Debonding of a soft adhesive fibril in contact with an elastomeric pillar

• Published in: Soft matter 2022-08, Vol.18 (31), p.5857-5866
• Main Authors: Duigou-Majumdar, Aymeric, Cortet, Pierre-Philippe, Poulard, Christophe
• Format: Article
• Language: English
• Subjects: Adhesives; Condensed Matter; Criteria; Debonding; Elastomers; Elongation; Fibrils; Mechanical analysis; Physics; Pressure sensitive adhesives; Scaling laws; Soft Condensed Matter; Viscoelasticity
• ISSN: 1744-683X; 1744-6848
• DOI: 10.1039/d2sm00532h

The debonding criterion of fibrils of soft adhesive materials is a key element regarding the quantitative modelisation of pressure sensitive adhesive tapes' peeling energy. We present in this article an experimental study of the detachment of a commercial acrylic adhesive tape from the top surface of a single micrometric pillar of PDMS elastomer. During an experiment, the pillar and the adhesive, after being put in contact, are separated at a constant displacement rate, resulting in the formation, the elongation and the final detachment of a fibril of adhesive material. A systematic study allows us to uncover power laws for the maximum force and the critical elongation of the fibril at debonding as a function of the diameter of the cylindrical pillar which controls the diameter of the fibril. The scaling law evidenced for the critical elongation appears as a first step toward the understanding of the debonding criterion of fibrils of soft adhesive materials. In addition, viscoelastic digitation at the triple debonding line is observed during detachment for large pillar diameters. The wavelength and penetration length of the fingers that we report appear to be consistent with existing models based on pure elastic mechanical response. We study the debonding of a soft adhesive layer from a micrometric pillar. We uncover power laws as a function of the pillar diameter for the maximum force and the critical elongation of the fibril of adhesive material formed during debonding.