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Onset of antiferromagnetism in heavy-fermion metals
There are two main theoretical descriptions of antiferromagnets. The first arises from atomic physics, which predicts that atoms with unpaired electrons develop magnetic moments. In a solid, the coupling between moments on nearby ions then yields antiferromagnetic order at low temperatures. The seco...
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| Published in: | Nature (London) 2000-09, Vol.407 (6802), p.351-355 |
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| container_title | Nature (London) |
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| creator | Coleman, P Coldea, R Adams, M Ramazashvili, R Löhneysen, H.v Aeppli, G Stockert, O Bucher, E Schröder, A |
| description | There are two main theoretical descriptions of antiferromagnets. The first
arises from atomic physics, which predicts that atoms with unpaired electrons
develop magnetic moments. In a solid, the coupling between moments on nearby
ions then yields antiferromagnetic order at low temperatures.
The second description, based on the physics of electron fluids or 'Fermi
liquids', states that Coulomb interactions can drive the fluid to adopt
a more stable configuration by developing a spin density wave.
It is at present unknown which view is appropriate at a 'quantum critical
point', where the antiferromagnetic transition temperature vanishes. Here we report neutron scattering and bulk magnetometry
measurements of the metal CeCu6-xAux,
which allow us to discriminate between the two models. We find evidence for
an atomically local contribution to the magnetic correlations which develops
at the critical gold concentration (xc = 0.1
), corresponding to a magnetic ordering temperature of zero. This contribution
implies that a Fermi-liquid-destroying spin-localizing transition, unanticipated
from the spin density wave description, coincides with the antiferromagnetic
quantum critical point. |
| doi_str_mv | 10.1038/35030039 |
| format | article |
| fullrecord | <record><control><sourceid>gale_hal_p</sourceid><recordid>TN_cdi_hal_primary_oai_HAL_hal_02156728v1</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><galeid>A188067786</galeid><sourcerecordid>A188067786</sourcerecordid><originalsourceid>FETCH-LOGICAL-c699t-101488d3ac7eb05dcd6119e9e2406f4eeb1c13c4a4d1c4ba76cf88daecf019713</originalsourceid><addsrcrecordid>eNp90vFr1DAUB_Agijun4F8ghwxxSGdek6bpj8ehbnA40Ik_hlz62mW06S1ph_vvzXH16skm_SHw8ukL-eYR8hroGVAmP7KMMkpZ8YTMgOci4ULmT8mM0lQmVDJxRF6EcEMpzSDnz8kRAAUOMpsRdukC9vOummvX2wq971pdO-xtaOfWza9R390nsd7azs1b7HUTXpJnVVzw1bgekx-fP10tz5PV5ZeL5WKVGFEUfbI9Q8qSaZPjmmalKQVAgQWmnIqKI67BADNc8xIMX-tcmCp6jaaiUOTAjsnpru-1btTG21b7e9Vpq84XK7Wt0RQykafybmvf7ezGd7cDhl61NhhsGu2wG4JKc8ElzdII3_8XxlQKxgGARfr2H3rTDd7FK6uUci75rl-yQ7VuUFlXdb3XpkaHXjedw8rG8gKkpCLPpZiaHnizsbfqb3T2AIpfia01D3Y9Pfghmh5_9bUeQlAX378d2g-P28XVz-XXQz3mZXwXgsdq_xJA1Xb41J_hi_TNmNewbrGc4DhtEZyMQAejm8prZ2yYXIxUCDZdJsQdV6Ofcn_8TKf7weO-1x78Bjot8FU</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>204484052</pqid></control><display><type>article</type><title>Onset of antiferromagnetism in heavy-fermion metals</title><source>Springer Nature - Connect here FIRST to enable access</source><creator>Coleman, P ; Coldea, R ; Adams, M ; Ramazashvili, R ; Löhneysen, H.v ; Aeppli, G ; Stockert, O ; Bucher, E ; Schröder, A</creator><creatorcontrib>Coleman, P ; Coldea, R ; Adams, M ; Ramazashvili, R ; Löhneysen, H.v ; Aeppli, G ; Stockert, O ; Bucher, E ; Schröder, A</creatorcontrib><description>There are two main theoretical descriptions of antiferromagnets. The first
arises from atomic physics, which predicts that atoms with unpaired electrons
develop magnetic moments. In a solid, the coupling between moments on nearby
ions then yields antiferromagnetic order at low temperatures.
The second description, based on the physics of electron fluids or 'Fermi
liquids', states that Coulomb interactions can drive the fluid to adopt
a more stable configuration by developing a spin density wave.
It is at present unknown which view is appropriate at a 'quantum critical
point', where the antiferromagnetic transition temperature vanishes. Here we report neutron scattering and bulk magnetometry
measurements of the metal CeCu6-xAux,
which allow us to discriminate between the two models. We find evidence for
an atomically local contribution to the magnetic correlations which develops
at the critical gold concentration (xc = 0.1
), corresponding to a magnetic ordering temperature of zero. This contribution
implies that a Fermi-liquid-destroying spin-localizing transition, unanticipated
from the spin density wave description, coincides with the antiferromagnetic
quantum critical point.</description><identifier>ISSN: 0028-0836</identifier><identifier>EISSN: 1476-4687</identifier><identifier>DOI: 10.1038/35030039</identifier><identifier>PMID: 11014185</identifier><identifier>CODEN: NATUAS</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>Applied sciences ; Condensed Matter ; Condensed matter: electronic structure, electrical, magnetic, and optical properties ; Exact sciences and technology ; Heavy metals ; Humanities and Social Sciences ; Iron ; letter ; Low temperature ; Magnetic properties and materials ; Magnetically ordered materials: other intrinsic properties ; Magnetism ; Metals ; Metals. Metallurgy ; multidisciplinary ; Physics ; Science ; Science (multidisciplinary) ; Strongly Correlated Electrons ; Transition temperatures ; Valence fluctuation, kondo lattice, and heavy-fermion phenomena</subject><ispartof>Nature (London), 2000-09, Vol.407 (6802), p.351-355</ispartof><rights>Macmillan Magazines Ltd. 2000</rights><rights>2000 INIST-CNRS</rights><rights>COPYRIGHT 2000 Nature Publishing Group</rights><rights>Copyright Macmillan Journals Ltd. Sep 21, 2000</rights><rights>Distributed under a Creative Commons Attribution 4.0 International License</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c699t-101488d3ac7eb05dcd6119e9e2406f4eeb1c13c4a4d1c4ba76cf88daecf019713</citedby><cites>FETCH-LOGICAL-c699t-101488d3ac7eb05dcd6119e9e2406f4eeb1c13c4a4d1c4ba76cf88daecf019713</cites><orcidid>0000-0001-5133-8253</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>230,314,780,784,885,2726,27923,27924</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=1484663$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/11014185$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink><backlink>$$Uhttps://hal.science/hal-02156728$$DView record in HAL$$Hfree_for_read</backlink></links><search><creatorcontrib>Coleman, P</creatorcontrib><creatorcontrib>Coldea, R</creatorcontrib><creatorcontrib>Adams, M</creatorcontrib><creatorcontrib>Ramazashvili, R</creatorcontrib><creatorcontrib>Löhneysen, H.v</creatorcontrib><creatorcontrib>Aeppli, G</creatorcontrib><creatorcontrib>Stockert, O</creatorcontrib><creatorcontrib>Bucher, E</creatorcontrib><creatorcontrib>Schröder, A</creatorcontrib><title>Onset of antiferromagnetism in heavy-fermion metals</title><title>Nature (London)</title><addtitle>Nature</addtitle><addtitle>Nature</addtitle><description>There are two main theoretical descriptions of antiferromagnets. The first
arises from atomic physics, which predicts that atoms with unpaired electrons
develop magnetic moments. In a solid, the coupling between moments on nearby
ions then yields antiferromagnetic order at low temperatures.
The second description, based on the physics of electron fluids or 'Fermi
liquids', states that Coulomb interactions can drive the fluid to adopt
a more stable configuration by developing a spin density wave.
It is at present unknown which view is appropriate at a 'quantum critical
point', where the antiferromagnetic transition temperature vanishes. Here we report neutron scattering and bulk magnetometry
measurements of the metal CeCu6-xAux,
which allow us to discriminate between the two models. We find evidence for
an atomically local contribution to the magnetic correlations which develops
at the critical gold concentration (xc = 0.1
), corresponding to a magnetic ordering temperature of zero. This contribution
implies that a Fermi-liquid-destroying spin-localizing transition, unanticipated
from the spin density wave description, coincides with the antiferromagnetic
quantum critical point.</description><subject>Applied sciences</subject><subject>Condensed Matter</subject><subject>Condensed matter: electronic structure, electrical, magnetic, and optical properties</subject><subject>Exact sciences and technology</subject><subject>Heavy metals</subject><subject>Humanities and Social Sciences</subject><subject>Iron</subject><subject>letter</subject><subject>Low temperature</subject><subject>Magnetic properties and materials</subject><subject>Magnetically ordered materials: other intrinsic properties</subject><subject>Magnetism</subject><subject>Metals</subject><subject>Metals. Metallurgy</subject><subject>multidisciplinary</subject><subject>Physics</subject><subject>Science</subject><subject>Science (multidisciplinary)</subject><subject>Strongly Correlated Electrons</subject><subject>Transition temperatures</subject><subject>Valence fluctuation, kondo lattice, and heavy-fermion phenomena</subject><issn>0028-0836</issn><issn>1476-4687</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2000</creationdate><recordtype>article</recordtype><recordid>eNp90vFr1DAUB_Agijun4F8ghwxxSGdek6bpj8ehbnA40Ik_hlz62mW06S1ph_vvzXH16skm_SHw8ukL-eYR8hroGVAmP7KMMkpZ8YTMgOci4ULmT8mM0lQmVDJxRF6EcEMpzSDnz8kRAAUOMpsRdukC9vOummvX2wq971pdO-xtaOfWza9R390nsd7azs1b7HUTXpJnVVzw1bgekx-fP10tz5PV5ZeL5WKVGFEUfbI9Q8qSaZPjmmalKQVAgQWmnIqKI67BADNc8xIMX-tcmCp6jaaiUOTAjsnpru-1btTG21b7e9Vpq84XK7Wt0RQykafybmvf7ezGd7cDhl61NhhsGu2wG4JKc8ElzdII3_8XxlQKxgGARfr2H3rTDd7FK6uUci75rl-yQ7VuUFlXdb3XpkaHXjedw8rG8gKkpCLPpZiaHnizsbfqb3T2AIpfia01D3Y9Pfghmh5_9bUeQlAX378d2g-P28XVz-XXQz3mZXwXgsdq_xJA1Xb41J_hi_TNmNewbrGc4DhtEZyMQAejm8prZ2yYXIxUCDZdJsQdV6Ofcn_8TKf7weO-1x78Bjot8FU</recordid><startdate>20000921</startdate><enddate>20000921</enddate><creator>Coleman, P</creator><creator>Coldea, R</creator><creator>Adams, M</creator><creator>Ramazashvili, R</creator><creator>Löhneysen, H.v</creator><creator>Aeppli, G</creator><creator>Stockert, O</creator><creator>Bucher, E</creator><creator>Schröder, A</creator><general>Nature Publishing Group UK</general><general>Nature Publishing</general><general>Nature Publishing Group</general><scope>IQODW</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>ATWCN</scope><scope>3V.</scope><scope>7QG</scope><scope>7QL</scope><scope>7QP</scope><scope>7QR</scope><scope>7RV</scope><scope>7SN</scope><scope>7SS</scope><scope>7ST</scope><scope>7T5</scope><scope>7TG</scope><scope>7TK</scope><scope>7TM</scope><scope>7TO</scope><scope>7U9</scope><scope>7X2</scope><scope>7X7</scope><scope>7XB</scope><scope>88A</scope><scope>88E</scope><scope>88G</scope><scope>88I</scope><scope>8AF</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>8FH</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8G5</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BBNVY</scope><scope>BEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>BHPHI</scope><scope>BKSAR</scope><scope>C1K</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FYUFA</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>GUQSH</scope><scope>H94</scope><scope>HCIFZ</scope><scope>K9.</scope><scope>KB.</scope><scope>KB0</scope><scope>KL.</scope><scope>L6V</scope><scope>LK8</scope><scope>M0K</scope><scope>M0S</scope><scope>M1P</scope><scope>M2M</scope><scope>M2O</scope><scope>M2P</scope><scope>M7N</scope><scope>M7P</scope><scope>M7S</scope><scope>MBDVC</scope><scope>NAPCQ</scope><scope>P5Z</scope><scope>P62</scope><scope>P64</scope><scope>PATMY</scope><scope>PCBAR</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PSYQQ</scope><scope>PTHSS</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>R05</scope><scope>RC3</scope><scope>S0X</scope><scope>SOI</scope><scope>7X8</scope><scope>H8D</scope><scope>L7M</scope><scope>1XC</scope><orcidid>https://orcid.org/0000-0001-5133-8253</orcidid></search><sort><creationdate>20000921</creationdate><title>Onset of antiferromagnetism in heavy-fermion metals</title><author>Coleman, P ; Coldea, R ; Adams, M ; Ramazashvili, R ; Löhneysen, H.v ; Aeppli, G ; Stockert, O ; Bucher, E ; Schröder, A</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c699t-101488d3ac7eb05dcd6119e9e2406f4eeb1c13c4a4d1c4ba76cf88daecf019713</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2000</creationdate><topic>Applied sciences</topic><topic>Condensed Matter</topic><topic>Condensed matter: electronic structure, electrical, magnetic, and optical properties</topic><topic>Exact sciences and technology</topic><topic>Heavy metals</topic><topic>Humanities and Social Sciences</topic><topic>Iron</topic><topic>letter</topic><topic>Low temperature</topic><topic>Magnetic properties and materials</topic><topic>Magnetically ordered materials: other intrinsic properties</topic><topic>Magnetism</topic><topic>Metals</topic><topic>Metals. 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The first
arises from atomic physics, which predicts that atoms with unpaired electrons
develop magnetic moments. In a solid, the coupling between moments on nearby
ions then yields antiferromagnetic order at low temperatures.
The second description, based on the physics of electron fluids or 'Fermi
liquids', states that Coulomb interactions can drive the fluid to adopt
a more stable configuration by developing a spin density wave.
It is at present unknown which view is appropriate at a 'quantum critical
point', where the antiferromagnetic transition temperature vanishes. Here we report neutron scattering and bulk magnetometry
measurements of the metal CeCu6-xAux,
which allow us to discriminate between the two models. We find evidence for
an atomically local contribution to the magnetic correlations which develops
at the critical gold concentration (xc = 0.1
), corresponding to a magnetic ordering temperature of zero. This contribution
implies that a Fermi-liquid-destroying spin-localizing transition, unanticipated
from the spin density wave description, coincides with the antiferromagnetic
quantum critical point.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>11014185</pmid><doi>10.1038/35030039</doi><tpages>5</tpages><orcidid>https://orcid.org/0000-0001-5133-8253</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0028-0836 |
| ispartof | Nature (London), 2000-09, Vol.407 (6802), p.351-355 |
| issn | 0028-0836 1476-4687 |
| language | eng |
| recordid | cdi_hal_primary_oai_HAL_hal_02156728v1 |
| source | Springer Nature - Connect here FIRST to enable access |
| subjects | Applied sciences Condensed Matter Condensed matter: electronic structure, electrical, magnetic, and optical properties Exact sciences and technology Heavy metals Humanities and Social Sciences Iron letter Low temperature Magnetic properties and materials Magnetically ordered materials: other intrinsic properties Magnetism Metals Metals. Metallurgy multidisciplinary Physics Science Science (multidisciplinary) Strongly Correlated Electrons Transition temperatures Valence fluctuation, kondo lattice, and heavy-fermion phenomena |
| title | Onset of antiferromagnetism in heavy-fermion metals |
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