Novel Method of Quantifying Radioactive Cesium-Rich Microparticles (CsMPs) in the Environment from the Fukushima Daiichi Nuclear Power Plant

• Published in: Environmental science & technology 2018-06, Vol.52 (11), p.6390-6398
• Main Authors: Ikehara, Ryohei, Suetake, Mizuki, Komiya, Tatsuki, Furuki, Genki, Ochiai, Asumi, Yamasaki, Shinya, Bower, William R, Law, Gareth T. W, Ohnuki, Toshihiko, Grambow, Bernd, Ewing, Rodney C, Utsunomiya, Satoshi
• Format: Article
• Language: English
• Subjects: Airborne particulates; Autoradiography; Cesium; Chemical Sciences; Computational chemistry; Environmental impact; Mathematical models; Microparticles; Migration; Nuclear accidents; Nuclear energy; Nuclear power plants; Radioactive materials; Radioactivity; Radiochemistry; Regression coefficients; Soil surfaces; Soils
• ISSN: 0013-936X; 1520-5851
• DOI: 10.1021/acs.est.7b06693

Highly radioactive cesium-rich microparticles (CsMPs) were released from the Fukushima Daiichi nuclear power plant (FDNPP) to the surrounding environment at an early stage of the nuclear disaster in March of 2011; however, the quantity of released CsMPs remains undetermined. Here, we report a novel method to quantify the number of CsMPs in surface soils at or around Fukushima and the fraction of radioactivity they contribute, which we call “quantification of CsMPs” (QCP) and is based on autoradiography. Here, photostimulated luminescence (PSL) is linearly correlated to the radioactivity of various microparticles, with a regression coefficient of 0.0523 becquerel/PSL/h (Bq/PSL/h). In soil collected from Nagadoro, Fukushima, Japan, CsMPs were detected in soil sieved with a 114 μm mesh. There was no overlap between the radioactivities of CsMPs and clay particles adsorbing Cs. Based on the distribution of radioactivity of CsMPs, the threshold radioactivity of CsMPs in the size fraction of