Air pollution characteristics in China during 2015–2016: Spatiotemporal variations and key meteorological factors

• Published in: The Science of the total environment 2019-01, Vol.648, p.902-915
• Main Authors: Li, Rui, Wang, Zhenzhen, Cui, Lulu, Fu, Hongbo, Zhang, Liwu, Kong, Lingdong, Chen, Weidong, Chen, Jianmin
• Format: Article
• Language: English
• Subjects: Air pollution; China; Meteorological factors; Physics; Spatial econometric model
• ISSN: 0048-9697; 1879-1026
• DOI: 10.1016/j.scitotenv.2018.08.181

With rapid economic development and urbanization, China has suffered from severe and persistent air pollution during the past years. In the work, the hourly data of PM2.5, PM10, SO2, NO2, CO, and O3 in all of the prefecture-level cities (336 cities) during 2015–2016 were collected to uncover the spatiotemporal variations and influential factors of these pollutants in China. The average concentrations of PM2.5, PM10, SO2, NO2, and CO decreased by 19.32%, 15.34%, 29.30%, 9.39%, and 8.00% from 2015 to 2016, suggesting the effects of efficient control measurements during this period. On the contrary, the O3 concentration increased by 4.20% during the same period, which mainly owed to high volatile organic compounds (VOCs) loading. The concentrations of PM2.5, PM10, SO2, CO and NO2 showed the highest and the lowest ones in winter and summer, respectively. However, the O3 concentration peaked in summer, followed by ones in spring and autumn, and presented the lowest one in winter. All of the pollutants exhibited significantly weekly and diurnal cycle in China. PM2.5, PM10, SO2, CO and NO2 presented the higher concentrations on weekdays than those at weekends, all of which showed the bimodal pattern with two peaks at late night (21:00–22:00) and in morning (9:00–10:00), respectively. However, the O3 concentration exhibited the highest value around 15:00. The statistical analysis suggested that the PM2.5, PM10, and SO2 concentrations were significantly associated with precipitation (Prec), atmosphere temperature (T), and wind speed (WS). The CO and NO2 concentrations displayed the significant relationship with T, while the O3 concentration was closely linked to the sunshine duration (Tsun) and relative humidity (RH). T and WS were major factors affecting the accumulation of PM and gaseous pollutants at a national scale. At a spatial scale, Prec and T played the important roles on the PM distribution in Northeast China, and the effect of Prec on CO concentration decreased from Southeast China to Northwest China. The results shown herein provide a scientific insight into the meteorology impacts on air pollution over China. [Display omitted] •The concentrations of air pollutants except O3 decreased significantly during 2015–2016.•T and WS were major factors for all of these air pollutants in China.•The effects of Prec and T on the PM displayed the higher values in Northeast China.