2015-08, Vol.51 (64), p.12752-12755
Main Authors: Vamvakeros, A, Jacques, S D M, Middelkoop, V, Di Michiel, M, Egan, C K, Ismagilov, I Z, Vaughan, G B M, Gallucci, F, van Sint Annaland, M, Shearing, P R, Cernik, R J, Beale, A M
Format: Article
Language:English
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Summary:We report the results from an operando XRD-CT study of a working catalytic membrane reactor for the oxidative coupling of methane. These results reveal the importance of the evolving solid state chemistry during catalytic reaction, particularly the chemical interaction between the catalyst and the oxygen transport membrane.
ISSN:1359-7345
1364-548X
DOI:10.1039/c5cc03208c